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31.
Mössbauer spectra (MS) of blue, green and yellow beryl (ideally Be3Al2Si6O18) containing approximately 1% of iron were obtained at 295 and 500 K. Room temperature (RT) spectra of both blue and green samples showed the presence of an asymmetric Fe2+ doublet (ΔE Q~2.7 mm/s, δ~1.1 mm/s), with a very broad low-velocity peak. There is no clear evidence for the presence of a ferric component. The MS of the yellow sample at RT consists of an intense central absorption with parameters typical for Fe3+E Q~0.4 mm/s, δ~0.29 mm/s), plus an apparently symmetrical Fe2+ doublet. This sample acquires a light-blue shade upon heating in air at about 620 K. Thermal treatments at high temperatures caused no significant changes in the MS, but the green and yellow beryl acquire a blue colour. All these results are interpreted in relation to the existence of channel water and the distribution of iron among the available crystallographic sites.  相似文献   
32.
Summary ?Retrievals of atmospheric aerosol optical thickness are highly dependent on the choice of the class describing the aerosol properties leading to significant errors while using classes available in the literature. High spectral resolution measurements from GOME (Global Ozone Monitoring Experiment) between the ultraviolet and the near infrared can be used for an accurate characterization of the aerosol optical properties. The radiometer MVIRI (METEOSAT Visible and Infrared Imager) on board the geostationary satellite METEOSAT, while being equipped only with broadband VIS channel, ensures an adequate half-hourly monitoring of the atmospheric conditions over a large portion of the Earth. The present algorithm is based on a combination of data from both sensors for the retrieval of the aerosol optical thickness at the reference wavelength of 0.55 μm (AOT). A case of a desert dust outbreak from the African continent over the Atlantic Ocean is examined. AOT values obtained using a priori fixed classes taken from the literature are compared with those retrieved with this algorithm using the GOME-derived classes. Systematic differences of the order of a few tenths on average are found which remain significant also after considering the measurement errors. This represents a novelty introduced by the synergetic use of both sensors. Received March 13, 2002  相似文献   
33.
在简述盆地地质环境和含水系统、水文地质期与水压系统类型定位的基础上,通过建立数学模型,采用反演、比拟和地静压力等方法,模拟计算了各研究层在各研究时期泥岩压出水水头值(m),Es^2层的依次为2-28,2-26,2-6,2-16,0.5-3.5;Es^1层的依次为2-42,2-26,2-6,10-54,1-14;Ed层的依次为2-22,2-54,2-12;Ng层的依次为10-24,1-5;Nm层的为12-24。各研究层在各研究时期的压挤式水交替强度均小于1,累加值Es^2,Es^1,Ed层的均大于1,Ng,Nm层的小于1;Ed层渗入水交替强度为0.44。各研究层在各研究时期渗流场的高水压带位置和流动态具有相似性,并均以离心型流动型为主要特征。  相似文献   
34.
35.
A novel method for synthesis of aluminium hematites, based upon the homogeneous precipitation of Fe and Al oxinates in various proportions, is presented. The precursor precipitates are heated in air at 700?°C. X-ray diffraction, thermal analyses, BET, FTIR, optical reflection analysis, TEM and Mössbauer spectroscopy at room temperature and 80?K of the resulting products indicate that single-phase hematites are formed with structural Al substitution of up to 10 at%. Interestingly, the particle size (>100?nm) is not substantially reduced by the Al content. Although it remains difficult to obtain a homogeneously distributed Al substitution in the final hematite, this processing line offers a unique opportunity to separate the effects of grain size and Al substitution on the Morin transition temperature (T M) of Al hematite. From the comparison between the present hematites and a series of Al-substituted hematites with lepidocrocite as precursor, it could be shown that the effect on T M, associated with a change of a factor 10 in grain size, is about 1/3 of the effect caused by a change of 10 in the degree of substitution. Finally, it is suggested that proper thermal treatments under different conditions of the same precursors are likely to produce spinel phases.  相似文献   
36.
The magnetotelluric (MT) method has been applied to the determination of the deep resistivity structure of the northeastern margin of the Parnaiba Basin. Transient electromagnetic (TEM) and MT data were collected in early 1999 along a 95 km long N–S line, extending from the coast across the projected subcrop position of a discontinuous fault found to the west of the study area that is believed to be a possible basin‐bounding fault. The MT data were processed to yield the TE‐ and TM‐mode responses and then corrected for static shift using central‐loop and single‐loop TEM data, respectively. Regularized 2D MT inversion was subsequently undertaken using a structured initial model with the near‐surface constrained by TEM inversion results. As a consistency check, we performed another set of 2D inversions using different smooth initial models. The various optimal 2D inversion models show clearly the presence of a major basement trough, over 2 km deep, located about 70 km from the coast. We interpret it as possibly marking the main basin margin and suggest that it may have implications for groundwater resource development in the area.  相似文献   
37.
