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181.
William G. Sunda 《Marine Chemistry》1984,14(4):365-378
Equilibria between Chelex 100* and manganese, zinc and cadmium ions were used to determine the complexation of these trace metals in 36‰ Gulf Stream seawater at 25°C and pH 8.2. The method utilized radiotracers (54Mn, 65Zn, and 109Cd) to quantify trace metal adsorption from trace metal-amended seawater and from seawater containing a series of ethylenediaminetetracetate (EDTA)—metal ion buffers. Results were consistent with Chelex adsorption of both trace metal ions and trace metal—EDTA chelates. Equilibrium models fitted to the data were used to establish conditional stability constants for Chelex adsorption of manganese, zinc and cadmium ions and for adsorption of EDTA-chelates. These models also yielded ratios of free metal ions to total dissolved trace metal concentrations in seawater: 10−0.1 for manganese, 10−0.2 for zinc, and 10−1.5 for cadmium. Independent measurements with a cadmium ion-selective electrode also yielded a free: total cadmium ratio of 10−1.5. 相似文献
182.
We study the reaction of a global ocean–sea ice model to an increase of fresh water input into the northern North Atlantic under different surface boundary conditions, ranging from simple restoring of surface salinity to the use of an energy balance model (EBM) for the atmosphere. The anomalous fresh water flux is distributed around Greenland, reflecting increased melting of the Greenland ice sheet and increasing fresh water export from the Arctic Ocean. Depending on the type of surface boundary condition, the large circulation reacts with a slow-down of overturning and gyre circulations. Restoring of the total or mean surface salinity prevents a large scale redistribution of the salinity field that is apparent under mixed boundary conditions and with the EBM. The control run under mixed boundary conditions exhibits large and unrealistic oscillations of the meridional overturning. Although the reaction to the fresh water flux anomaly is similar to the response with the EBM, mixed boundary conditions must thus be considered unreliable. With the EBM, the waters in the deep western boundary current initially become saltier and a new fresh water mass forms in the north-eastern North Atlantic in response to the fresh water flux anomaly around Greenland. After an accumulation period of several decades duration, this new North East Atlantic Intermediate Water spreads towards the western boundary and opens a new southward pathway at intermediate depths along the western boundary for the fresh waters of high northern latitudes. 相似文献
183.
Quantum yield for the photochemical production of dissolved inorganic carbon in seawater 总被引:2,自引:0,他引:2
The direct photooxidation of coloured dissolved organic matter (CDOM) to dissolved inorganic carbon (DIC) may provide a significant sink for organic carbon in the ocean. To calculate the rate of this reaction on a global scale, it is essential to know its quantum yield, or photochemical efficiency. We have determined quantum yield spectra, φ(λ), (moles DIC/mole photons absorbed) for 14 samples of seawater from environments ranging from a turbid, eutrophic bay to the Gulf Stream. The spectra vary among locations, but can be represented quite well by three pooled spectra for zones defined by location and salinity: inshore φ(λ)=e−(6.66+0.0285(λ−290)); coastal φ(λ)=e−(6.36+0.0140(λ−290)); and open ocean φ(λ)=e−(5.53+0.00914(λ−290)). Production efficiency increases offshore, which suggests that the most highly absorbing and quickly faded terrestrial chromophores are not those directly responsible for DIC photoproduction. 相似文献
184.
