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161.
Magnesian calcites are the most abundant authigenic minerals associated with hydrocarbon vents at 25 sites, in water depths ranging from 100 to 600 m in the Green Canyon area and about 2200 m in the Alaminos Canyon area on the Continental Slope of the northern Gulf of Mexico. The most frequently encountered magnesian calcites have 10–15 mol% MgCO3 and the apparent structural disorder revealed by XRD peak widths increases with Mg substitution. There are no systematic variations in Mg content with respect to water depth or geographic location. The calcite saturation state of the precipitating fluid is primarily determined by the nature of the fluids escaping from the vents, not the ambient seawater. 相似文献
162.
Alkalinity, dissolved inorganic carbon (DIC), and 13C profiles from seep sites on the northwestern Gulf of Mexico upper slope show anomalously negative 13C values of up to –4.5 PDB, increased levels of DIC of up to 2.45 mmole/liter, and slight alkalinity rises of up to 2.54 meq/liter, relative to water column profiles from a seep-free site (0.63, 2.04 mmole/liter, and 2.39 meq/liter). The observed DIC enrichments coupled with the13C-depletions are attributed to the release of CO2 by microbial oxidation of crude oil in the seep environment, and its migration into the water column. The 13C composition of the migrating CO2 is estimated to be –26.0 on the basis of dissolved carbon inventory. Manifestation of DIC and 13C anomalies in the water column caused by hydrocarbon seepage holds promise to be useful for hydrocarbon reconnaissance surveys over large offshore tracts on account of the simplicity of sampling acquisition, and rapidity of analytical techniques in the laboratory. 相似文献
163.
The likelihood that the carbon fluxes measured as part of the US-JGOFS field program in the equatorial Pacific ocean (EgPac) during 1992 yielded a balanced carbon budget for the surface ocean was determined. The major carbon fluxes incorporated into a surface carbon budget were: new production, particulate organic carbon (POC) and dissolved organic carbon (DOC) export, CaC03 export, C02 gas evasion, dissolved inorganic carbon (DIC) supply, and the time rate of charge. The ratio of the measured concentration gradients of DOC and DIC provided a constraint on the ratio of POC/DOC export. Uncertainties of ±30–50% for individual carbon flux measurements reduce the likelihood that a carbon balance can be measured during a JGOFS process-type study. As a benchmark, carbon fluxes were prescribed to yield a hypothetical surface carbon budget that was, on average, balanced. Given the typical errors in the individual carbon fluxes, however, there was only about a 30% chance that this hypothetical budget could be measured to be balanced to ±50%. Using this benchmark, it was determined that there was a 95 % chance that the carbon flux measurements yielded a surface DIC budget balanced (to ±50%) during El Nino conditions in boreal spring 1992, when the total organic carbon export rate was - 5 mmol C m-2 day- 1 and the POC export was 3 mmol C m−2 day−1. In boreal fall 1992, during cold period conditions, there was a 70% chance that the surface carbon DIC budget was balanced when the total organic carbon export rate was 20 mmol C m−2 day−1 and export was -13 mmol C m-2 day-'. The DOC to DIC concentration gradient ratio of - -0.15, measured in depth profiles down to 100m and in surface waters, was used as an important constraint that most (> 70%) of the organic carbon exported from the euphotic zone was POC rather than DOC. If a balanced surface DIC budget was used to test the compatibility of individual carbon fluxes measured during EgPac, then a three- to four-fold increase in total and particulate organic carbon export between spring and fall is indicated. This increase was not reflected in the POC loss rates measured by drifting sediment trap collections or estimated by234Th deficiencies coupled with the C/Th measured on suspended particles. 相似文献
164.
165.
Noriaki Kimura 《Journal of Oceanography》2007,63(4):685-694
This paper examines the mechanism controlling the short time-scale variation of sea ice cover over the Southern Ocean. Sea
ice concentration and ice velocity datasets derived from images of the Defense Meteorological Satellite Program (DMSP) Special
Sensor Microwave Imager (SSM/I) are employed to reveal this mechanism. The contribution of both dynamic and thermodynamic
processes to the change in ice edge location is examined by comparing the meridional velocity of ice edge displacement and
sea ice drift. In the winter expansion phase, the thermodynamic process of new ice production off the ice edge plays an important
role in daily advances of ice cover, whereas daily retreats are mostly due to southward ice drift. On the other hand, both
advance and retreat of ice edges in the spring contraction phase are mostly caused by the dynamic process of the ice drift.
