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Jae-Seok Kim Anna Liza Bais Sun-hee Kang Jaehoon Lee Kihong Park 《Journal of Atmospheric Chemistry》2011,68(3):251-263
Ammonia has a short residence time in the atmosphere and rapidly neutralizes acid gases that occur near its source, requiring a rapid measurement system for ammonia and particulate ammonium concentrations to better understand their sources, temporal variation of ammonia emissions, and the formation of secondary ammonium aerosols. A semi-continuous measurement system, consisting of a diffusion scrubber, a particle growth chamber, an air-liquid separator, and a fluorescent detector, was developed to determine both gaseous ammonia (NH3) and particulate ammonium (NH 4 + ) in PM2.5 in the ambient atmosphere of Gwangju, South Korea, during the months of March, April, July, and September of 2007. During the sampling periods, the average concentrations of ammonia and ammonium were found to be 2.33?±?1.29 μg/m3 and 1.89?±?0.99 μg/m3, respectively. Although the average gaseous ammonia concentration was highest in March, the particulate ammonium concentration was higher during the warmer season, reaching 2.08?±?1.07 μg/m3 and 2.32?±?0.94 μg/m3 in April and July, respectively, while only 1.68?±?0.61 μg/m3 in March and 1.24?±?0.99 μg/m3 in September. It is proposed that the higher availability of acid species during the warmer months produced a significant amount of particulate ammonium sulfate. Diurnal fluctuation of ammonia and ammonium during the warmer months showed that their peak time occurred at approximately 10:00 am. Both ammonia and ammonium concentrations were better correlated during the warmer months than during the cooler months. Further, the data suggest that the ammonia and ammonium were measured under well dispersed conditions, and multiple sources contributed to the ammonia at the sampling site. 相似文献
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Simulation of the anthropogenic aerosols over South Asia and their effects on Indian summer monsoon 总被引:4,自引:2,他引:2
Zhenming Ji Shichang Kang Dongfeng Zhang Chunzi Zhu Jia Wu Ying Xu 《Climate Dynamics》2011,36(9-10):1633-1647
A regional climate model coupled with a chemistry-aerosol model is employed to simulate the anthropogenic aerosols including sulfate, black carbon and organic carbon and their direct effect on climate over South Asia. The model is driven by the NCAR/NCEP re-analysis data. Multi-year simulations with half, normal and double emission fluxes are conducted. Results show that the model performs well in reproducing present climate over the region. Simulations of the aerosol optical depth and surface concentration of aerosols are also reasonable although to a less extent. The negative radiative forcing is found at the top of atmosphere and largely depended on emission concentration. Surface air temperature decreases by 0.1?C0.5°C both in pre-monsoon and monsoon seasons. The range and intensity of cooling areas enlarge while aerosol emission increases. Changes in precipitation are between ?25 and 25%. Different diversifications of rainfall are showed with three emission scenarios. The changes of precipitation are consistent with varieties of monsoon onset dates in pre-monsoon season. In the regions of increasing precipitation, monsoon onset is advanced and vice versa. In northeast India and Myanmar, aerosols lead the India summer monsoon onset advancing 1?C2 pentads, and delaying by 1?C2 pentads in central and southeast India. These changes are mainly caused by the anomaly of local Hadley circulations and enhancive precipitation. Tibetan Plateau played a crucial role in the circulation changes. 相似文献
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对一幢具有转换层的复杂退台式框架剪力墙高层建筑的1/35缩尺模型进行了模拟地震振动台试验,深入研究该结构的动力特性和地震反应特征.试验及理论分析表明:该结构的抗震性能基本满足现行规范要求;由于结构上部逐渐退台,因而结构顶部有较明显的鞭端效应;结构首层和结构转换层及其相邻层的剪力墙、转换层上下层柱是受力较大的区域,应当局... 相似文献
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为改善近断层地震动作用下隔震桥梁结构的抗震性能,基于Benchmark结构振动控制问题,研究附加黏滞阻尼器、磁流变(MR)阻尼器的组合隔震策略.非线性动力分析过程中,优化了黏滞阻尼器的阻尼系数和速度指数,并设计了分散模糊控制器来确定施加给磁流变阻尼器的电压.研究结果表明:采用黏滞阻尼器和磁流变阻尼器可提高隔震桥梁结构在... 相似文献