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61.
Pollution history and recovery of a boreal lake exposed to a heavy bleached pulping effluent load 总被引:4,自引:0,他引:4
Juhani Hynynen Arja Palomäki Jarmo J. Meriläinen Allan Witick Keijo Mäntykoski 《Journal of Paleolimnology》2004,32(4):351-374
We examined the effects of heavy pulp mill discharges on the Lake Lievestuoreenjärvi ecosystem and the later recovery of diatom and chironomid communities from age-dated short core samples. Beginning in 1927 the lake received a heavy effluent load from a sulphite pulp mill. Except for the recession during the Second World War and the temporary closure of the mill from 1967 to 1971, the industrial load, containing large quantities of nutrients, organic matter and toxic compounds, increased continuously. In the early 1980s, laboratory documents were falsified by the directors of the mill and the systematic illegal effluent overload led to a collapse of the whole lake ecosystem. In 1985, the outdated plant was finally closed down. Based on the assessment of chemical properties and biological remains of the sediment, we distinguished five developmental phases in the ecological state of the lake. In the pre-industrial phase, the pelagic and profundal benthic communities were dominated by species preferring ultraoligotrophic or oligotrophic lakes. Concomitant with the increasing discharge and deposition of chlorine compounds, resin acids, and mercury, as well as strong acidity and hypolimnetic and epilimnetic anoxia, the ecological status changed in a short period from excellent to bad. Finally, in the early 1960s, the majority of the lake was virtually dead and the aquatic life survived only in the uppermost littoral zone. Since 1985, a fast recovery in the water quality has led to a strong, but temporary eutrophy in pelagic communities. The main peak of eutrophication was caused by the invasion of a species new to the lake,Aulacoseira granulata var.angustissima. Later, the pelagic communities shifted towards oligotrophy, but the original, pre-industrial status has not been re-established. The profundal benthic communities have not achieved the pre-industrial structure, but at present indicate mesotrophy. 相似文献
62.
The changing nature of, and approaches to, UK coastal management at the start of the twenty-first century 总被引:2,自引:0,他引:2
Peter W French 《The Geographical journal》2004,170(2):116-125
As we enter the twenty-first century, effective coastal management will become more of a central issue for coastal users and governors alike. The new century sees the review of many of the UK's existing management plans, and the subsequent publication of revised versions. Some of these new editions will have to show changes from their predecessors because of natural processes of erosion and accretion, yet other changes will be because of human interference. In this, we mean the continued ignoring of previous management plan recommendations regarding new development and coastal usage. Coastal management needs to adapt and develop, yet along with this, increased education and awareness is also necessary to allow users to understand and appreciate what is being recommended in management plans. 相似文献
63.
基于二维小波变换的FMI图象分割 总被引:1,自引:0,他引:1
为了从FMI资料中定量提取参数,一个重要的步骤是从实际FMI资料中分离出反映溶孔、溶洞、裂缝的子图像。本文给出的方法,考虑图像像元邻域的特征,应用二维小波变换求出目标与背景边缘的点集,按这个边缘点集的坐标点所对应的原图像像素灰度值的平均值作为分割阈值进行图像分割。实际资料处理表明,应用这种方法可以从实际的FMI资料中准确地分割出孔洞、裂缝的子图像并且可以按深度段连续自动处理,为后续定量计算参数奠定了良好基础。 相似文献
64.
65.
