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71.
星叶石族矿物红外光谱研究 总被引:4,自引:0,他引:4
在新测定的星叶石晶体结构资料的基础上,对星叶石矿物进行了详细和红外光谱研究,对比了单斜及三斜星叶石的红光谱特征,并对星叶石中工外吸收振动的归属问题进行了讨论。 相似文献
72.
The broadband diffuse radiation method is improved to retrieve the aerosol refractive index imaginary part (AIP) and broadband (400-1000 nm mean) single scattering albedo (SSA). In this method, four sets of SSA selection criteria are proposed for quality control. The method is used to retrieve AIP, SSA and absorptive optical thickness (AbOT) from routine hourly-exposed pyrheliometer and paranometer measurements over 11 sites (meteorological observatories) in China during 1998-2003. Apart from one suburban site (Ejin Qi), the other urban sites are all located around big or medium cities. As shown in the retrieval results, annual mean SSA during 1998-2003 changes from 0.941 (Wuhan) to 0.849 (Lanzhou), and AIP from 0.0054 to 0.0203. The 11-site average annual mean SSA and AIP are 0.898 and 0.0119, respectively. SSA during winter is smaller for most sites. There is an evidently positive correlation between SSA and aerosol optical thickness (AOT) for all sites. There is also a positive correlation between SSA and relative humidity for most sites, but a negative correlation for a few sites, such as Kashi and ǚrǚmqi in Northwest China. 相似文献
73.
An advanced one-dimensional radiative-convective model (RCM) is used to estimate the past, present and fu-ture climatic forcings induced by greenhouse gases of anthropogenic origin, such as CO2, CH4, N2O and CFCs, in this paper. The results show that the decadal climatic forcing for the last decade is one-order bigger than that prior to the year 1900, and in the case of no control on the emission of the greenhouse gases the climatic forcing for the year 2100 will be almost 4 times as much as now. 相似文献
74.
The climate–population relationship has long been conceived. Although the topic has been repeatedly investigated, most of
the related works are Eurocentric or qualitative. Consequently, the relationship between climate and population remains ambiguous.
In this study, fine-grained temperature reconstructions and historical population data sets have been employed to statistically
test a hypothesized relationship between temperature change and population growth (i.e., cooling associated with below average
population growth) in China over the past millennium. The important results were: (1) Long-term temperature change significantly
determined the population growth dynamics of China. However, spatial variation existed, whilst population growth in Central
China was shown to be responsive to both long- and short-term temperature changes; in marginal areas, population growth was
only sensitive to short-term temperature fluctuations. (2) Temporally, the temperature–population relationship was obscured
in some periods, which was attributable to the factors of drought and social buffers. In summary, a temperature–population
relationship was mediated by geographic factors, the aridity threshold, and social factors. Given the upcoming threat posed
by climate change to human societies, this study seeks to improve our knowledge and understanding of the climate–society relationship. 相似文献
75.
Adequate high-quality data on three-dimensional velocities in the atmospheric surface layer (height \(\delta \)) were acquired in the field at the Qingtu Lake Observation Array. The measurement range occupies nearly the entire logarithmic layer from approximately \(0.006\delta \)–\(0.2\delta \). The turbulence intensity and eddy structures of the velocity fluctuations in the logarithmic region were primarily analyzed, and their variations in the z (wall-normal) direction were revealed. The primary finding was that the turbulent intensity of wall-normal velocity fluctuations exhibits a sharp upswing in the logarithmic region, which differs from classic scaling law and laboratory results. The upswing of the wall-normal turbulence intensity in the logarithmic region is deemed to be linear based on an ensemble of 20 sets of data. In addition, the wall-normal extent of the correlated structures and wall-normal spectra were compared to low Reynolds number results in the laboratory. 相似文献
76.
UV attenuation in the cloudy atmosphere 总被引:1,自引:0,他引:1
Jianhui Bai 《Journal of Atmospheric Chemistry》2009,62(3):211-228
Ultraviolet (UV) energy absorption plays a very important role in the Earth–atmosphere system. Based on observational data
for Beijing, we suggest that some atmospheric constituents utilize or transfer UV energy in chemical and photochemical (C&P) reactions, in addition to those which absorb UV energy directly. These constituents are primarily volatile organic compounds
(VOCs) emitted from both vegetative and anthropogenic sources. The total UV energy loss in the cloudy atmosphere for Beijing
in 1990 was 78.9 Wm−2. This attenuation was caused by ozone (48.3 Wm−2), other compounds in the atmosphere (26.6 Wm−2) and a scattering factor (4.0 Wm−2). Our results for a cloudy atmosphere in the Beijing area show that the absorption due to these other compounds occurs largely
through the mediation of water vapor. This fraction of energy loss has not been fully accounted for in previous models. Observations
and previous models results suggest that 1) a cloudy atmosphere absorbs 25∼30 Wm−2 more solar shortwave radiation than models predict; and 2) aerosols can significantly decrease the downward mean UV-visible
radiation and the absorbed solar radiation at the surface by up to 28 and 23 Wm−2, respectively. Thus, quantitative study of UV and visible absorption by atmospheric constituents involved in homogeneous
and heterogeneous C&P reactions is important for atmospheric models. 相似文献
77.
