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581.
Microscopic and spectroscopic studies were conducted to assess mineral transformation processes in aqueous suspensions of illite (Il), vermiculite (Vm) and montmorillonite (Mt) that were subjected to weathering in a simulated high-level radioactive tank waste leachate (0.05 m AlT, 2 m Na+, 1 m NO3−, pH ∼14, Cs+ and Sr2+ present as co-contaminants). Time series (0 to 369 d) experiments were conducted at 298 K, with initial [Cs]0 and [Sr]0 concentrations from 10−5 to 10− mol kg−. Incongruent clay dissolution resulted in an accumulation of secondary aluminosilicate precipitates identified as nitrate-sodalite, nitrate-cancrinite and zeolite X, by molecular spectroscopy and electron microscopy (XRD, IR, NMR, SEM-EDS and TEM-EDS). Contaminant fate was dependent on competing uptake to parent clays and weathering products. TEM-EDS results indicated that high Il affinity for Cs was due to adsorption at frayed edge sites. The Il system also comprised Sr-rich aluminous precipitates after 369 d reaction time. In Mt systems, Cs and Sr were co-precipitated into increasingly recalcitrant spheroidal precipitates over the course of the experiment, whereas contaminant association with montmorillonite platelets was less prevalent. In contrast, Cs and Sr were found in association with weathered Vm particles despite the formation of spheroidal aluminosilicate precipitates that were comparable to those formed from Mt dissolution. 相似文献
582.
Earthquakes in Switzerland and surrounding regions during 2004 总被引:1,自引:0,他引:1
Manfred Baer Nicolas Deichmann Jochen Braunmiller Stephan Husen Donat F?h Domenico Giardini Philipp K?stli Urs KRadolfer Stefan Wiemer 《Eclogae Geologicae Helvetiae》2005,98(3):407-418
This report of the Swiss Seismological Service summarizes the seismic activity in Switzerland and surrounding regions during
2004. During this period, 677 earthquakes and 96 quarry blasts were detected and located in the region under consideration.
With 22 events with ML≥2.5, the seismic activity in the year 2004 was close to the average over the last 30 years. As in previous years, most of
the activity was concentrated in the Valais and in Graubünden. In addition, several moderate earthquakes occurred in the lower
crust below the northern Alpine foreland. Unusual was that five earthquakes were sufficiently strong to cause ground shaking
of intensity IV over large portions of the territory. Two were located in Switzerland (Liestal, ML 3.8, and Brugg, ML 4.0). The epicenters of the other three strong events were located outside Switzerland (Besan?on in the French Jura, ML 4.8, Waldkirch in southern Germany, ML 5.1, and Lago di Garda in northern Italy, ML 5.3). 相似文献
583.
We present detailed experimental results on the partitioning of rare earth elements (REE) between titanite and a range of different silicate melts. Our results show that Henry’s law of trace element partitioning depends on bulk composition, the available partners for heterovalent substitution, crystal composition, and melt composition. We illustrate that the partition coefficients for Sm depend very strongly on the bulk concentration of Sm in the system. The substitution mechanism, by which rare earth elements are incorporated into the crystal structure, plays an important role for trace element partitioning and also for the onset of Henry’s law. Our data show that there are clear differences between substitution mechanisms of major elements compared to elements which are present only as traces. Our experiments also clearly show that the onset of Henry’s law depends on the concentrations of the sum of all trace elements which are incorporated into the crystal by the same substitution mechanism. For geochemical modelling of magmatic processes involving titanite, and indeed other accessory phases, it is of crucial importance to first evaluate whether the REE, and other trace elements, are present as traces or as major elements, only then appropriate D values may be chosen. 相似文献
584.
Tobias Diehl Nicholas Deichmann John Clinton Stephan Husen Toni Kraft Katrin Plenkers Benjamin Edwards Carlo Cauzzi Clotaire Michel Philipp Kästli Stefan Wiemer Florian Haslinger Donat Fäh Urs Kradolfer Jochen Woessner 《Swiss Journal of Geoscience》2013,106(3):543-558
This report of the Swiss Seismological Service summarizes the seismic activity in Switzerland and surrounding regions during 2012. During this period, 497 earthquakes and 88 quarry blasts were detected and located in the region under consideration. With a total of only 13 events with ML ≥ 2.5, the seismic activity in the year 2012 was far below the average over the previous 37 years. Most noteworthy were the earthquake sequence of Filisur (GR) in January with two events of ML 3.3 and 3.5, the ML 4.2 and ML 3.5 earthquakes at a depth of 32 km below Zug in February and the ML 3.6 event near Vallorcine in October. The epicentral intensity of the ML 4.2 event close to Zug was IV, with a maximum intensity of V reached in a few areas, probably due to site amplification effects. 相似文献
585.
