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351.
352.
Mustafa Yücel Sergey K. Konovalov Tommy S. Moore Christopher P. Janzen George W. Luther 《Chemical Geology》2010,269(3-4):364-375
We report solid phase sulfur speciation of six cores from sediments underlying oxic, suboxic and anoxic-sulfidic waters of the Black Sea. Our dataset includes the five sulfur species [pyrite-sulfur, acid volatile sulfides (AVS), zerovalent sulfur (S(0)), organic polysulfides (RSx), humic sulfur] together with reactive iron and manganese, as quantified by dithionite extraction, and total organic carbon. Pyrite – sulfur was the major phase in all cores [200-400 µmol (g dry wt)- 1] except for the suboxic core. However, zerovalent sulfur and humic sulfur also reached very significant levels: up to about 109 and 80 µmol (g dry wt)- 1, respectively. Humic sulfur enrichment was observed in the surface fluff layers of the eastern central basin sediments where Unit-1 type depositional conditions prevail. Elemental sulfur accumulated as a result of porewater sulfide oxidation by reactive iron oxides in turbidities from the anoxic basin margin and western central basin sediments. The accumulation of elemental sulfur to a level close to that of pyrite-S in any part of central Black Sea sediments has never been reported before and our finding indicates deep basin turbidites prevent the build-up of dissolved sulfide in the sediment. This process also contributes to diagenetic pyrite formation whereas in the non-turbiditic parts of the deep basin water column formed (syngenetic) pyrite dominates the sulfur inventory. In slope sediments under suboxic waters, organic sulfur (humic sulfur + organic polysulfides) account for 33-42% of total solid phase S, indicating that the suboxic conditions favor organosulfur formation. Our study shows that the interactions between depositional patterns (Unit 1 vs. turbidite), redox state of overlying waters (oxic-suboxic-sulfidic) and organic matter content determine sulfur speciation and enable the accumulation of elemental sulfur and organic sulfur species close to a level of pyrite-S. 相似文献
353.
Nadezhda Alexandrovna Krivolutskaya Alexandr Vladimirovich Sobolev Sergey Grigor’evich Snisar Bronislav Iosiphovich Gongalskiy Dmitry Vladimirovich Kuzmin Folkmar Hauff Irina Nikolaevna Tushentsova Natalya Mikhailovna Svirskaya Natalya Nikolaevna Kononkova Tatyana B. Schlychkova 《Mineralium Deposita》2012,47(1-2):69-88
We report new data on the stratigraphy, mineralogy and geochemistry of the rocks and ores of the Maslovsky Pt–Cu–Ni sulfide deposit which is thought to be the southwestern extension of the Noril’sk 1 intrusion. Variations in the Ta/Nb ratio of the gabbro-dolerites hosting the sulfide mineralization and the compositions of their pyroxene and olivine indicate that these rocks were produced by two discrete magmatic pulses, which gave rise to the Northern and Southern Maslovsky intrusions that together host the Maslovsky deposit. The Northern intrusion is located inside the Tungusska sandstones and basalt of the Ivakinsky Formation. The Southern intrusion cuts through all of the lower units of the Siberian Trap tuff-lavas, including the Lower Nadezhdinsky Formation; demonstrating that the ore-bearing intrusions of the Noril’sk Complex post-date that unit. Rocks in both intrusions have low TiO2 and elevated MgO contents (average mean TiO2 <1 and MgO?=?12?wt.%) that are more primitive than the lavas of the Upper Formations of the Siberian Traps which suggests that the ore-bearing intrusions result from a separate magmatic event. Unusually high concentrations of both HREE (Dy+Yb+Er+Lu) and Y (up to 1.2 and 2.1?ppm, respectively) occur in olivines (Fo79.5 and 0.25% NiO) from picritic and taxitic gabbro-dolerites with disseminated sulfide mineralization. Thus accumulation of HREE, Y and Ni in the melts is correlated with the mineral potential of the intrusions. The TiO2 concentration in pyroxene has a strong negative correlation with the Mg# of both host mineral and Mg# of host rock. Sulfides from the Northern Maslovsky intrusion are predominantly chalcopyrite–pyrrhotite–pentlandite with subordinate and minor amounts of cubanite, bornite and millerite and a diverse assemblage of rare precious metal minerals including native metals (Au, Ag and Pd), Sn–Pd–Pt–Bi–Pb compounds and Fe–Pt alloys. Sulfides from the Southern Maslovsky intrusion have δ 34S?=?5–6‰ up to 10.8‰ in two samples whereas the country rock basalt have δ 34S?=?3–4‰, implying there was no in situ assimilation of surrounding rocks by magmas. 相似文献
354.