The recent sea-ice reduction in the Arctic Ocean is not spatially uniform, but is disproportionally large around the Northwind
Ridge and Chukchi Plateau compared to elsewhere in the Canada Basin. In the Northwind Ridge region, Pacific Summer Water (PSW)
delivered from the Bering Sea occupies the subsurface layer. The spatial distribution of warm PSW shows a quite similar pattern
to the recent ice retreat, suggesting the influence of PSW on the sea-ice reduction. To understand the regionality of the
recent ice retreat, we examine the dynamics and timing of the delivery of the PSW into this region. Here, we adopt a two-layer
linearized potential vorticity equation to investigate the behavior of Rossby waves in the presence of a topographic discontinuity
in the high latitude ocean. The analytical results show a quite different structure from those of mid-latitude basins due
to the small value of β. Incident barotropic waves excited by the sea-ice motion with large annual variation can be scattered
into both barotropic and baroclinic modes at the discontinuity. Since the scattered baroclinic Rossby wave with annual frequency
cannot propagate freely, a strong baroclinic current near the topographic discontinuity is established. The seasonal variation
of current near the topographic discontinuity would cause a kind of selective switching system for shelf water transport into
the basin. In our simple analytical model, the enhanced northward transport of summer water and reduced northward transport
of winter water are well demonstrated. The present study indicates that these basic dynamics imply that a strengthening of
the surface forcing during winter in the Canada Basin could cause sea-ice reduction in the Western Arctic through the changes
of underlying Pacific Summer Water. 相似文献
185.
The upper layer (above 140 m depth) temperature in the western Philippine Sea near Taiwan was sampled using a coastal monitoring
buoy (CMB) with 15 attached thermistors during July 28–August 7, 2005. The data were collected every 10 min at 1, 3, 5, 10,
15, and 20 m using the CMB sensors, and every 15 sec at 15 different depths between 25 m and 140 m. Internal waves and solitons
were identified from the time-depth plot of the temperature field. Without the internal waves and solitons, the power spectra,
structure functions, and singular measures (representing the intermittency) of temperature field satisfy the power law with
multi-scale characteristics at all depths. The internal waves do not change the basic characteristics of the multifractal
structure. However, the internal solitons change the power exponent of the power spectra drastically, especially in the low
wave number domain; they also break down the power law of the structure function and increase the intermittency parameter.
The physical mechanisms causing these different effects need to be explored further. 相似文献
186.
Mesoscale features in the eastward extension of the Kuroshio were investigated using assimilation of TOPEX/POSEIDON (T/P)
data into a three-layer quasi-geostrophic model. The T/P data exhibited an elongated state of the southern recirculation gyre
in 1993–95 and 1997, between whose two periods the gyre had a contracted state in 1995–96. A few stationary eddies were located
in the southern gyre during the contracted state. The baroclinic instability, which was indicated by the phase shift from
the uppermost-to the lowest-layer anomalies toward the downstream side, was evident near the Kuroshio Extension (KE) path.
Since the instability never appeared in the artificial model without bottom topography, the topographic barrier for the eastward
flow in the lowest layer was a necessary condition for the instability. The instability synchronized with the transition in
the western region of the KE axis from the elongated to the contracted states. This evolution was interpreted as if the baroclinic
instability played some part in the KE states and was a trigger for the transition from the elongated to the contracted states. 相似文献
187.
Following our previous study (Sugimoto and Hanawa, 2005b), we further investigate the reason why reemergence of winter sea
surface temperature anomalies does not occur in the North Pacific eastern subtropical mode water (NPESTMW) area, despite its
occurrence in the North Pacific subtropical mode water and North Pacific central mode water areas. We use vertical temperature
and salinity profiles of the World Ocean Circulation Experiment Hydrographic Program and Argo floats with high vertical and
temporal resolution, together with heat flux data through the sea surface. We point out first that one of the causes for non-occurrence
of reemergence is that the thickness of NPESTMW is very thin. In addition to this basic cause, two major reasons are found:
a vigorous mixing in the lower portion of NPESTMW and less heat input from the atmosphere in the warming season. Since, in
the lower portion of NPESTMW and deeper, the stratification is favorable for salt-finger type convection to occur compared
with the other mode water areas, vigorous mixing takes place. This is confirmed by both a large Turner Angle there and the
existence of staircase structures in vertical temperature and salinity profiles. From the viewpoint of heat input, the NPESTMW
area gradually gains heat in the warming season compared with other mode water areas. As a result, NPESTMW cannot be capped
so quickly by the shallow summer mixed layer, and water properties of NPESTMW are to be gradually modified, even in the upper
portion. 相似文献
188.
