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41.
The soil leakage ratio in the Mudu watershed,China 总被引:3,自引:0,他引:3
42.
The Removal of Dissolved Metals by Hydroxysulphate Precipitates during Oxidation and Neutralization of Acid Mine Waters, Iberian Pyrite Belt 总被引:4,自引:0,他引:4
J. Sánchez España E. López Pamo E. Santofimia Pastor J. Reyes Andrés J. A. Martín Rubí 《Aquatic Geochemistry》2006,12(3):269-298
This study examines the removal of dissolved metals during the oxidation and neutralization of five acid mine drainage (AMD)
waters from La Zarza, Lomero, Esperanza, Corta Atalaya and Poderosa mines (Iberian Pyrite Belt, Huelva, Spain). These waters
were selected to cover the spectrum of pH (2.2–3.5) and chemical composition (e.g., 319–2,103 mg/L Fe; 2.85–33.3 g/L SO4=) of the IPB mine waters. The experiments were conducted in the laboratory to simulate the geochemical evolution previously
recognized in the field. This evolution includes two stages: (1) oxidation of dissolved Fe(II) followed by hydrolysis and
precipitation of Fe(III), and (2) progressive pH increase during mixing with fresh waters. Fe(III) precipitates at pH < 3.5
(stages 1 and 2) in the form of schwertmannite, whereas Al precipitates during stage 2 at pH 5.0 in the form of several hydroxysulphates
of variable composition (hydrobasaluminite, basaluminite, aluminite). During these stages, trace elements are totally or partially
sorbed and/or coprecipitated at different rates depending basically on pH, as well as on the activity of the SO4=
anion (which determines the speciation of metals). The general trend for the metals which are chiefly present as aqueous
free cations (Pb2+, Zn2+, Cu2+, Cd2+, Mn2+, Co2+, Ni2+) is a progressive sorption at increasing pH. On the other hand, As and V (mainly present as anionic species) are completely
scavenged during the oxidation stage at pH < 3.5. In waters with high activities (> 10−1) of the SO 4= ion, some elements like Al, Zn, Cd, Pb and U can also form anionic bisulphate complexes and be significantly sorbed at pH
< 5. The removal rates at pH 7.0 range from around 100% for As, V, Cu and U, and 60–80% for Pb, to less than 20% for Zn, Co,
Ni and Mn. These processes of metal removal represent a significant mechanism of natural attenuation in the IPB. 相似文献
43.
Eclogites formed by the Lufilian (post-Katanga) metamorphism of gabbros intruded into rocks of the Katanga System (Upper Proterozoic) occur in the Central Province of Zambia. Typical constituents of these rocks are omphacite, almandine garnet with significant contents of the pyrope and grossular components, kyanite and rutile. Eclogites from some localities display well preserved, relict ophitic texture inherited from the original gabbro. Hornblende-scapolite metagabbro and coronite metagabbro often accompany the eclogites, and metalherzolite and serpentinite occur at a few localities. The Zambian eclogites are broadly associated with a variety of relatively high-pressure, kyanite-bearing mineral assemblages some of which are possibly in the eclogite facies. It is suggested that, in addition to temperature and load pressure, fluid pressure, fluid composition (H2O, CO2, Cl, SO3) and permeability of the gabbro due to deformation were important factors for the transformation of gabbro to eclogite in the environment of the Lufilian Arc. 相似文献
44.
