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31.
STEPHAN BORRMANN REAS THOMAS VLADIMIR RUDAKOV VLADIMIR YUSHKOV BORIS LEPUCHOV TERRY DESHLER NIKOLAI VINNICHENKO VYACHESLAV KHATTATOV LEOPOLDO STEFANUTTI 《Tellus. Series B, Chemical and physical meteorology》2000,52(4):1088-1103
In‐situ aerosol measurements were performed in the northern hemispheric stratosphere up to altitudes of 21 km between 13 November 1996 and 14 January 1997, inside and outside of the polar vortex during the Airborne Polar Experiment (APE) field campaign. These are measurements of particle size distributions with a laser optical particle counter of the FSSP‐300 type operated during 9 flights on the Russian M‐55 high‐altitude research aircraft Geophysika. For specific flights, the FSSP‐300 measurements are compared with balloon‐borne data (launched from Kiruna, Sweden). It was found that the stratospheric aerosol content reached levels well below the background concentrations measured by the NASA operated ER‐2 in 1988/89 in the northern hemisphere. During the APE campaign, no PSC particle formation was observed at flight altitudes although the temperatures were below the NAT condensation point during one flight. The measured correlations between ozone and aerosol give an indication of the subsidence inside the 1996/97 polar vortex. Despite the lower aerosol content in the winter 1996/97 compared to the 1989 background, the heterogeneous reactivity of the aerosol (as calculated from the measured data with additional model input) is comparable. This is due to the dependency of the reactive uptake coefficients on the atmospheric water vapor content. Under the described assumptions the reaction rates on the background aerosol are significantly smaller than for competing gas phase chlorine activation, as can be expected for stratospheric background conditions especially inside the polar vortex. 相似文献
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LLOYD H. BURCKLE DAVIDA E. KELLOGG THOMAS B. KELLOGG JAMES L. FASTOOK 《Boreas: An International Journal of Quaternary Research》1997,26(1):55-60
The occurrence of diatoms (both marine and freshwater) in sediments beneath the West Antarctic Ice Sheet (WAIS) is suggestive of past ice-sheet collapse. However, it is not the only model explaining such occurrences. We propose another mechanism for introducing diatoms beneath ice sheets by considering the fate of a diatom placed (by eolian processes) on top of an ice sheet. Mathematical modeling indicates that the route the diatom will take through the ice sheet is dictated by the basal melting rate. If no basal melting takes place, flowlines will crop out at the ice-sheet margin. However, if basal melting is as low as 0.01 m/yr the trajectories of all Howlines except for those nearest the margin will intersect the bed, with those diatoms deposited near the dome reaching the bed about halfway down the Howband. Larger values of basal melting lead to the diatoms reaching the bed even faster and closer to the point of origin. In light of these results, the presence of diatoms in sediments beneath the WAIS does not lead to a unique solution; it is not necessary to invoke past ice-sheet collapse to account for their presence. 相似文献
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CALVIN J. HEUSSER THOMAS V. LOWELL LINDA E. HEUSSER ARTURO HAUSER BJ
RN G. ANDERSEN GEORGE H. DENTON 《第四纪科学杂志》1996,11(3):173-184
Palaeoecological studies carried out in the Chilean Lake District and Chilotan Archipelago (41°–43°S) record full-glacial and late-glacial pollen assemblages beginning just after 21000 and beetle assemblages after 18000, both sets extending until 10000 14C yr BP. Pollen records indicate that Subantarctic Parkland, the vegetation of the early millennia of record, changed after about 14000 yr BP to become open woodland and later North Patagonian Evergreen Forest. Assemblages of plants and beetles, responding more or less in unison to a strong rise in temperature (≥ 6°C), behaved in accord at around 14000 until 13000–12500 yr BP, the beetle fauna displaying a marked increase in obligate forest types. During full-glacial conditions (17400–16100 and 15300 and 14400 yr BP) and in the late-glacial interval (after about 13000 yr BP), however, climate evidently coerced populations dissimilarly, the pollen sequence showing an increase in plant taxa indicative of colder climate, whereas the beetle fauna underwent little or no variation. Contrasting climate modes implied by plants and beetles may be attributed to differential responses to apparent low-order temperature changes (≤ 2–3°C). 相似文献