改进的能量守恒方法及其在CHAMP重力场恢复中的应用 总被引:1,自引:0,他引:1
XU Tianhe HE Kaifei Xi’an Research Institute of Surveying Mapping Middle Yanta Road Xi’an China. 《地球空间信息科学学报》2008,11(3):168-173
An efficient method for gravity field determination from CHAMP orbits and accelerometer data is referred to as the energy balance approach. A new CHAMP gravity field recovery strategy based on the improved energy balance approach IS developed in this paper. The method simultaneously solves the spherical harmonic coefficients, daily Integration constant, scale and bias parameters. Two 60 degree and order gravitational potential models, XISM-CHAMPO1S from the classical energy balance approach, and XISM-CHAMPO2S from the improved energy balance, are determined using about one year's worth of CHAMP kinematic orbits from TUM and accelerometer data from GFZ. Comparisons among XISM-CHAMPO1S, XISM-CHAMPO2S, EIGEN-CGO3C, EIGEN-CHAMPO3S, EIGEN2, ENIGNIS and EGM96 are made. The results show that the XISM-CHAMPO2S model is more accurate than EGM96, EIGENIS, EIGEN2 and XISM-CHAMPO1S at the same degree and order, and has almost the same accuracy as EIGEN-CHAMPO3S. 相似文献
66.
Using microprobe laser-desorption, laser-ionization mass spectrometry (μL2MS), we measured the distributions of alkylated and unalkylated polycyclic aromatic hydrocarbons (PAHs) in the free organic material of 20 carbonaceous chondrites. These meteorites represent a variety of meteorite classes and alteration histories, including CI, CK, CM, CO, CR, CV, and Tagish Lake. This work provides information on free organic compounds that is complementary to studies of the structure and composition of meteoritic macromolecular content.For the nine CM2 meteorites analyzed, we observe that higher relative abundances of alkylated PAHs correlate with more intense aqueous activity. We attribute this correlation to the differences in solubility and volatility between unalkylated and alkylated PAHs. Naphthalene and its alkylation series are more susceptible to the effects of aqueous exposure than the less-soluble PAH phenanthrene and its alkylated derivatives. These observations are consistent with the possibility of chromatographic separations on the meteorite parent bodies. We identify six CM2 meteorites with similar PAH distributions that may represent the original, unaltered organic composition of the parent body.Increased metamorphic intensity reduces the abundance of all PAHs. The thermally metamorphosed CK chondrites had no detectable levels of typical meteoritic PAHs. This observation might be explained either by a loss of PAHs caused by volatilization or by a significantly different organic content of the CK parent body. 相似文献
67.
Here we report iron (Fe) isotopic data of three pure Fe solution standards (IRMM-014, GSB Fe, and NIST 3126a) and five widely used geological reference materials (RMs) from the United States Geological Survey and Geological Survey of Japan obtained on a Neptune Plus multi-collector–inductively coupled plasma–mass spectrometer (MC-ICP-MS) in our laboratory over the past 3 years. The instrumental mass bias was corrected by three independent methods: sample-standard bracketing (SSB), Ni doping?+?SSB, and 57Fe–58Fe double spike?+?SSB. Measurements reveal that both the Ni doping and double spike methods helped calibrate short-term fluctuations in mass bias. Collectively, almost all measurements of RMs yielded δ56Fe within?±?0.05 of recommended values, provided that each sample was measured four times on MC-ICP-MS. For the first time, new recommended values for NIST SRM3126a are reported (δ56Fe?=?0.363?±?0.006, 2SE, 95% CI; and δ57Fe?=?0.534?±?0.010, 2SE). 相似文献
68.
Calcite was synthesized by four methods, and the luminescence decay-time was measured for nine samples before and after heating
hydrothermally in the temperature range 200–400°C. Decay-time data were collected between room temperature and approximately
15 K. The decay time at room temperature is approximately 50 ms, with little difference between a given calcite before and
after hydrothermal treatment. The decay time at 15 K is always greater than at room temperature as the effect of thermal quenching
diminishes. Differences in decay time before and after heating are more apparent at low temperature owing to this reduction
in thermal quenching. The decay time decreased significantly in two samples, and an increase in decay time was observed in
the remaining seven samples following heating. Among the latter group, the change in decay time was insignificant in three
samples. The results are compared with previous data in which it was shown that the effect of heating is to increase the intensity
of luminescence. 相似文献
69.
