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971.
Near-infrared (J, H and K bands) spectra of nine dark asteroids (chosen among a sample of supposed primitive objects between C and D classes) have been obtained at the Mauna Kea Observatory (Hawaii) with the 2.2-m telescope using KSPEC as spectrograph. The aim of this work was to search for evidence of the presence of organic materials in these objects as found in other planetary bodies as 5145 Pholus, and in some cometary nuclei. A careful analysis of the data has revealed flat or slightly redder spectra than the solar one for all observed asteroids. No evidence of distinct absorption features was found. 相似文献
972.
The kinetics of the aqueous phase reactions of NO3 radicals with HCOOH/HCOO– and CH3COOH/CH3COO– have been investigated using a laser photolysis/long-path laser absorption technique. NO3 was produced via excimer laser photolysis of peroxodisulfate anions (S2O
8
2–
) at 351 nm followed by the reactions of sulfate radicals (SO
4
–
) with excess nitrate. The time-resolved detection of NO3 was achieved by long-path laser absorption at 632.8 nm. For the reactions of NO3 with formic acid (1) and formate (2) rate coefficients ofk
1=(3.3±1.0)×105 l mol–1 s–1 andk
2=(5.0±0.4)×107 l mol–1 s–1 were found atT=298 K andI=0.19 mol/l. The following Arrhenius expressions were derived:k
1(T)=(3.4±0.3)×1010 exp[–(3400±600)/T] l mol–1 s–1 andk
2(T)=(8.2±0.8)×1010 exp[–(2200±700)/T] l mol–1 s–1. The rate coefficients for the reactions of NO3 with acetic acid (3) and acetate (4) atT=298 K andI=0.19 mol/l were determined as:k
3=(1.3±0.3)×104 l mol–1 s–1 andk
4=(2.3±0.4)×106 l mol–1 s–1. The temperature dependences for these reactions are described by:k
3(T)=(4.9±0.5)×109 exp[–(3800±700)/T] l mol–1 s–1 andk
4(T)=(1.0±0.2)×1012 exp[–(3800±1200)/T] l mol–1 s–1. The differences in reactivity of the anions HCOO– and CH3COO– compared to their corresponding acids HCOOH and CH3COOH are explained by the higher reactivity of NO3 in charge transfer processes compared to H atom abstraction. From a comparison of NO3 reactions with various droplets constituents it is concluded that the reaction of NO3 with HCOO– may present a dominant loss reaction of NO3 in atmospheric droplets. 相似文献
973.
O'Neill BC Gaffin SR Tubiello FN Oppenheimer M 《Tellus. Series B, Chemical and physical meteorology》1994,46(5):378-389
Non-steady state timescales are complicated and their application to specific geophysical systems requires a common theoretical foundation. We first extend reservoir theory by quantifying the difference between turnover time and transit time (or residence time) for time-dependent systems under any mixing conditions. We explicitly demonstrate the errors which result from assuming these timescales are equal, which is only true at steady state. We also derive a new response function which allows the calculation of age distributions and timescales for well-mixed reservoirs away from steady state, and differentiate between timescales based on gross and net fluxes. These theoretical results are particularly important to tracer-calibrated "box models" currently used to study the carbon cycle, which usually approximate reservoirs as well-mixed. We then apply the results to the important case of anthropogenic CO2 in the atmosphere, since timescales describing its behavior are commonly used but ambiguously defined. All relevant timescales, including lifetime, transit time, and adjustment time, are precisely defined and calculated from data and models. Apparent discrepancies between the current, empirically determined turnover time of 30-60 years and longer model-derived estimates of expected lifetime and adjustment time are explained within this theoretical framework. We also discuss the results in light of policy issues related to global warming, in particular since any comparisons of the "lifetimes" of different greenhouse gases (CO2, CH4, N2O, CFC's etc.) must use a consistent definition to be meaningful. 相似文献
974.
S. Sudhakar Arvind Kumar M. L. Arrawatia S. Sengupta 《Journal of the Indian Society of Remote Sensing》1994,22(3):155-168
Remote sensing techniques have been applied to classify tour density classes within each of the forest type along with other major landuse/landcover classes in the East district, Sikkim using IRS-1A LISS II satellite data pertaining to the period of November, 1988. The shadow problem in rugged terrain and difficulty in acquiring cloud free data for different seasons pose problems to achieve considerable mapping accuracy. In the present study, the forests of the district were delineated through supervised classification techniques using maximum likelihood algorithm into five forest types as sal forests, subtropical broad-leaved forests, Himalayan wet temperate forests, Rhododendron forests and alpine forests. The alpine forests were further stratified into two categories as moist alpine scrub and dry alpine scrub. The statistical data obtained from the present study shows that 55.47 percent of the total geographical area of the East district was under forest cover. An overall accuracy of more than 85 percent in correctly delineating forest classes was achieved. 相似文献
975.
