工业部门污染物治理协同控制温室气体效应评价——基于重庆市的实证分析

以高能耗为主要特征的工业部门是大气污染物和温室气体的重要排放源.为推动协同管控,文中结合生态环境部在重庆市组织开展的试点工作,对工业企业NOx污染治理协同控制温室气体的效应进行了量化分析.结果表明,以末端治理为手段的NOx治理措施协同控制温室气体的效果为负,即工业企业去除1 t NOx会直接或间接增加CO2排放1.81...     

暴雨模拟中多普勒雷达径向速度变分同化的应用

针对2008年6月广东地区的一次强降雨过程,利用WRF中尺度数值模式及其三维变分同化系统(WRF-3DVAR),进行了多普勒雷达径向速度变分同化对暴雨过程模拟效果影响研究。结果表明:WRF-3DVAR能够有效地同化多普勒雷达径向速度,同化后的主要影响在于改进了初始动力场,使得初始场包含有更详尽的中尺度特征信息,进而显著提高模式对广东局地暴雨过程的模拟效果。在高分辨率中尺度数值模式中有效地利用多普勒天气雷达资料,是提高中尺度降雨预报的关键。     

Some Insights into Topographic,Elastic and Self-gravitation Interaction in Modelling Ground Deformation and Gravity Changes in Active Volcanic Areas

Surface displacements and gravity changes due to volcanic sources are influenced by medium properties. We investigate topographic, elastic and self-gravitation interaction in order to outline the major factors that are significant in data modelling. While elastic-gravitational models can provide a suitable approximation to problems of volcanic loading in areas where topographic relief is negligible, for prominent volcanoes the rough topography could affect deformation and gravity changes to a greater extent than self-gravitation. This fact requires the selection, depending on local relief, of a suitable model for use in the interpretation of surface precursors of volcanic activity. We use the three-dimensional Indirect Boundary Element Method to examine the effects of topography on deformation and gravity changes in models of magma chamber inflation/deflation. Topography has a significant effect on predicted surface deformation and gravity changes. Both the magnitude and pattern of the geodetic signals are significantly different compared to half-space solutions. Thus, failure to account for topographic effects in areas of prominent relief can bias the estimate of volcanic source parameters, since the magnitude and pattern of deformation and gravity changes depend on such effects.     

Absorption properties of urban/suburban aerosols in China

The broadband diffuse radiation method is improved to retrieve the aerosol refractive index imaginary part （AIP） and broadband （400-1000 nm mean） single scattering albedo （SSA）. In this method, four sets of SSA selection criteria are proposed for quality control. The method is used to retrieve AIP, SSA and absorptive optical thickness （AbOT） from routine hourly-exposed pyrheliometer and paranometer measurements over 11 sites （meteorological observatories） in China during 1998-2003. Apart from one suburban site （Ejin Qi）, the other urban sites are all located around big or medium cities. As shown in the retrieval results, annual mean SSA during 1998-2003 changes from 0.941 （Wuhan） to 0.849 （Lanzhou）, and AIP from 0.0054 to 0.0203. The 11-site average annual mean SSA and AIP are 0.898 and 0.0119, respectively. SSA during winter is smaller for most sites. There is an evidently positive correlation between SSA and aerosol optical thickness （AOT） for all sites. There is also a positive correlation between SSA and relative humidity for most sites, but a negative correlation for a few sites, such as Kashi and ǚrǚmqi in Northwest China.     

Cloud Variations under Subtropical High Conditions

The cloud variations under subtropical high(STH) conditions during summers over a ten-year period are studied using combined data from the International Satellite Cloud Climatology Project and the National Centers for Environmental Prediction.The results reveal that clouds mainly experience an isolated evolution in the STHs,which is designated in this study by the 1540 gpm geopotential lines at 850 hPa.In the STH domain throughout the Northern Hemisphere,the average amount of total clouds exceeds 30%.Low clouds dominate in the STH domain,contributing over 60%of total cloud amount within the Pacific subtropical high and over 40%within the Atlantic subtropical high.The prevalence of low clouds in above regions is determined by the circulation pattern around 150°-180°E and 850 hPa,which suppresses both the upward development of the cloud tops and the water vapor divergences near the surface.Furthermore,clouds present great geographical incoherence within the STH domain.In the eastern STHs,the amount of middle and low clouds increases to peak in the early morning and decreases to a trough in the afternoon,while the amount of high clouds remains stable throughout the day.Conversely,in the western STHs,the diurnal amplitude of low and middle clouds is less than three,while high clouds dramatically reach the maximum in the afternoon and drop to the minimum in the evening.Among the nine cloud categories,stratocumulus clouds with greater optical thickness account for the most under STH conditions,no matter their occurrence or amount,causing more shortwave cloud radiative forcing to cool the local atmosphere and surface as a consequence.     

Extreme precipitation events identified using detrended fluctuation analysis (DFA) in Anhui,China

Extreme weather events include unusual, severe or unseasonal weather, and weather at the extremes of the historical distribution. They have become more frequent and intense under global warming, especially in mid-latitude areas. They bring about great agricultural and economic losses. It is important to define the threshold of extreme weather event because it is the starting point of extreme weather event research, though it has been of seldom concern. Taking extreme precipitation events in Anhui, China as an example, the detrended fluctuation analysis (DFA) method is introduced to define the threshold of extreme weather events. Based on it, the spatial and temporal distributions of extreme precipitation events are analyzed. Compared to the traditional percentile method, DFA is based on the long-term correlation of time series. Thresholds calculated by DFA are much higher than the 99th percentile and the values are higher in the south and lower in the north. This spatial pattern is similar to the annual precipitation spatial pattern. There is an obvious increasing trend in the number of days with extreme precipitation, especially after the 1980s. This observation supports the point that more extreme events happen under global warming.     