Based on the above mechanism and the linear relation between the degree of ice production at the ice edge and northward wind
speed, the seasonal advance of ice cover can be roughly reproduced using the meridional velocity of ice drift at the ice edge. 相似文献
166.
Two distinct series of slumps deform the upper part of the sedimentary sequence along the continental margin of the Levant.
One series is found along the base of the continental slope, where it overlies the disrupted eastern edge of the Messinian
evaporites. The second series of slumps transects the continental margin from the shelf break to the Levant Basin. It seemed
that the two series were triggered by two unrelated, though contemporaneous, processes. The shore-parallel slumps were initiated
by basinwards flow of the Messinian salt, that carried along the overlying Plio-Quaternary sediments. Seawater that percolated
along the detachment faults dissolved the underlying salt to form distinctly disrupted structures. The slope-normal slumps
are located on top of large canyons that cut into the pre-Messinian sedimentary rocks. A layer of salt is found in the canyons,
and the Plio-Quaternary sediments were deposited on that layer. The slumps are bounded by large, NW-trending faults where
post-Messinian faulted offset was measured. We presume that the flow of the salt in the canyons also drives the slope-normal
slumps. Thus thin-skinned halokynetic processes generated the composite post-Tortonian structural patterns of the Levant margin.
The Phoenician Structures are a prime example of the collapse of a distal continental margin due to the dissolution of a massive
salt layer. 相似文献
167.
168.
Andrew R. Bowie Eric P. Achterberg Peter L. Croot Hein J.W. de Baar Patrick Laan James W. Moffett Simon Ussher Paul J. Worsfold 《Marine Chemistry》2006
The first large-scale international intercomparison of analytical methods for the determination of dissolved iron in seawater was carried out between October 2000 and December 2002. The exercise was conducted as a rigorously “blind” comparison of 7 analytical techniques by 24 international laboratories. The comparison was based on a large volume (700 L), filtered surface seawater sample collected from the South Atlantic Ocean (the “IRONAGES” sample), which was acidified, mixed and bottled at sea. Two 1-L sample bottles were sent to each participant. Integrity and blindness were achieved by having the experiment designed and carried out by a small team, and overseen by an independent data manager. Storage, homogeneity and time-series stability experiments conducted over 2.5 years showed that inter-bottle variability of the IRONAGES sample was good (< 7%), although there was a decrease in iron concentration in the bottles over time (0.8–0.5 nM) before a stable value was observed. This raises questions over the suitability of sample acidification and storage. 相似文献
169.
Brent L. Lewis Brian T. Glazer Paul J. Montbriand George W. Luther III Donald B. Nuzzio Timothy Deering Shufen Ma Stephen Theberge 《Marine Chemistry》2007,105(3-4):296-308
A combination of CTD casts, discrete bottle sampling and in situ voltammetric microelectrode profiling was used to examine changing redox conditions in the water column at a single station south of the Bay Bridge in the upper Chesapeake Bay in late July/early August, 2002–2005. Short-term (2–4 h) fluctuations in the oxic/suboxic/anoxic interface were documented using in situ voltammetric solid-state electrodes. Profiles of dissolved oxygen and sulfide revealed tidally-driven vertical fluctuations of several meters in the depth and thickness of the suboxic zone. Bottom water concentrations of sulfide, Mn2+ and Fe2+ also varied over the tidal cycle by approximately an order of magnitude. These data indicate that redox species concentrations at this site varied more due to physical processes than biogeochemical processes. Based on analysis of ADCP data, tidal currents at this station were strongly polarized, with the principal axis of tidal currents aligned with the mainstem channel. Together with the chemical data, the ADCP analysis suggests tidal flushing of anoxic bottom waters with suboxic water from north of the site. The present study is thus unique because while most previous studies have focused on processes across relatively stable redox interfaces, our data clearly demonstrate the influence of rapidly changing physical mixing processes on water column redox chemistry.Also noted during the study were interannual differences in maximum bottom water concentrations of sulfide, Mn2+ and Fe2+. In 2003, for example, heavy spring rains resulted in severe hypoxia/anoxia in June and early July. While reported storm-induced mixing in late July/early August 2003 partially alleviated the low-oxygen conditions, bottom water concentrations of sulfide, Mn2+ and Fe2+ were still much higher than in the previous year. The latter implies that the response time of the microbial community inhabiting the suboxic/anoxic bottom waters to changing redox conditions is slow compared to the time scale of episodic mixing events. Bottom water concentrations of the redox-sensitive chemical species should thus be useful as a tracer to infer prior hypoxic/anoxic conditions not apparent from ambient oxygen levels at the time of sampling. 相似文献
170.