Xavi Gallach Ludovic Ravanel Markus Egli Dagmar Brandova Michael Schaepman Marcus Christl Stephan Gruber Philip Deline Julien Carcaillet François Pallandre 《Landslides》2018,15(10):1991-2000
Rockfalls and rock avalanches are a recurrent process in high mountain areas like the Mont Blanc massif. These processes are surveyed due to the hazard they present for infrastructure and alpinists. While rockfalls and rock avalanches have been documented for the last 150 years, we know very little about their frequency since the Last Glacial Maximum (LGM). In order to improve our understanding, it is imperative to date them on a longer timescale. A pilot campaign using Terrestrial Cosmogenic Nuclide (TCN) dating of five samples was carried out in 2006 at the Aiguille du Midi (3842 m a.s.l.). In 2011, a larger scale study (20 samples) was carried out in five other test sites in the Mont Blanc massif. This paper presents the exposure ages of the 2011 TCN study as well as the updated exposure ages of the 2006 study using newer TCN dating parameters. Most of these exposure ages lie within the Holocene but three ages are Pleistocene (59.87?±?6.10 ka for the oldest). A comparison of these ages with air temperature and glacier cover proxies explored the possible relationship between the most active rockfall periods and the warmest periods of the Holocene: two clusters of exposure ages have been detected, corresponding to the Middle Holocene (8.2–4.2 ka) and the Roman Warm Period (c. 2 ka) climate periods. Some recent rockfalls have also been dated (<?0.56 ka). 相似文献
586.
Beth Ellen Clark Richard P. Binzel Ellen S. Howell Edward A. Cloutis Maureen Ockert-Bell Phil Christensen Maria Antonietta Barucci Francesca DeMeo Dante S. Lauretta Harold Connolly Jr. Alicia Soderberg Carl Hergenrother Lucy Lim Josh Emery Michael Mueller 《Icarus》2011,216(2):462-475
We present reflectance spectra from 0.4 to 2.4 μm of Asteroid (101955) 1999 RQ36, the target of the OSIRIS-REx spacecraft mission. The visible spectral data were obtained at the McDonald Observatory 2.1-m telescope with the ES2 spectrograph. The infrared spectral data were obtained at the NASA Infrared Telescope Facility using the SpeX instrument. The average visible spectrum is combined with the average near-infrared wavelength spectrum to form a composite spectrum. We use three methods to constrain the compositional information in the composite spectrum of Asteroid (101955) 1999 RQ36 (hereafter RQ36). First, we perform a least-squares search for meteorite spectral analogs using 15,000 spectra from the RELAB database. Three most likely meteorite analogs are proposed based on the least-squares search. Next, six spectral parameters are measured for RQ36 and their values are compared with the ranges in parameter values of the carbonaceous chondrite meteorite classes. A most likely meteorite analog group is proposed based on the depth of overlap in parameter values. The results of the least-squares search and the parametric comparisons point to CIs and/or CMs as the most likely meteorite analogs for RQ36, and COs and CHs as the least likely. RQ36 has a spectrally “blue” continuum slope that is also observed in carbonaceous chondrites containing magnetite. We speculate that RQ36 is composed of a “CM1”-like material. Finally, we compare RQ36 to other B-type asteroids measured by Clark et al. (Clark, B.E. et al. [2010]. J. Geophys. Res. 115, E06005). The results of this comparison are inconclusive. RQ36 is comparable to Themis spectral properties in terms of its albedo, visible spectrum, and near-infrared spectrum from 1.1 to 1.45 μm. However, RQ36 is more similar to Pallas in terms of its near-infrared spectrum from 1.6 to 2.3 μm. Thus it is possible that B-type asteroids form a spectral continuum and that RQ36 is a transitional object, spectrally intermediate between the two end-members. This is particularly interesting because Asteroid 24 Themis was recently discovered to have H2O ice on the surface (Rivkin, A., Emery, J. [2010]. Nature 464, 1322–1323; Campins, H. et al. [2010a]. Nature 464, 1320–1321). 相似文献
587.
Julia ROSZJAR Knut METZLER Addi BISCHOFF Jean‐Alix BARRAT Thorsten GEISLER Richard C. GREENWOOD Ian A. FRANCHI Stephan KLEMME 《Meteoritics & planetary science》2011,46(11):1754-1773
Abstract– We report on the bulk chemical composition, petrology, oxygen isotopic composition, trace element composition of silicates, and degree of self‐irradiation damage on zircon grains of the eucrite Northwest Africa (NWA) 5073 to constrain its formation and postcrystallization thermal history, and to discuss their implications for the geologic history of its parent body. This unequilibrated and unbrecciated meteorite is a new member of the rare Stannern‐trend eucrites. It is mainly composed of elongated, zoned pyroxene phenocrysts up to 1.2 cm, plagioclase laths up to 0.3 cm in length, and is rich in mesostasis. The latter contains zircon grains up to 30 μm in diameter, metal, sulfide, tridymite, and Ca‐phosphates. Textural observations and silicate compositions, coupled with the occurrence of extraordinary Fe‐rich olivine veins that are restricted to large pyroxene laths, indicate that NWA 5073 underwent a complex thermal history. This is also supported by the annealed state of zircon grains inferred from μ‐Raman spectroscopic measurements along with U and Th data obtained by electron probe microanalyses. 相似文献
588.
Nicholas Deichmann John Clinton Stephan Husen Benjamin Edwards Florian Haslinger Donat Fäh Domenico Giardini Philipp Kästli Urs Kradolfer Iris Marschall Stefan Wiemer 《Swiss Journal of Geoscience》2010,103(3):535-549
This report of the Swiss Seismological Service summarizes the seismic activity in Switzerland and surrounding regions during 2009. During this period, 450 earthquakes and 68 quarry blasts were detected and located in the region under consideration. The three strongest events occurred about 15 km NW of Basel in southern Germany (ML 4.2), near Wildhaus in the Toggenburg (ML 4.0) and near Bivio in Graubünden (ML 3.5). Although felt by the population, they were not reported to have caused any damage. With a total of 24 events with ML ≥ 2.5, the seismic activity in the year 2009 was close to the average over the previous 34 years. 相似文献