Climatic change and Chinese population growth dynamics over the last millennium

The climate–population relationship has long been conceived. Although the topic has been repeatedly investigated, most of the related works are Eurocentric or qualitative. Consequently, the relationship between climate and population remains ambiguous. In this study, fine-grained temperature reconstructions and historical population data sets have been employed to statistically test a hypothesized relationship between temperature change and population growth (i.e., cooling associated with below average population growth) in China over the past millennium. The important results were: (1) Long-term temperature change significantly determined the population growth dynamics of China. However, spatial variation existed, whilst population growth in Central China was shown to be responsive to both long- and short-term temperature changes; in marginal areas, population growth was only sensitive to short-term temperature fluctuations. (2) Temporally, the temperature–population relationship was obscured in some periods, which was attributable to the factors of drought and social buffers. In summary, a temperature–population relationship was mediated by geographic factors, the aridity threshold, and social factors. Given the upcoming threat posed by climate change to human societies, this study seeks to improve our knowledge and understanding of the climate–society relationship.     

UV attenuation in the cloudy atmosphere

Ultraviolet (UV) energy absorption plays a very important role in the Earth–atmosphere system. Based on observational data for Beijing, we suggest that some atmospheric constituents utilize or transfer UV energy in chemical and photochemical (C&P) reactions, in addition to those which absorb UV energy directly. These constituents are primarily volatile organic compounds (VOCs) emitted from both vegetative and anthropogenic sources. The total UV energy loss in the cloudy atmosphere for Beijing in 1990 was 78.9 Wm⁻². This attenuation was caused by ozone (48.3 Wm⁻²), other compounds in the atmosphere (26.6 Wm⁻²) and a scattering factor (4.0 Wm⁻²). Our results for a cloudy atmosphere in the Beijing area show that the absorption due to these other compounds occurs largely through the mediation of water vapor. This fraction of energy loss has not been fully accounted for in previous models. Observations and previous models results suggest that 1) a cloudy atmosphere absorbs 25∼30 Wm⁻² more solar shortwave radiation than models predict; and 2) aerosols can significantly decrease the downward mean UV-visible radiation and the absorbed solar radiation at the surface by up to 28 and 23 Wm⁻², respectively. Thus, quantitative study of UV and visible absorption by atmospheric constituents involved in homogeneous and heterogeneous C&P reactions is important for atmospheric models.     

Estimation of Surface-Layer Scaling Parameters in the Unstable Boundary Layer: Implications for Orographic Flow Speed-Up

A method is proposed for estimating the surface-layer depth \((z_s)\) and the friction velocity \((u_*)\) as a function of stability (here quantified by the Obukhov length, L) over the complete range of unstable flow regimes. This method extends that developed previously for stable conditions by Argaín et al. (Boundary-Layer Meteorol 130:15–28, 2009), but uses a qualitatively different approach. The method is specifically used to calculate the fractional speed-up \((\varDelta S)\) in flow over a ridge, although it is suitable for more general boundary-layer applications. The behaviour of \(z_s \left( L\right) \) and \(u_*\left( L\right) \) as a function of L is indirectly assessed via calculation of \(\varDelta S\left( L\right) \) using the linear model of Hunt et al. (Q J R Meteorol Soc 29:16–26, 1988) and its comparison with the field measurements reported in Coppin et al. (Boundary-Layer Meteorol 69:173–199, 1994) and with numerical simulations carried out using a non-linear numerical model, FLEX. The behaviour of \(\varDelta S\) estimated from the linear model is clearly improved when \(u_*\) is calculated using the method proposed here, confirming the importance of accounting for the dependences of \(z_s\left( L \right) \) and \(u_*\left( L \right) \) on L to better represent processes in the unstable boundary layer.     

Characteristics of carbonyl compounds in ambient air of Shanghai,China

The levels of carbonyl compounds in Shanghai ambient air were measured in five periods from January 2007 to October 2007 (covering winter, high-air-pollution days, spring, summer and autumn). A total of 114 samples were collected and eighteen carbonyls were identified. Formaldehyde, acetaldehyde and acetone were the most abundant carbonyls and their mean concentrations of 19.40 ± 12.00, 15.92 ± 12.07 and 11.86 ± 7.04 μg m⁻³ respectively, in the daytime for five sampling periods. Formaldehyde and acetaldehyde showed similar diurnal profiles with peak mixing ratios in the morning and early afternoon during the daytime. Their mean concentrations were highest in summer and lowest in winter. Acetone showed reversed seasonal variation. The high molecular weight (HMW, ≥C5) carbonyls also showed obvious diurnal variations with higher concentrations in the daytime in summer and autumn, while they were all not detected in winter. Formaldehyde and acetaldehyde played an important role in removing OH radicals in the atmosphere, but the contribution of acetone was below 1%. The carbonyls levels in high-air-pollution days were reported. More carbonyl species with higher concentrations were found in high-air-pollution days than in spring. These carbonyls were transported with other pollutants from north and northwest in March 27 to April 2, 2007 and then mixed with local sources. Comparing with Beijing and Guangzhou, the concentrations of formaldehyde and acetaldehyde in Shanghai were the highest, which indicated that the air pollution in Shanghai was even worse than expected.