A geomorphological and statistical analysis of slope canyons from the northern KwaZulu-Natal continental margin is documented
and compared with submarine canyons from the Atlantic margin of the USA. The northern KwaZulu-Natal margin is characterized
by increasing upslope relief, concave slope-gradient profiles and features related to upslope growth of the canyon forms.
Discounting slope-gradient profile, this morphology is strikingly similar to canyon systems of the New Jersey slope. Several
phases of canyon incision indicate that downslope erosion is also an important factor in the evolution of the northern KwaZulu-Natal
canyon systems. Despite the strong similarities between the northern KwaZulu-Natal and New Jersey slope-canyon systems, key
differences are evident: (1) the concavity of the northern KwaZulu-Natal slope, contrasting with the ∼linear New Jersey slope;
(2) the relative isolation of the northern KwaZulu-Natal canyons, rather than the dense clustering of the New Jersey canyons;
and (3) the absence of strongly shelf-breaching canyons along the northern KwaZulu-Natal margin. In comparison with the New
Jersey margin, we surmise a more youthful stage of canyon evolution, a result of either the canyons themselves being younger
or the formative processes being less active. Less complicated patterns of erosion resulting from reduced sediment availability
have developed in northern KwaZulu-Natal. The reduction in slope concavity on the New Jersey margin may be the result of grading
of the upper slope by intensive headward erosion, a process more subdued—or less evident—on the KwaZulu-Natal margin. 相似文献
189.
A complexometric titration technique was employed to measure the total capacity of a variety of marine organisms to adsorb Cu2+. Measured adsorption capacities were 0.22 meq g−1 for phytoplankton, 0.3–1.0 meq g−1 for macrophytes, 1.0–2.5 meq g−1 for zooplankton and 0.3 meq g−1 for suspended particulate matter. The capacity of these materials to adsorb Cu2+ was reduced significantly in the presence of Mg2+ at seawater concentrations. Competition between Mgt2+ and Cu2+ for adsorption sites at pH 6 is described by an average conditional equilibrium constant of 103.7. This constant is such that very little Cu2+ may be adsorbed onto particulates and marine phytoplankton in the presence of Mg2+. Further, primary productivity data and estimates of the detrital carbon sedimentation in Long Island Sound suggest that the flux of particulate carbon is insufficient to remove significant amounts of Cu from the water column to sediments by adsorption mechanisms. 相似文献
190.
The effects of scattering and resonance on the energy dissipation of an internal tide were investigated using a two-dimensional
model which is a reassembled version of the theoretical generation model devised by Rattray et al. (1969) for internal tide. The basic character of the scattering process at the step bottom was first investigated with a
wide shelf model. When the internal wave incited from a deep region (Region II) into the shallow shelf region (Region I),
a passing wave into the shallow region, a reflected wave into the deep region, and a beam-like wave, i.e. a scattered wave
(SW), emanated at the step bottom. The SW, which consists of the superposition of numerous internal modes, propagated upward/downward
into both regions. The general properties of the SW were well expressed around the shelf edge, even in the present model with
viscosity effect. The amplitude of the SW decreased dramatically when the depth of the velocity maximum of the incident internal
wave in Region II corresponded with the depth of the shelf edge. In the narrow shelf model, where the decay distance of the
internal wave in Region I is longer than the shelf width, the incident internal wave reflected at the coast to form a standing
wave. When the internal wave in Region I is enhanced by the resonance, the energy of the SW in Region II is also intensified.
Furthermore, the energy of the modes in Region II predominated when the velocity maximum is identical to that of the dominant
mode in Region I. These results suggest that the spatial scale of shelf region is a very important factor governing the energy
dissipation of the internal tide through reflection and scattering in a narrow shelf. 相似文献