Fast data assimilation using a nonlinear Kalman filter and a model surrogate: An application to the Columbia River estuary 总被引:3,自引:0,他引:3
Sergey Frolov Antnio M. Baptista Todd K. Leen Zhegdong Lu Rudolph van der Merwe 《Dynamics of Atmospheres and Oceans》2009,48(1-3):16
A fast and adjoint-free nonlinear data assimilation (DA) system was developed to simulate 3D baroclinic circulation in estuaries, leveraging two recently developed technologies: (1) a nonlinear model surrogate that executes forward simulation three orders of magnitude faster than a forward numerical circulation code and (2) a nonlinear extension to the reduced-dimension Kalman filter that estimates the state of the model surrogate. The noise sources in the Kalman filter were calibrated using empirical cross-validation and accounted for errors in model and model forcing.The DA system was applied to assimilate in situ measurements of water levels, salinities, and temperatures in simulations of the Columbia River estuary. To validate the DA results, we used a combination of cross-validation studies, process-oriented studies, and tests of statistical and dynamical consistency. The validation studies showed that DA improved the representation of several important processes in the estuary, including nonlinear tidal propagation, salinity intrusion, estuarine residual circulation, heat balance, and response of the estuary to coastal winds. 相似文献
355.
Mort Webster Andrei P. Sokolov John M. Reilly Chris E. Forest Sergey Paltsev Adam Schlosser Chien Wang David Kicklighter Marcus Sarofim Jerry Melillo Ronald G. Prinn Henry D. Jacoby 《Climatic change》2012,112(3-4):569-583
Although policymaking in response to the climate change threat is essentially a challenge of risk management, most studies of the relation of emissions targets to desired climate outcomes are either deterministic or subject to a limited representation of the underlying uncertainties. Monte Carlo simulation, applied to the MIT Integrated Global System Model (an integrated economic and earth system model of intermediate complexity), is used to analyze the uncertain outcomes that flow from a set of century-scale emissions paths developed originally for a study by the U.S. Climate Change Science Program. The resulting uncertainty in temperature change and other impacts under these targets is used to illustrate three insights not obtainable from deterministic analyses: that the reduction of extreme temperature changes under emissions constraints is greater than the reduction in the median reduction; that the incremental gain from tighter constraints is not linear and depends on the target to be avoided; and that comparing median results across models can greatly understate the uncertainty in any single model. 相似文献
356.
Zhang Yinglong Joseph Wu Chin Anderson Joshua Danilov Sergey Wang Qiang Liu Yuli Wang Qian 《Ocean Dynamics》2023,73(3-4):219-230
Ocean Dynamics - We develop a single-class ice and snow model embedded inside a 3D hydrodynamic model on unstructured grids and apply it to lake studies using highly variable mesh resolution. The... 相似文献
357.
The electric inversion technique reconstructs the subsurface medium distribution from acquired data. On the basis of electric inversion, objects buried under the earth or seabed, such as pipelines and unexploded ordnance, are detected and located in a contactless manner. However, the process of accurately reconstructing the shape of the target object is challenging because electric inversion is a nonlinear and ill-posed problem. In this work, we present an inverse multiquadric (IMQ) regularization method based on the level set function for reconstructing buried pipelines. In the case of locating underwater objects, the unknown inversion area is split into two parts, the background and the pipeline with known conductivity. The geometry of the pipeline is represented based on the level set function for achieving a noiseless inversion image. To obtain a binary image, the IMQ is used as the regularization term, which 'pushes' the level set function away from 0. We also provide an appropriate method to select the bandwidth and regularization pa-rameters for the IMQ regularization term, resulting in reconstructed images with sharp edges. The simulation results and analysis show that the proposed method performs better than classical inversion methods. 相似文献