In the Négron River catchment area (162 km2), surface‐sediment stores are composed of periglacial calcareous ‘grèze’ (5 × 106 t) and loess (21 × 106 t), and Holocene alluvium (12·6 × 106 t), peat (0·6 × 106 t) and colluvium (18·5 × 106 t). Seventy‐five per cent of the Holocene sediments is stored along the thalwegs. Present net sediment yield, calculated from solid discharge at the Négron outlet, is low (0·6 t km?2 a?1) due to the dominance of carbonate rocks in the catchment. Mean sediment yield during the Holocene period is 7·0 t km?2 a?1 from alluvium stores and 7·6 t km?2 a?1 from colluvium stores. Thus, the gross sediment yield during the Holocene period is about 18·7 t km?2 a?1 and the sediment delivery ratio 3 per cent. The yield considerably varies from one sub‐basin to another (3·9 to 24·5 t km?2 a?1) according to lithology: about 25 per cent and 50 per cent of initial stores of periglacial grèze and loess respectively were reworked during the Holocene period. Sediment yield has increased by a factor of 6 in the last 1000 years, due to the development of agriculture. The very high rate of sediment storage on the slope during that period (88 per cent of the yield) can be accounted for by the formation of cultivation steps (‘rideaux’). It is predicted that the current destruction of these steps will result in a sediment wave reaching the valley floors in the coming decades. Subboreal and Subatlantic sediments and pollen assemblages in the Taligny marsh, where one‐third of the alluvium is stored, show the predominant influence of human activity during these periods in the Négron catchment. Copyright © 2002 John Wiley & Sons, Ltd.  相似文献   
38.
This paper presents results recently obtained for generating site-specific ground motions needed for design of critical facilities. The general approach followed in developing these ground motions using either deterministic or probabilistic criteria is specification of motions for rock outcrop or very firm soil conditions followed by adjustments for site-specific conditions. Central issues in this process include development of appropriate attenuation relations and their uncertainties, differences in expected motions between Western and Eastern North America, and incorporation of site-specific adjustments that maintain the same hazard level as the control motions, while incorporating uncertainties in local dynamic material properties. For tectonically active regions, such as the Western United States (WUS), sufficient strong motion data exist to constrain empirical attenuation relations for M up to about 7 and for distances greater than about 10–15 km. Motions for larger magnitudes and closer distances are largely driven by extrapolations of empirical relations and uncertainties need to be substantially increased for these cases.

For the Eastern United States (CEUS), due to the paucity of strong motion data for cratonic regions worldwide, estimation of strong ground motions for engineering design is based entirely on calibrated models. The models are usually calibrated and validated in the WUS where sufficient strong motion data are available and then recalibrated for applications to the CEUS. Recalibration generally entails revising parameters based on available CEUS ground motion data as well as indirect inferences through intensity observations. Known differences in model parameters such as crustal structure between WUS and CEUS are generally accommodated as well. These procedures are examined and discussed.  相似文献   

39.
High spatial resolution U–Pb dates of zircons from two consanguineous ignimbrites of contrasting composition, the high-silica rhyolitic Toconao and the overlying dacitic Atana ignimbrites, erupted from La Pacana caldera, north Chile, are presented in this study. Zircons from Atana and Toconao pumice clasts yield apparent 238U/206Pb ages of 4.11±0.20 Ma and 4.65±0.13 Ma (2σ), respectively. These data combined with previously published geochemical and stratigraphic data, reveal that the two ignimbrites were erupted from a stratified magma chamber. The Atana zircon U–Pb ages closely agree with the eruption age of Atana previously determined by K–Ar dating (4.0±0.1 Ma) and do not support long (>1 Ma) residence times. Xenocrystic zircons were found only in the Toconao bulk ignimbrite, which were probably entrained during eruption and transport. Apparent 238U/206Pb zircon ages of 13 Ma in these xenocrysts provide the first evidence that the onset of felsic magmatism within the Altiplano–Puna ignimbrite province occurred approximately 3 Myr earlier than previously documented.  相似文献   
40.
Oxygen isotope studies were carried out across units of a Neoproterozoic nappe system, south of São Francisco Craton. A temperature decrease toward the base of the system is found, consistent with a previously recognized inverted metamorphic pattern. The tectonic contact of the basal unit and the reworked southern São Francisco craton show a steep temperature gradient, suggesting that low temperature thrusting acted as the dominant tectonic process. The contrasts between the δ18O values of the Três Pontas-Varginha and Carmo da Cachoeira nappes and the differences among the samples and minerals are consistent with the preservation of sedimentary isotopic composition during metamorphism. The small differences in the δ18O values between the undeformed and the deformed calc-silicate samples (1.6‰) suggest that the δ18O value of mylonitization fluids was close to that which equilibrated with the metamorphic assemblage. The distinct δ18O values of metapelitic and calc-silicate samples and the great temperature difference from one type to the other indicate that no large-scale fluid interaction processes occurred during metamorphism. Oxygen isotopic estimations of both Três Pontas-Varginha undeformed rocks and Carmo da Cachoeira unaltered equivalents indicate δ18O values of up to 18‰. Comparison between these values and those from the ‘basement’ orthogneisses (8.3–8.5‰) indicates the latter are not sources for the metapelites.  相似文献   
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