Borja A Barbone E Basset A Borgersen G Brkljacic M Elliott M Garmendia JM Marques JC Mazik K Muxika I Magalhães Neto J Norling K Rodríguez JG Rosati I Rygg B Teixeira H Trayanova A 《Marine pollution bulletin》2011,62(3):499-513
In recent times many benthic indices have been proposed to assess the ecological quality of marine waters worldwide. In this study we compared single metrics and multi-metric methods to assess coastal and transitional benthic status along human pressure gradients in five distinct environments across Europe: Varna bay and lake (Bulgaria), Lesina lagoon (Italy), Mondego estuary (Portugal), Basque coast (Spain) and Oslofjord (Norway). Hence, 13 single metrics (abundance, number of taxa, and several diversity and sensitivity indices) and eight of the most common indices used within the European Water Framework Directive (WFD) for benthic assessment were selected: index of size spectra (ISS), Benthic assessment tool (BAT), Norwegian quality index (NQI), Multivariate AMBI (M-AMBI), Benthic quality index (BQI), (Benthic ecosystem quality index (BEQI), Benthic index based on taxonomic sufficiency (BITS), and infaunal quality index (IQI). Within each system, sampling sites were ordered in an increasing pressure gradient according to a preliminary classification based on professional judgement. The different indices are largely consistent in their response to pressure gradient, except in some particular cases (i.e. BITS, in all cases, or ISS when a low number of individuals is present). Inconsistencies between indicator responses were most pronounced in transitional waters (i.e. IQI, BEQI), highlighting the difficulties of the generic application of indicators to all marine, estuarine and lagoonal environments. However, some of the single (i.e. ecological groups approach, diversity, richness) and multi-metric methods (i.e. BAT, M-AMBI, NQI) were able to detect such gradients both in transitional and coastal environments, being these multi-metric methods more consistent in the detection than single indices. This study highlights the importance of survey design and good reference conditions for some indicators. The agreement observed between different methodologies and their ability to detect quality trends across distinct environments constitutes a promising result for the implementation of the WFD’s monitoring plans. Moreover, these results have management implications, regarding the dangers of misclassification, uncertainty in the assessment, use of conflicting indices, and testing and validation of indices. 相似文献
45.
María Charco José Fernández Francisco Luzón Kristy F. Tiampo John B. Rundle 《Pure and Applied Geophysics》2007,164(4):865-878
Surface displacements and gravity changes due to volcanic sources are influenced by medium properties. We investigate topographic,
elastic and self-gravitation interaction in order to outline the major factors that are significant in data modelling. While
elastic-gravitational models can provide a suitable approximation to problems of volcanic loading in areas where topographic
relief is negligible, for prominent volcanoes the rough topography could affect deformation and gravity changes to a greater
extent than self-gravitation. This fact requires the selection, depending on local relief, of a suitable model for use in
the interpretation of surface precursors of volcanic activity. We use the three-dimensional Indirect Boundary Element Method
to examine the effects of topography on deformation and gravity changes in models of magma chamber inflation/deflation. Topography
has a significant effect on predicted surface deformation and gravity changes. Both the magnitude and pattern of the geodetic
signals are significantly different compared to half-space solutions. Thus, failure to account for topographic effects in
areas of prominent relief can bias the estimate of volcanic source parameters, since the magnitude and pattern of deformation
and gravity changes depend on such effects. 相似文献
46.
E. García-Bustamante J. F. González-Rouco J. Navarro E. Xoplaki P. A. Jiménez J. P. Montávez 《Climate Dynamics》2012,38(1-2):141-160
The variability and predictability of the surface wind field at the regional scale is explored over a complex terrain region in the northeastern Iberian Peninsula by means of a downscaling technique based on Canonical Correlation Analysis. More than a decade of observations (1992–2005) allows for calibrating and validating a statistical method that elicits the main associations between the large scale atmospheric circulation over the North Atlantic and Mediterranean areas and the regional wind field. In an initial step the downscaling model is designed by selecting parameter values from practise. To a large extent, the variability of the wind at monthly timescales is found to be governed by the large scale circulation modulated by the particular orographic features of the area. The sensitivity of the downscaling methodology to the selection of the model parameter values is explored, in a second step, by performing a systematic sampling of the parameters space, avoiding a heuristic selection. This provides a metric for the uncertainty associated with the various possible model configurations. The uncertainties associated with the model configuration are considerably dependent on the spatial variability of the wind. While the sampling of the parameters space in the model set up moderately impact estimations during the calibration period, the regional wind variability is very sensitive to the parameters selection at longer timescales. This fact illustrates that downscaling exercises based on a single configuration of parameters should be interpreted with extreme caution. The downscaling model is used to extend the estimations several centuries to the past using long datasets of sea level pressure, thereby illustrating the large temporal variability of the regional wind field from interannual to multicentennial timescales. The analysis does not evidence long term trends throughout the twentieth century, however anomalous episodes of high/low wind speeds are identified. 相似文献
47.