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Temperatures of Granulite-facies Metamorphism: Constraints from Experimental Phase Equilibria and Thermobarometry Corrected for Retrograde Exchange 总被引:17,自引:7,他引:17
PATTISON DAVID R. M.; CHACKO THOMAS; FARQUHAR JAMES; MCFARLANE CHRISTOPHER R. M. 《Journal of Petrology》2003,44(5):867-900
This study assesses temperatures of formation of common granulitesby combining experimental constraints on the PT stabilityof granulite-facies mineral associations with a garnetorthopyroxene(GrtOpx) thermobarometry scheme based on Al-solubilityin Opx, corrected for late FeMg exchange. We appliedthis scheme to 414 granulites of mafic, intermediate and aluminousbulk compositions. Our findings suggest that granulites aremuch hotter than traditionally assumed and that the PTconditions of the amphibolitegranulite transition portrayedin current petrology textbooks are significant underestimatesby over 100°C. For aluminous and intermediate granulites,mean corrected temperatures based on our method are 890 ±17 and 841 ± 11°C, respectively (uncertainties reportedas 95% confidence limits on the mean), consistent with minimumtemperatures for orthopyroxene production by fluid-absent partialmelting in these bulk compositions. In contrast, mean temperaturesbased on GrtOpx FeMg exchange equilibria, usingthe same thermodynamic data, are 732 ± 22 and 723 ±11°C, respectively, well below the minimum temperaturesfor Opx stability. For mafic granulites, the mean correctedtemperature using our method is 816 ± 12°C, similarto the mean temperature of 793 ± 13°C from FeMgexchange. Reasons for the differences between the mafic granulitesand aluminousintermediate granulites are unclear butmay be due to the lower Al concentrations in Opx in the maficrocks and possible deficiencies in the thermodynamic modellingof these low concentrations. We discuss a number of well-knowngranulite terrains in the context of our findings, includingthe Adirondacks, the Acadian granulites of New England, theincipient charnockites of southern India and Sri Lanka, andthe Kerala Khondalite Belt. Our findings carry implicationsfor thermotectonic models of granulite formation. A computerprogram to perform our thermobarometry calculations, RCLC, isavailable from the Journal of Petrology website at http://www.petrology.oupjournals.orgor from the authors at http://www.geo.ucalgary.ca/~pattison/drm_pattison-rclc.htm. KEY WORDS: granulite-facies metamorphism; thermobarometry; garnet; orthopyroxene 相似文献
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By HEATHER D. GRAVEN † BRITTON B. STEPHENS THOMAS P. GUILDERSON TERESA L. CAMPOS DAVID S. SCHIMEL J. ELLIOTT CAMPBELL RALPH F. KEELING 《Tellus. Series B, Chemical and physical meteorology》2009,61(3):536-546
Measurements of Δ14 C in atmospheric CO2 are an effective method of separating CO2 additions from fossil fuel and biospheric sources or sinks of CO2 . We illustrate this technique with vertical profiles of CO2 and Δ14 C analysed in whole air flask samples collected above Colorado, USA in May and July 2004. Comparison of lower tropospheric composition to cleaner air at higher altitudes (>5 km) revealed considerable additions from respiration in the morning in both urban and rural locations. Afternoon concentrations were mainly governed by fossil fuel emissions and boundary layer depth, also showing net biospheric CO2 uptake in some cases. We estimate local industrial CO2 :CO emission ratios using in situ measurements of CO concentration. Ratios are found to vary by 100% and average 57 mole CO2 :1 mole CO, higher than expected from emissions inventories. Uncertainty in CO2 from different sources was ±1.1 to ±4.1 ppm for addition or uptake of −4.6 to 55.8 ppm, limited by Δ14 C measurement precision and uncertainty in background Δ14 C and CO2 levels. 相似文献
39.
Evaluation of the results of factor analysis of sets of spectroscopically detected chromatograms is carriedout by examining the shapes of the abstract factors.This is done either by visual inspection or by analysisof the power density spectra produced from them.Owing to constraints imposed by the column functionand the spectroscopic instrument function,the information content of the chromatograms necessarilyoccurs at low spatial frequencies.As a consequence,it appears as relatively broad features in the abstractchromatograms and as a peak in the low-frequency region of the corresponding power density plot.Onthe basis of examination of the power density distribution,a well-defined distinction is made betweenprimary and secondary abstract factors.The major uncertainty encountered in determining the numberof chemical components appears to arise from effects of contaminants in reagents. 相似文献
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