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11.
Brent L. Lewis Pamela D. Holt Steven W. Taylor Steven W. Wilhelm Charles G. Trick Alison Butler George W. Luther III 《Marine Chemistry》1995,50(1-4)
Thermodynamic stability constants have been estimated for the complexation of iron(III) with catecholate-type siderophores isolated from the marine bacterium Alteromonas luteoviolacea and from the marine cyanobacterium Synechococcus sp. PCC 7002. Stability constants were determined utilizing the “chelate scale” of Taylor et al. (1994). The scale is based upon a linear relationship between the reduction potentials and the pH-independent thermodynamic stability constants for known iron(III) complexes. Log K values for the alterobactin B ferric iron complex are 43.6 ± 1.5 at pH 8.2 and 37.6 ± 1.2 at pH 6, consistent with a shift from bis-catecholate to monosalicylate/monocatecholate iron coordination with decreasing pH. Synechococcus isolates PCC 7002 Nos. 1 and 3 formed iron(III) complexes with stability constants of approximately 38.1 ± 1.2 and 42.3 ± 1.5, respectively. The binding strengths of the iron(III) complexes examined in this study are quite high, suggesting that catecholate siderophores may play a role in the solubilization and biological uptake of iron in the marine environment. 相似文献
12.
An elongated sea bed depression (pit), 80 by 125 m and 10 m deep located on the Grand Banks of Newfoundland was identified on high resolution surficial geophysical survey lines and investigated using a manned submersible. The pit occurs at the termination of a long (greater than 3 km) iceberg scour, 1.5 m deep, and 80 m wide in 91 m of water. It is similar to other depressions in the region that indent the sea bed up to seven times deeper than the surrounding deepest iceberg furrows. The pit is interpreted to be the sea bed response to impact and loading by a rolling and grounding iceberg. The iceberg scour and pit appear to be of recent origin. 相似文献
13.
Rates for nitrification, phytoplankton uptake of ammonium, and regeneration of ammonium were measured in the Delaware River as functions of irradiance and nutrient concentrations, using 15N labeling methods. Phytoplankton uptake increased and nitrification rates declined with increased light intensity. The irradiance level required for maximum uptake by phytoplankton was similar to that for maximal inhibition of nitrification (about 300μEm−2 s−1). Daily, water-column averaged rates, calculated by integration of the observed rate-intensity relationships, indicate that light plays a key role in regulating the balance between oxidation of NH4+ by bacteria and assimilation by phytoplankton in the Delaware. The results show that uptake of ammonium by phytoplankton in the dark may exceed uptake in the light in optically thick systems. 相似文献
14.
G. H. Sutton F. K. Duennebier B. Iwatake J. D. Tuthill B. T. R. Lewis J. Ewing 《Marine Geophysical Researches》1981,5(1):3-34
The purpose of the experiment was to determine the effects of coupling and bottom currents on ocean bottom seismometers. Twelve operational OBSs, three specially designed three-component systems, and a hydrophone were compared with each other. Unlike seismometers placed on hard rock at land stations, ocean bottom seismometers can be affected by soft sediments (which act as lossy mechanical springs) and by buoyancy. Coupling through soft sediments can modify the response to ground motion much as a low pass filter does, and high buoyancy tends to counteract this effect. These effects are observed in the Lopez data, which consist of signals from mechanical transient tests, cap shots, airgun pulses, and general background noise. The modification of response is pronounced for some instruments and barely noticeable in others. Instruments that stand high in the water relative to their base width tend to be susceptible to rocking motion that shows up as a mechanical cross coupling between horizontal and vertical motion. Correlation of Lopez results with coupling theory suggests that it is possible to design ocean bottom seismometers that will couple well to any sediment. Current levels at the Lopez site (<5 cm s-1) were too small to produce noticeable effect on any of the instruments; however, the same design criteria that will minimize coupling problems will also lessen problems caused by ocean currents.Hawaii Institute of Geophysics Contribution No. 1171. 相似文献
15.