Summary ?During recent years, numerous studies have examined the Buenos Aires urban climate, but the relationship between large-scale
weather conditions and the Buenos Aires urban heat island (UHI) intensity has not been studied. The goal of this paper is
to apply an objective synoptic climatological method to identify homogeneous air masses or weather types affecting Buenos
Aires during winter, and to relate the results to the UHI intensity. A K-means clustering method was used to define six different
air masses considering the 03:00, 09:00, 15:00 and 21:00 LT surface observations of dry bulb temperature, dew point, cloud
cover, atmospheric pressure and wind direction and velocity at Ezeiza, the most rural meteorological station of the Buenos
Aires metropolitan area (Fig. 1). Results show that the mean UHI intensity is at its maximum (2.8 °C) a few hours before sunrise
when conditions are dominated by cold air masses associated with cold-core anticyclones, weak winds and low cloud cover. Inverse
heat islands are found during the afternoon for all air masses indicating that surface processes are not dominant at that
time. The relatively infrequent and warmest air mass is the only one that presents a mean negative urban-rural temperature
difference (−0.1 °C) during the afternoon with the smallest diurnal cycle of the UHI intensity probably due to the prevailing
high humidity and cloudy sky conditions. The paper provides an insight into the Buenos Aires urban–rural temperature difference
under a variety of winter weather types and results could be useful to improve local daily temperature forecasts for the metropolitan
area of Buenos Aires on the basis of the routine forecasts of weather types.
Received October 24, 2001; revised June 12, 2002; accepted October 10, 2002 相似文献
48.
C. Serra G. Fernández Mills M. C. Periago X. Lana 《Theoretical and Applied Climatology》1998,59(1-2):29-49
Summary Catalonian daily precipitation patterns were obtained by means of S-mode Principal Component Analysis (PCA) applied to subsets
built up according to synoptic surface airflow. Daily data from November to April 1990–1994 from 45 raingauge sites in Catalonia
without missing data were used. Eight circulation classes for days in this period were considered. A Precipitation Activity
Index (PAI) was calculated for each station and class, leading to the determination of the highest activity regions for each
subset. In addition, we determined which circulation type produced most precipitation at each station of the network. Separate
PCAs were performed for each of the eight classes considered and the first four Varimax rotated solutions were interpreted
for each circulation type. The physical meaning of the rest of the factors were omitted as they were associated with local
behaviour. Finally, some concluding remarks on the cyclogenic properties of the Western Mediterranean Basin and the diversity
of the extracted patterns are presented and supported by the authors experience in forecasting in Catalonia.
Received February, 11, 1997 Revised May 23, 1997 相似文献
49.
General purpose Computational Fluid Dynamics (CFD) solvers are frequently used in small-scale urban pollution dispersion simulations
without a large extent of ver- tical flow. Vertical flow, however, plays an important role in the formation of local breezes,
such as urban heat island induced breezes that have great significance in the ventilation of large cities. The effects of
atmospheric stratification, anelasticity and Coriolis force must be taken into account in such simulations. We introduce a
general method for adapting pressure based CFD solvers to atmospheric flow simulations in order to take advantage of their
high flexibility in geometrical modelling and meshing. Compressibility and thermal stratification effects are taken into account
by utilizing a novel system of transformations of the field variables and by adding consequential source terms to the model
equations of incompressible flow. Phenomena involving mesoscale to microscale coupled effects can be analyzed without model
nesting, applying only local grid refinement of an arbitrary level. Elements of the method are validated against an analytical
solution, results of a reference calculation, and a laboratory scale urban heat island circulation experiment. The new approach
can be applied with benefits to several areas of application. Inclusion of the moisture transport phenomena and the surface
energy balance are important further steps towards the practical application of the method. 相似文献
50.
The surface renewal (SR) method was applied for the first time to measurements of air temperature over four Amazonian forest sites and different seasons in order to obtain estimates of buoyancy heat flux. The required calibration of this method against eddy covariance resulted in a value for a specific parameter that is close to the range reported in other studies, contributing to the generalization of the SR method to different kinds of canopies. The comparison with fluxes obtained using the eddy covariance technique revealed a good match between the two methods for different sites, heights and seasons. Sites with high levels of non-stationarity in the signals of temperature and wind speed presented higher scatter in the regression with fluxes from eddy covariance. For a particular site with previously reported influence of low-frequency motions, the regression was only satisfactory, i.e., slope parameter close to unity and small offset, when oscillations with periods longer than $\approx $ ≈ 13 min were filtered out. The SR method has a great potential due to the simplicity of the instrumentation required. However, care should be taken when measuring under the influence of mesoscale motions, which can lead to high levels of non-stationarity, compromising the fundamental concepts of the SR theory. 相似文献