José Luís Argaín Miguel A. C. Teixeira Pedro M. A. Miranda 《Boundary-Layer Meteorology》2017,165(1):145-160
A method is proposed for estimating the surface-layer depth \((z_s)\) and the friction velocity \((u_*)\) as a function of stability (here quantified by the Obukhov length, L) over the complete range of unstable flow regimes. This method extends that developed previously for stable conditions by Argaín et al. (Boundary-Layer Meteorol 130:15–28, 2009), but uses a qualitatively different approach. The method is specifically used to calculate the fractional speed-up \((\varDelta S)\) in flow over a ridge, although it is suitable for more general boundary-layer applications. The behaviour of \(z_s \left( L\right) \) and \(u_*\left( L\right) \) as a function of L is indirectly assessed via calculation of \(\varDelta S\left( L\right) \) using the linear model of Hunt et al. (Q J R Meteorol Soc 29:16–26, 1988) and its comparison with the field measurements reported in Coppin et al. (Boundary-Layer Meteorol 69:173–199, 1994) and with numerical simulations carried out using a non-linear numerical model, FLEX. The behaviour of \(\varDelta S\) estimated from the linear model is clearly improved when \(u_*\) is calculated using the method proposed here, confirming the importance of accounting for the dependences of \(z_s\left( L \right) \) and \(u_*\left( L \right) \) on L to better represent processes in the unstable boundary layer. 相似文献
78.
Juan Huang Yanli Feng Jian Li Bin Xiong Jialiang Feng Sheng Wen Guoying Sheng Jiamo Fu Minghong Wu 《Journal of Atmospheric Chemistry》2008,61(1):1-20
The levels of carbonyl compounds in Shanghai ambient air were measured in five periods from January 2007 to October 2007 (covering
winter, high-air-pollution days, spring, summer and autumn). A total of 114 samples were collected and eighteen carbonyls
were identified. Formaldehyde, acetaldehyde and acetone were the most abundant carbonyls and their mean concentrations of
19.40 ± 12.00, 15.92 ± 12.07 and 11.86 ± 7.04 μg m−3 respectively, in the daytime for five sampling periods. Formaldehyde and acetaldehyde showed similar diurnal profiles with
peak mixing ratios in the morning and early afternoon during the daytime. Their mean concentrations were highest in summer
and lowest in winter. Acetone showed reversed seasonal variation. The high molecular weight (HMW, ≥C5) carbonyls also showed
obvious diurnal variations with higher concentrations in the daytime in summer and autumn, while they were all not detected
in winter. Formaldehyde and acetaldehyde played an important role in removing OH radicals in the atmosphere, but the contribution
of acetone was below 1%. The carbonyls levels in high-air-pollution days were reported. More carbonyl species with higher
concentrations were found in high-air-pollution days than in spring. These carbonyls were transported with other pollutants
from north and northwest in March 27 to April 2, 2007 and then mixed with local sources. Comparing with Beijing and Guangzhou,
the concentrations of formaldehyde and acetaldehyde in Shanghai were the highest, which indicated that the air pollution in
Shanghai was even worse than expected. 相似文献
79.
General purpose Computational Fluid Dynamics (CFD) solvers are frequently used in small-scale urban pollution dispersion simulations
without a large extent of ver- tical flow. Vertical flow, however, plays an important role in the formation of local breezes,
such as urban heat island induced breezes that have great significance in the ventilation of large cities. The effects of
atmospheric stratification, anelasticity and Coriolis force must be taken into account in such simulations. We introduce a
general method for adapting pressure based CFD solvers to atmospheric flow simulations in order to take advantage of their
high flexibility in geometrical modelling and meshing. Compressibility and thermal stratification effects are taken into account
by utilizing a novel system of transformations of the field variables and by adding consequential source terms to the model
equations of incompressible flow. Phenomena involving mesoscale to microscale coupled effects can be analyzed without model
nesting, applying only local grid refinement of an arbitrary level. Elements of the method are validated against an analytical
solution, results of a reference calculation, and a laboratory scale urban heat island circulation experiment. The new approach
can be applied with benefits to several areas of application. Inclusion of the moisture transport phenomena and the surface
energy balance are important further steps towards the practical application of the method. 相似文献
80.
年代际气候变率问题的研究 总被引:7,自引:3,他引:7
对年代际气候变率的研究工作和主要结果作了综合评述,并对该领域的研究前景作了一定的阐述。 相似文献