Surface complexation modeling of Cu(II) adsorption on mixtures of hydrous ferric oxide and kaolinite
Tracy J Lund Carla M Koretsky Christopher J Landry Melinda S Schaller Soumya Das 《Geochemical transactions》2008,9(1):9
Background
The application of surface complexation models (SCMs) to natural sediments and soils is hindered by a lack of consistent models and data for large suites of metals and minerals of interest. Furthermore, the surface complexation approach has mostly been developed and tested for single solid systems. Few studies have extended the SCM approach to systems containing multiple solids. 相似文献16.
Schinus terebinthifolius (Brazilian pepper), a native of South America, is currently naturalized in 20 countries worldwide and can alter native systems
by displacing flora and forming monotypic stands. The primary described mechanism of seed dispersal is through consumption
of fruits by birds and mammals. We evaluated an alternative dispersal method by evaluating the potential for S. terebinthifolius growing in freshwater and estuarine environments to disperse via water currents. Specifically, we: (1) determined the duration
fruits remained buoyant in three salinities, (2) estimated the viability of seeds after 7 days in water, (3) estimated the
dispersal rate of floating solitary fruits, and (4) examined the role of boat wakes in moving seeds above mean high water
at the shoreline. The length of time fruits floated in 0 ppt water (4.9 days) was significantly less than 15 ppt saltwater
(6.2 days), and 30 ppt saltwater (6.9 days). After 7 days, over 13% of seeds remained viable in 0 ppt, 15 ppt, and 30 ppt
water. By combining mean dispersal rates and the mean number of days fruits floated, we calculated individual fruits could
be transported 16.9 km in 0 ppt and over 22 km in 15 and 30 ppt water. To increase germination, seeds must be stranded above
the intertidal zone. Wind wakes alone never achieved this result; however, boat wakes plus wind wakes significantly increased
the movement of fruits above the intertidal region into drier soils. The use of both vertebrate dispersal vectors and water
dispersal may potentially increase the rate of invasion, establishment, and survival of S. terebinthifolius in freshwater and estuarine environments. 相似文献
17.
18.
"This paper establishes and discusses briefly regional patterns and trends in crude birth, death, and natural increase rates in Russia and the USSR from the turn of the century to 1989. The study is based on a comparable regional framework and placed in the context of the demographic transition theory. It discusses sources, collection, and quality of data, as well as necessary estimating procedures. An attempt also is made to examine briefly regional age-standardized rates." 相似文献
19.
Chemical equilibrium calculations on the stability of pure and dissolved graphite and cohenite (Fe3C), several other carbides, and several carbonates have been carried out for a system with solar elemental abundances over a very wide range of temperature and pressure. The calculated abundances of condensed carbon compounds are similar to the observed inventories on Earth and Venus, but fully 10 times smaller than the minimum carbon abundance found in ordinary chondrites. The total carbon content of most iron meteorites is compatible with their origin as a cooling FeNiCSP solution which was saturated with dissolved carbon at the solidus, such as would be produced by melting an ordinary chondrite, not by direct condensation from or equilibrium with the primitive solar nebula. It is argued that the carbon content of Mars need not be appreciably greater than that of the Earth. Material with even lower formation temperatures than Mars, such as the primitive material in the asteroid belt, may retain substantially more carbon as disequilibrium polymeric organic matter, possibly by the Fischer-Tropsch mechanism favored by Anders. Carbonates are not found as equilibrium products in a solar-composition system, and are probably secondary alteration products. CaCO3 might, however, persist in a solar-composition gas at temperatures below 460°K and pressures below 10?6.6 bar. The most stable condensed carbon compounds are found to be graphite, Fe3C, and possibly TiC, all in solid solution in the metal phase. 相似文献
20.
The thermochemistry of several hundred compounds of twelve selected trace elements (Ge, Se, Ga, As, Te, Pb, Sn, Cd, Sb, Tl, In, and Bi) has been investigated for solar composition material along a Jupiter adiabat. The results indicate that AsF3, InBr, TlI, and SbS, in addition to CO, PH3, GeH4, AsH3, H2Se, HCl, HF, and H3BO3 proposed by Barshay and Lewis (1978), may be potential chemical tracers of atmospheric dynamics. The reported observations of GeH4 is interpreted on the basis of new calculations as implying rapid vertical transport from levels where T ? 800°K. Upper limits are also set on the abundances of many gaseous compounds of the elements investigated. 相似文献