Friedrich Lucassen Peter Dulski Rainer Abart Gerhard Franz Dieter Rhede Rolf L. Romer 《Contributions to Mineralogy and Petrology》2010,160(2):279-295
Titanite growth at the expense of rutile during retrograde hydration of eclogite into amphibolite is a common phenomenon. We investigated an amphibolite sample from the Tromsø eclogite facies terrain in Northern Norway to gain insight into the trace element distribution between rutile and titanite during incomplete resorption of the rutile by titanite. Patchy compositional zoning of Al, Ti, and F in titanite relates to the presence of a fluid with variable Ti/Al and/or F during its growth. Laser ablation ICP–MS and electron microprobe data for high field strength elements (HFSE: Nb, Zr, Ta, and Hf) of rutile resorbed by titanite indicate a pronounced enrichment of these elements in the rim of a large single rutile crystal (~8 mm) and a systematic decrease towards uniform HFSE contents in the large core. HFSE contents of smaller rutile grains (~0.5 mm) and rutile inclusions (<100 μm) in the titanite overgrowth are similar or higher than in the rims of large rutile crystals. Element profiles from the rim inward demonstrate that HFSE enrichment in rutile is controlled by diffusion. HFSE ratios in diffusion-altered rutile show systematic variations compared with the uniform core composition of the large rutile. Modelling of Zr and Nb diffusion in rutile indicates that diffusion coefficients in rutile in fluid-dominated natural systems must be considerably higher than those determined experimentally at 1 bar in dry systems. Variations of HFSE contents in the newly formed titanite show no systematic spatial distribution. HFSE ratios in titanite and the rims of rutile are different, indicating different solid/fluid distribution coefficients in these minerals. Element fractionation by diffusion into the relict rutile and during fluid-mediated growth of new titanite could substantially change the HFSE budget of these minerals and could affect their use for geochemical tracing and other applications, such as Zr-based geothermobarometry. 相似文献
70.
Bradley D. Eyre Søren Rysgaard Tage Dalsgaard Peter Bondo Christensen 《Estuaries and Coasts》2002,25(6):1077-1087
Denitrification has been measured during the last few years using two different methods in particular: isotope pairing measured on a triple-collector isotopic ratio mass spectrometer and N2:Ar ratios measured on a membrane inlet mass spectrometer (MIMS). This study compares these two techniques in short-term batch experiments. Rates obtained using the original N2∶Ar method were up to 3 to 4 times higher than rates obtained using the isotope pairing technique due to O2 reacting with the N2 during MIMS analysis. Oxygen combines with N2 within the mass spectrometer ion source forming NO+ which reduces the N2 concentration. The decrease in N2 is least at lower O2 concentrations and since oxygen is typically consumed during incubations of sediment cores, the result is often a pseudo-increase in N2 concentration being interpreted as denitrification activity. The magnitude of this ocygen effect may be instrument specific. The reaction of O2 with N2 and the subsequent decrease in N2 was only partly correctly using an O2 correction curve for the relationship between N2 and O2 concentrations. The O2 corrected N2∶Ar denitrification rates were lower, but still did not match the isotope pairing rates and the variability between replicates was much higher. Using a copper reduction column heated to 600°C to remove all of the O2 from the sample before MIMS analysis resulted in comparable rates (slightly lower), and comparable variability between replicates, to the isotope pairing technique. The N2:Ar technique determines the net N2 production as the difference between N2 production by denitrification and N2 consumption by N-fixation, while N-fixation has little effect on the isotope pairing technique which determines a rate very close to the gross N2 production. When the two different techniques were applied on the same sediment, the small difference in rates obtained by the two methods seemed to reflect N-fixation as also supported from measurements of ethylene production in acetylene enriched sediment cores. The N2:Ar and isotope pairing techniques may be combined to provide simultaneous measurements of denitrification and N-fixation. Both techniques have several assumptions that must be met to achieve accurate rates; a number of tests are outlined that can be applied to demonstrate that these assumptions are being meet. 相似文献