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841.
13C and 1H NMR spectra were obtained for humic acids isolated from marine sediments. NMR shows great promise in identifying structural components of humic acids as some new and interesting structural features are identified. Aliphatic structures were found to constitute a much larger fraction of humic acids than previously thought, and they appeared to be highly branched. Although the aromatic content of terrestrial humic acid was found to be lower than expected, the aromaticity appears to be a specific discriminator of terrestrial/aquatic source types. A humic acid isolated from an anoxic algal sapropel was found to be composed predominantly of polyuronic acids and different than other aquatic sedimentary humic substances. 相似文献
842.
Mark J. Valencia 《Quaternary Research》1977,8(3):339-354
Global atmospheric and oceanic circulation effects of expansion of continental ice sheets initiated upwelling in the western equatorial Pacific and simultaneously intensified upwelling in the eastern equatorial Pacific; contraction of the ice sheets reversed the process. Published Pleistocene paleoclimatic stratigraphies correlated across the entire equatorial Pacific exhibit eight such cycles in the Brünhes epoch. The extrapolated chronostratigraphies for the equatorial Pacific compare favorably with published paleoclimatic schemes for the southeastern, eastern, and northern Pacific Ocean. The Southern Ocean record exhibits fewer, and possibly also consistently older, climatic variations. A time progression or lack of synchrony of marine Pleistocene climatic events is not inconsistent with modified “Milankovitch” hypotheses, such as that involving Antarctic ice-sheet instability. 相似文献
843.
Sungshan Wang Ian McDougall Neil Tetley T. Mark Harrison 《Earth and Planetary Science Letters》1980,49(1):117-131
The Kirin meteorite, a large (2800kg) H5 chondrite, fell in Kirin Province, China in 1976. A sample from each of the two largest fragments (K-1, K-2) yield40Ar/39Ar total fusion ages of 3.63 ± 0.02b.y. and 2.78 ± 0.02b.y. respectively.40Ar/39Ar age spectra show typical diffusional argon loss profiles. Maximum apparent ages of 4.36 b.y. (K-1) and ~4.0 b.y. (K-2) are interpreted as possible minimum estimates for the age of crystallization of the parent body.The40Ar/39Ar ages found for gas released at low temperature are about 2.2 b.y. for K-1 and about 0.5 b.y. for K-2, suggesting that this meteorite may have suffered two discrete collisional events that caused degassing of radiogenic argon. Modelling of possible thermal events in the parent body indicates that samples K-1 and K-2 were at a depth of less than 3 m from the base of an impact melt of a thickness less than 7 m and separated by no more than ~2 m from one another at the time of the heating event about 0.5 b.y. ago. Further, the duration of heating was probably less than a few years.Calculations from38Ar data yield exposure ages for samples K-1 and K-2 of about 5 m.y., similar to that found for many other H chondrites. 相似文献
844.
Mark K. Chang Jan W. Kwiatkowski Robert F. Nau Robert M. Oliver Karl S. Pister 《地震工程与结构动力学》1982,10(5):651-662
This paper outlines the use of discrete, autoregressive/moving-average (ARMA) models for identification and estimation of parameters in models derived from analysis of uniformly digitized earthquake ground motion acceleration data. Such models are of equal generality as compared to continuous-time models and have a number of significant advantages for purposes of digital analysis and simulation. The structure of ARMA models is briefly described, their relation to continuous models noted, and results of their application to a number of recorded accelerograms summarized. 相似文献
845.
Calculation of multicomponent chemical equilibria and reaction processes in systems involving minerals,gases and an aqueous phase 总被引:1,自引:0,他引:1
Mark H Reed 《Geochimica et cosmochimica acta》1982,46(4):513-528
The compositional characteristics of many geochemical systems which involve the interaction of natural aqueous solutions with minerals and gases are conveniently described using the following thermodynamic components: Cl?, SO4=, HS?, CO3=, H+, Na+, K+, Ca++, Mg++, Fe++, Zn++, Cu+, Al+++, SiO2 and H2O. A set of mass balance and mass action equations equal in number to the number of components plus the number of saturated minerals (and gases) is defined for a specified temperature, pressure and bulk composition. The mass balance equations include terms for minerals, gases and the molalities of aqueous complexes and dissociated species. This set of non-linear equations can be solved with the aid of a computer using'a Newton-Raphson technique. The calculation takes account of aqueous ion complexing, oxidation-reduction equilibria, activity coefficients, non-unit water activity and solid solutions. The use of H+, SO4=, HS? and H2O as components allows straightforward treatment of processes involving oxidation-reduction, evaporation, boiling and changes of total aqueous H+ due to hydrolysis, mineral reaction or temperature change. One product of this approach is a technique for calculating pH at high temperature from measurement of pH at room temperature.By linking a series of discrete overall heterogeneous equilibrium calculations in which incremental changes of bulk composition, temperature or pressure are made, dynamic geochemical processes can be modeled. Example calculations for two such processes are given. These are the heating of seawater from 25° to 300°C and the isothermal irreversible reaction of rhyolite with an aqueous solution at 250°C. 相似文献
846.
