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601.
M. N. Taran K. Langer A. N. Platonov V. Indutny 《Physics and Chemistry of Minerals》1994,21(6):360-372
The effect of raising temperature on spin-allowed dd-transitions of octahedral Cr3+ was studied for various point symmetries of the Cr3+-bearing structural sites, i.e. 3 m and 3 with inversion center in spinel and garnets, respectively, or 32, 3, 2 and 1, lacking the inversion centre, in beryl, corundum, diopside and topaz, respectively. For this purpose, crystals of Cr3+-bearing spinel, pyrope, andradite, grossular, uvarovite, emerald, ruby, diopside and topaz were analyzed by microprobe, oriented, and measured in polarized radiation (except for the cubic minerals) in the spectral range 30 000 to 11 100 cm-1 and at temperatures between 77 and 797 K. The evaluation of the intensities, half widths, and energy positions of bands due to Cr3+-transitions derived from
4
A
2g
4
T
2g
(F) and
4
T
1g
(F) as well as of Dq- and B-values derived, had the following results:In all cases, red shift of the above bands and, hence, independent on the site symmetry of Cr3+, decreases in the Dq-values were obtained. The dependcies of Dq on T are nearly linear above room temperature and amount between -1.6% in topaz and -5.1% in pyrope in the temperature range studied. From this, values for the local thermal expansion of the Cr3+-centered octahedra,
loc, were derived on the basis of the R
M-0
-5
-proportionality of 10Dq. Such values are consistently higher than those obtained from X-ray refinements, a method averaging rm-o for all the respective octahedral positions. 相似文献
602.
M. T. McCulloch T. K. Kyser J. D. Woodhead L. Kinsley 《Contributions to Mineralogy and Petrology》1994,115(3):303-312
A comprehensive Sr–Nd–Pb–O isotopic study is reported for rhyolites from the Maroa Volcanic Centre in the Taupo Volcanic Zone (TVZ) of New Zealand. The Sr–Nd isotopic compositions of the rhyolites (87Sr/86Sr=0.705236 to 0.705660 and Nd = 2.0 to 0.2) are intermediate between those of primitive basalts (87Sr/86Sr=0.70387 and Nd = 5.3) and the Torlesse basement (87Sr/86Sr=0.709 and Nd = -4.5). The relatively low mantle-like oxygen isotopic compositions of 18 O = 7 ± 0.5 are consistent with the Nd-Sr isotopic constraints in that they can be accounted for by 15% to 25% crustal contamination of a basaltic parent by relatively 18 O-rich Torlesse metasediment. High precision Pb isotopic analyses of plagioclase separates from the Maroa rhyolites show that they have essentially the same compositions as the Torlesse metasedimentary terrane which is itself distinctive from the Western or Waipapa metasediments. Due to the high concentration of Pb in the Torlesse metasediments (>20 ppm) compared to the basalts (<2 ppm), the Pb isotopic composition of the volcanics may be controlled by relatively small amounts (>10%) of crustal contamination. All these results are shown to be consistent with derivation of the rhyolites by 15% to 25% contamination of relatively primitive basaltic magmas with Torlesse metasedimentary crust, followed by extensive, essentially closed system fractionation of the basalt to a magma of rhyolite composition. It is argued that the processes of assimilation and fractionation are separated in both space and time. The voluminous high silica rhyolites, which make up >97% of the exposed volcanism in the continental margin back-are basin environment of the TVZ, therefore appear to be a product of predominantly new additions to the crust with assimilation-recycling of pre-existing crust being of secondary importance. 相似文献
603.
Keller LP Thomas KL Clayton RN Mayeda TK DeHart JM McKay DS 《Geochimica et cosmochimica acta》1994,58(24):5589-5598
A petrographic, geochemical, and oxygen isotopic study of the Bali CV3 carbonaceous chondrite revealed that the meteorite has undergone extensive deformation and aqueous alteration on its parent body. Deformation textures are common and include flattened chondrules, a well-developed foliation, and the presence of distinctive (100) planar defects in olivine. The occurrence of alteration products associated with the planar defects indicates that the deformation features formed prior to the episode of aqueous alteration. The secondary minerals produced during the alteration event include well-crystallized Mg-rich saponite, framboidal magnetite, and Ca-phosphates. The alteration products are not homogeneously distributed throughout the meteorite, but occur in regions adjacent to relatively unaltered material, such as veins of altered material following the foliation. The alteration assemblage formed under oxidizing conditions at relatively low temperatures (<100 degrees C). Altered regions in Bali have higher Na, Ca, and P contents than unaltered regions which suggests that the fluid phase carried significant dissolved solids. Oxygen isotopic compositions for unaltered regions in Bali fall within the field for other CV3 whole-rocks, however, the oxygen isotopic compositions of the heavily altered material lie in the region for the CM and CR chondrites. The heavy-isotope enrichment of the altered regions in Bali suggest alteration conditions similar to those for the petrographic type-2 carbonaceous chondrites. 相似文献
604.