We report the first detection of interstellar nitrogen sulfide (NS) in cold dark clouds. Several components of the 2 pi 1/2, J = 3/2 --> 1/2 and J = 5/2 --> 3/2 transitions were observed in TMC-1 and L134N. The inferred column density for TMC-1 is NNS approximately 8 x 10(12)cm-2 toward the NH3 peak in that cloud, and in L134N is NNS approximately 3 x 10(12)cm-2 toward the position of peak NH3 emission. These values correspond to fractional abundances relative to molecular hydrogen of fNS approximately 8 x 10(-10) for TMC-1, and fNS approximately 6 x 10(-10) for L134N. The NS emission is extended along the TMC-1 ridge and is also extended in L134N. The measured abundances are significantly higher than those predicted by some recent gas phase ion-molecule models. 相似文献
976.
The tendency of network bright points (NBPs) to form in their surface distribution non-random, small-scale clusters is studied by a 2-D nearest-neighbours test, based on observational data for the distance between separate NBPs. High-resolution photographs taken from long time series obtained at4308 with the 50-cm refractor of Pic du Midi Observatory are used. Three different epochs of the solar cycle were chosen. The results obtained suggest that the degree of clustering depends on the solar cycle phase. Supposing that the NBPs are good tracers of the kilogauss small-scale magnetic field, we use them to obtain information about the subphotospheric small-scale magnetic field organisation and its dependence on the solar cycle phase. 相似文献
977.
A WKB approach, based on the method of Connor, Hastie, and Taylor (1979), is used to obtain simple estimates of the critical
conditions for the onset of ideal MHD instabilities in line-tied solar coronal loops. The method is illustrated for the constant
twist, Gold-Hoyle (1960) field, and the critical conditions are compared with previous and new numerical results. For the
force-free case, the WKB estimate for the critical loop length reduces to
. For the sufficiently non-force-free case the critical length can be expressed in the forml
0 +l
1/m. The results confirm the findings of De Bruyne and Hood (1992) that for force-free fields them = 1 mode is the first mode to become unstable but for the sufficiently strong non-force-free case this reverses with them → ∞ mode being excited first. 相似文献
978.
David J. Barber John R. Beckett Julie M. Paque Edward Stolper 《Meteoritics & planetary science》1994,29(5):682-690
Abstract The crystallography and crystal chemistry of a new calcium-titanium-aluminosilicate mineral (UNK) observed in synthetic analogs to calcium-aluminum-rich inclusions (CAIs) from carbonaceous chondrites was studied by electron diffraction techniques. The unit cell is primitive hexagonal or trigonal, with a = 0.790 ± 0.002 nm and c = 0.492 ± 0.002 nm, similar to the lattice parameters of melilite and consistent with cell dimensions for crystals in a mixer furnace slag described by Barber and Agrell (1994). The phase frequently displays an epitactic relationship in which melilite acts as the host, with (0001)UNK | (001)mel and <10T0>UNK | <100>mel. If one of the two space groups determined by Barber and Agrell (1994) for their sample of UNK is applicable (P3ml or P31m), then the structure is probably characterized by puckered sheets of octahedra and tetrahedra perpendicular to the c-axis with successive sheets coordinated by planar arrays of Ca. In this likely structure, each unit cell contains three Ca sites located in mirror planes, one octahedrally coordinated cation located along a three-fold axis and five tetrahedrally coordinated cations, three in mirrors and two along triads. The octahedron contains Ti but, because there are 1.3–1.9 cations of Ti/formula unit, some of the Ti must also be in tetrahedral coordination, an unusual but not unprecedented situation for a silicate. Tetrahedral sites in mirror planes would contain mostly Si, with lesser amounts of Al while those along the triads correspondingly contain mostly Al with subordinate Ti. The structural formula, therefore, can be expressed as with Si + Ti = 4. Compositions of meteoritic and synthetic Ti-bearing samples of the phase can be described in terms of a binary solid solution between the end-members Ca3TiAl2Si3O14 and Ca3Ti(AlTi)(AlSi2)O14. A Ti-free analog with a formula of Ca3Al2Si4O14 synthesized by Paque et al. (1994) is thought to be related structurally but with the octahedral site being occupied by Al, that is 相似文献
979.
980.
As part of the NASA Space Infrared telescope Facility (SIRTF), a low noise multiplexer has been developed. The hybridization of this multiplexer to a high indium antimonide (InSb) photodiode array has resulted in a MWIR detector of outstanding performance. The multiplexer is made of a 256×256 array of source follower amplifiers on a 30 m square pitch. Random access binary decoders are used to access each pixel of the array, allowing any read-out scheme to be implemented. Dark current has been measured at temperatures ranging from 4K to 77K. Generation recombination currents dominate above 45K. With 100mV of reverse bias applied, less than 3×10-17 A is typical below 50K with 8×10-19 A (5 e-/s) at 4K. Under the same conditions 0.25 pA was measured at 77K. Read noise has been measured as low as 186 e- using non-correlated techniques. Detector QE is 50 to 80 % through the entire 1 to 5 m band. 相似文献