Donald R. Whitehead Stephen T. Jackson Mark C. Sheehan Barbara W. Leyden 《Quaternary Research》1982,17(2):241-257
The Christensen Mastodon Site, located in central Indiana, contains a rich assemblage of vertebrates (including mastodon, caribou, and giant beaver), invertebrates, and plant macrofossils in situ in lake and bog sediments of late-glacial age. Studies of pollen and plant macrofossils suggest the existence of open, white spruce-dominated boreal forests from >; 14,000 yr B.P. to ca. 13,000 yr B.P. The regional decline of spruce, local occurrence of black spruce, white spruce, and larch, immigration of many hardwood taxa (e.g., ash, oak, elm), and the initiation of bog development are recorded beginning about 13,000 yr B.P. Recent reconstructions of late-glacial and early postglacial vegetational changes provide a context for understanding the disappearance of mastodons. The dramatic and rapid restriction of boreal forests along the retreating ice margin from 11,000 to 9000 yr B.P. may have caused a substantial reduction of mastodon populations. A diminished population would be more susceptible to small-scale, stochastic events such as short-term extremes of weather, outbreaks of disease, or predation pressure from paleoindian hunters. 相似文献
847.
Mark A.S. McMenamin David J. Blunt Keith A. Kvenvolden Scott E. Miller Leslie F. Marcus Richard R. Pardi 《Quaternary Research》1982,18(2):174-183
Low aspartic acid d:l ratios and modern collagenlike concentration values indicate that amino acids in bones from the Rancho La Brea asphalt deposit, Los Angeles, California are better preserved than amino acids in bones of equivalent age that have not been preserved in asphalt. Amino acids were recovered from 10 Rancho La Brea bone samples which range in age from less than 200 to greater than 36,000 yr. The calibrated rates of aspartic acid racemization range from 2.1 to 5.0 × 10?6yr?1. Although this wide range of rate constants decreases the level of confidence for age estimates, use of the larger rate constant of 5.0 × 10?6yr?1 provides minimum age estimates which fit the known stratigraphic and chronologic records of the Rancho La Brea deposits. 相似文献
848.
Replicate groups of larvae from each of three female grass shrimp,Palaemonetes pugio, collected at each of six sites within Chesapeake Bay were reared in the laboratory to metamorphosis at 25°C, 25 ppt salinity. They were provided with approximately 300Artemia nauplii/larva/day. Sites were selected to provide both suspected Kepone® contaminated and non-contamined shrimp populations. A sample of eggs, adult females with and without eggs, and newly hatched larvae from each site were analyzed by Virginia Institute of Marine Science for Kepone as were postlarvae obtained through laboratory rearings. Females and eggs from the James River had highest concentrations of Kepone (0.63 and 0.47 ppm, respectively) with samples from the Lafayette River at the mouth of the James River having the second highest levels (0.04 and 0.4 ppm). Concentrations in ovigerous females and eggs in the populations most distant from the James (mouth of Potomac and upper Potomac River) were at or below the limits of detectability (0.001 to 0.015 ppm). In laboratory reared postlarvae from each site, concentrations of Kepone were undetectable. Despite these apparent differences in Kepone concentrations in the various populations we found no significant differences in larval survival, larval duration, or length of post-larvae attributable to site of origin. Highly significant differences in larval duration and size of post-larvae were attributable to parental variation. 相似文献
849.
850.
Mark A. Flock 《Quaternary Research》1983,20(2):165-176
The Savanna Terrace, composed of alternating red and gray clayey sediments of late Wisconsinan age, can be found in five states along the upper Mississippi valley from Pepin County, Wisconsin, to Jackson County, Illinois. The terrace is the highest glaciofluvial-lacustrine deposit without a loess cover in the upper Mississippi valley. Chemical, physical, and mineralogical data show that two different sources provided sediment. The red clay is believed to have come from Lake Superior sources, while the gray clay is believed to have come from sources farther west. Large-scale flood events from glacial Lakes Agassiz, Grantsburg, and Superior were probably the main contributors of the sediments. The red clay in the terrace is similar in composition to red glaciolacustrine sediment found in eastern and northern Wisconsin. It also is mineralogically similar to the Hinckley Sandstone and the Fond du Lac Formation, which occur under and around Lake Superior. Radiocarbon dates obtained from the lower Illinois valley indicate that the terrace sediments were deposited sometime between about 13,100 and 9500 yr ago. Soils developed on the terrace are variable in their physical, chemical, and mineralogical properties, which reflect the composition of the clayey sediments. 相似文献