The correlation between the long-term intensity variations of cosmic rays at neutron monitor energies and the LDE index measure of solar flares with long-lasting soft X-ray emissions is reported. Three subsequent solar cycles, 20–22, are taken into account and half-monthly data are analyzed. Possible explanation of this correlation is discussed in terms of the recent concepts of cosmic-ray modulation, in particular with merged interaction regions affecting the cosmic-ray intensity. 相似文献
605.
Analysis of high-spatial-resolution (approximately 0.8 arcsec) methane band and continuum imagery of Neptune's relatively homogeneous Equatorial Region yields significant constraints on (1) the stratospheric gaseous methane mixing ratio (fCH4,s), (2) the column abundances and optical properties of stratospheric and tropospheric hydrocarbon hazes, and (3) the wavelength-dependent single-scattering albedo of the 3-bar opaque cloud. From the center-to-limb behavior of the 7270-angstroms and 8900-angstrom sCH4 bands, the stratospheric methane mixing ratio is limited to fCH4,s < 1.7 x 10(-3), with a nominal value of fCH4,s = 3.5 x 10(-4), one to two orders of magnitude less than pre-Voyager estimates, but in agreement with a number of recent ultraviolet and thermal infrared measurements, and largely in agreement with the tropopause mixing ratio implied by Voyager temperature measurements. Upper limits to the stratospheric haze mass column abundance and 6190-angstroms and 8900-angstroms haze opacities are 0.61 microgram cm-2 and 0.075 and 0.042, respectively, with nominal values of 0.20 microgram cm-2 and 0.025 and 0.014 for the 0.2-micrometer radius particles preferred by the recent Voyager PPS analysis of Pryor et al. (1992, Icarus 99, 302-316). The tropospheric CH4 haze opacities are comparable to that found in the stratosphere, upper limits of 0.104 and 0.065 at 6190 angstroms and 8900 angstroms, respectively, with nominal values of 0.085 and 0.058. This indicates a column abundance less than 11.0 micrograms cm-2, corresponding to the methane gas content within a well-mixed 3% methane tropospheric layer only 0.1 cm thick near the 1.5-bar CH4 condensation level. Constraints on the single-scattering albedos of these hazes include (1) for the stratospheric component, 6190-angstroms and 8900-angstroms imaginary indices of refraction less than 0.047 and 0.099, respectively, with 0.000 (conservative scattering) being the nominal value at both wavelengths, and (2) CH4 haze single-scattering albedos greater than 0.85 and 0.50 at these two wavelengths, with conservative scattering again begin the preferred value. However, conservative scattering is ruled out for the opaque cloud near 3 bars marking the bottom of the visible atmosphere. Specifically, we find cloud single-scattering albedos of 0.915 +/- 0.006 at 6340 angstroms, 0.775 +/- 0.012 at 7490 angstroms, and 0.803 +/- 0.010 at 8260 angstrom. Global models utilizing a complete global spectrum confirm the red-absorbing character of the 3-bar cloud. The global-mean model has approximately 7.7 times greater stratospheric aerosol content then the Equatorial Region. An analysis of stratospheric haze precipitation rates indicates a steady-state haze production rate of 0.185-1.5 x 10(-14) g cm-2 sec-1, in agreement with recent theoretical photochemical estimates. Finally, reanalysis of the Voyager PPS 7500-angstroms phase angle data utilizing the fCH4,s value derived here confirms the Pryor et al. result of a tropospheric CH4 haze opacity of a few tenths in the 22-30 degrees S latitude region, several times that of the Equatorial Region or of the globe. The factor-of-10 reduction in fCH4,s below that assumed by Pryor et al. implies decreased gas absorption and consequently a decrease in the forward-scattering component of tropospheric aerosols. 相似文献
606.
