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51.
Kinetics and Equilibrium Sorption Studies of 4-Nitrophenol on pyrolyzed and activated oil shale residue 总被引:1,自引:0,他引:1
Sorption of the organic pollutant 4-nitrophenol (4-NP) by pyrolyzed and activated Jordanian oil-shale was studied. Pyrolyzed oil shale was prepared using a fluidized bed reactor at 520 °C in the presence of nitrogen. Physical activation was carried out by treating the pyrolyzed oil shale with CO2 at 830 °C, while chemical activation was achieved by using KOH and ZnCl2 as impregnating agents. Batch kinetics and isotherm studies were conducted to evaluate the sorption process. Effects of contact time, initial sorbate concentration, sorbent concentration, temperature, pH and inorganic salts (NaCl and KCl) on the sorption process by the different sorbents were considered. Chemically activated oil shale, pretreated with ZnCl2, gave the highest uptake of 4-NP. The isotherm experimental data fit reasonably well to Langmuir, Freundlich and Redlich-Paterson models. Three kinetic models, namely the Morris-Weber, Lagergren, and Pseudo-Second-Order model (PSOM), were applied to represent the experimental results for both pyrolyzed and ZnCl2-oil shale sorbents. 相似文献
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In Europe, the Wide Wheel abrasion (WWA) test and the B?hme abrasion (BA) test are among the most widely used standard test
methods for determining abrasion resistance of natural stones, the former being the reference test method in EN 14157 Standard.
However, it is stated in the Annex-A (Informative) of EN 14157 Standard that very limited data are available to provide correlations
between these two test methods. To be able to fill this gap, in this study, 25 different natural stones belonging to sedimentary,
metamorphic and igneous groups were tested for their abrasion resistance as well as physico-mechanical properties. Also, for
a better interpretation of abrasion resistance characteristics of the tested stone materials, relationships between abrasion
resistance and physico-mechanical properties were statistically examined. A statistically significant linear correlation (R
2 = 0.85; P value = 0.000) was established between the WWA test and the BA test, which could be used in practice for converting the measured
abrasion resistance values from one testing method to another. It was also found that the correlation between these two test
methods improved significantly (R
2 = 0.93; P value = 0.001) when relatively high-porosity stone materials (porosity ≥1%) were separately evaluated. Both methods of abrasion
resistance employed in the present study showed statistically significant linear correlations with uniaxial compressive strength
and Brazilian tensile strength, the former proving to be a more influencing parameter on resistance to abrasion. Also, from
the point view of representing actual abrasion mechanism of stone materials in practice, the necessity of simulating multi-directional
foot traffic in abrasion testing methods was discussed. In this respect, the reference test method in the EN 14157 Standard
was criticized for not fully meeting this requirement. It was also pointed out that the reference method could have some drawbacks
when applied to coarse-grained granitic rocks having cleavable minerals such as plagioclase and orthoclase feldspars. 相似文献
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57.
Amino acid nitrogen in atmospheric aerosols: Occurrence,sources and photochemical modification 总被引:2,自引:0,他引:2
The presence of amino acids in atmospheric precipitation and aerosols has been noted for many years, yet relatively little is known about these or other nitrogen containing organic compounds in the atmosphere. Marine and continental rainwater analyses indicate that atmospheric aerosols, and subsequently atmospheric precipitation, may contain substantial levels of free and combined amino acids. The most likely source of amino N in the remote marine atmosphere appears to be the injection of proteinaceous material through the action of bursting bubbles at the sea-air interface or the long range transport from terrestrial sources. The capacity of these substrates to undergo photooxidation and photodegradation in the atmosphere to simpler species, such as ammonium ions, carboxylic acids, and for the S containing amino acids, oxidized forms of sulfur, has received little attention from atmospheric chemists. The photochemistry of covalently bound amino groups, particularly as found in peptides and amino acids, is discussed here with the purpose of summarizing what is known of their occurrence and their possible importance to atmospheric chemistry. 相似文献
58.
Kristie?L.?EbiEmail author Jessica?Hartman Nathan?Chan John?Mcconnell Michael?Schlesinger John?Weyant 《Climatic change》2005,73(3):375-393
Climate is one factor that determines the potential range of malaria. As such, climate change may work with or against efforts
to bring malaria under control. We developed a model of future climate suitability for stable Plasmodium falciparum malaria transmission in Zimbabwe. Current climate suitability for stable malaria transmission was based on the MARA/ARMA
model of climatic constraints on the survival and development of the Anopheles vector and the Plasmodium falciparum malaria parasite. We explored potential future geographic distributions of malaria using 16 projections of climate in 2100.
The results suggest that, assuming no future human-imposed constraints on malaria transmission, changes in temperature and
precipitation could alter the geographic distribution of malaria in Zimbabwe, with previously unsuitable areas of dense human
population becoming suitable for transmission. Among all scenarios, the highlands become more suitable for transmission, while
the lowveld and areas with low precipitation show varying degrees of change, depending on climate sensitivity and greenhouse
gas emission stabilization scenarios, and depending on the general circulation model used. The methods employed can be used
within or across other African countries. 相似文献
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