Rice paddies as a methane source 总被引:8,自引:0,他引:8
Rice fields are considered to be among the highest sources of atmospheric methane, an important source of global warming. In order to meet the projected rice needs of the increasing world population, it is estimated that the annual world's rough rice production must increase to 760 million tons (a 65% increase) in the next 30 years. This will increase methane emissions from ricefields if current technologies are kept. Methane emissions from ricefields are affected by climate, water regime, soil properties, and various cultural practices like irrigation and drainage, organic amendments, fertilization, and rice cultivars. Irrigated rice comprises 50% of the world-harvested rice area and contributes 70% to total rice production. Because of assured flooding during the growing period it is the primary source of methane. Rainfed rice emits less methane due to periods of droughts. Upland rice, being never flooded for a significant period of time, is not a significant source of methane. There is great potential to develop no regret mitigation options that are in accordance with increasing rice production. 相似文献
607.
The most promising response strategies are -sustainable practices in agriculture to improve productivity on existing arable land especially in developing countries to meet the food requirements of a still rising population -sustainable practices in forestry both in tropical forests as well as in forests of temperate and boreal zones, in the latter case to achieve sufficient fast adaption to climate change. 相似文献
608.
J. K. Kairu 《International Journal of Salt Lake Research》1994,3(1):31-48
Specimens of three species of birds were collected from Lake Nakuru, Kenya, between September and October 1990. Samples of liver, kidney, muscle, fat and brain tissue were removed and analyzed for organochlorine pesticide residues. Fat was extracted and the content of three lindane (BHC/HCH) isomers (, and ), aldrin, heptachlor, heptachlorepoxide, endrin, dieldrin, DDD, DDE and DDT was determined. The samples contained varying residue levels of 12 organochlorine pesticides. No residues of 0, p'-DDD were detected. The most prevalent compounds were DDE and -BHC, found in 95.5 per cent and 66.4 per cent of the samples, respectively. The highest median residue concentration was 207 mg kg–1×10–3 of DDE in pelican fat tissue. White pelicanPelecanus onocrotalus, and the white-necked cormorant,Phalacrocorax carbo, showed greater concentrations of organochlorine residues than the lesser flamingo,Phoenicopterus minor. The mean DDE concentrations in pelican liver samples in 1970 and 1990 were 64 mg kg–1×10–3 and 274 mg kg–1×10–3, respectively. In cormorant liver samples the mean DDE concentration was 15 mg kg–1×10–3 in 1970 and 52 mg kg–1×10–3 in 1990. The mean DDE concentration in flamingo liver remained more or less similar at 2 mg kg–1×10–3 in 1970 and 1990. 相似文献
609.
K. G. Strassmeier 《Solar physics》1994,152(1):314-314
Observations of rotational modulation of continuum brightness and photospheric and chromospheric spectral-line profiles of late-type stars indicate the presence of very inhomogeneous surface temperature distributions. We present three stellar examples (VY Ari, HR 7275, HU Vir) where time-series photometry is used to trace the evolution of spotted regions. Simultaneous spectroscopy and Doppler imaging for one of the three stars (HU Virgo, Fig. 1) makes it possible to compute the temperature distribution of the photosphere and the relative intensity distribution of parts of the chromosphere (from CaII K and H line profiles). The combination of time-series spot modeling and Doppler imaging enabled us to determine thesign and amount of differential surface rotation on HU Vir. We found a big, cool polar spot (see figure below) and a differential (surface) rotation law where higher-latitude regions rotate faster than lower-latitude regions (opposite to what we see on the Sun). Currently, this ensemble of techniques - time-series photometry and photospheric and chromospheric Doppler imaging - is only applicable to stars overactive by approximately a factor of 100 as compared to the active Sun, e.g. the evolved components in RS CVn-type binaries and some rapidly-rotating, single, pre-main sequence stars or giant stars. Stellar rotation is a fundamental parameter for (magnetic) activity. Starspots, or any other surface inhomogeneities, allow one to derive very precise stellar rotation rates and, if coupled with seismological observations of solar-type stars, could provide information on the internal angular momentum distribution in overactive late-type stars.To be published in Astronomy & Astrophysics. 相似文献
610.
In the framework of the MIT bag model we consider absolutely stable strange quark matter consisting of u, d, and s quarks and electrons. For a realistic range of parameters of the quark bag we compute the threshold density for the appearance of strange quark matter that is realized on the surface of self-sustaining strange stars. On the basis of twelve calculated equations of state we give a detailed study of the series of configurations of strange stars consistent with the best known observational data. We show that the binding energy of the models depends essentially on the quark-gluon interaction constant c.Translated fromAstrofizika, Vol. 37, No. 3, 1994.The authors are grateful to E. V. Chubaryan and A. M. Atoyan for assistance in overcoming the information blockade. The present paper was written in the framework of area 46/101 93-353, supported by the Ministry of Higher Education and Science of the Republic of Armenia. 相似文献