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91.
Progress in the introduction of coulometry for the analysis of total carbon dioxide (TCO2) in marine waters is described. An extractor—stripper removes CO2 that is measured coulometrically by the quantity of electricity (coulombs) used to electrogenerate OH? ions for the titration of the acid formed by the reaction of CO2 and ethanolamine. The equivalence point is detected photometrically with thymolphthalein as the indicator, and Faraday's Law relates coulombs to equivalents of titrant generated and CO2 determined so that there are no standard curves needed or titrants to standardize or store. Accuracy was determined by adding gelatin capsules containing 100–1500 μg C of pure CaCO3 into the stripper, and accuracies of better than ± 1 μg C were achieved. The best precision for natural seawater (± 1 standard error) of ± 0.5 μmol l?1 was found for 17 samples of Bermuda coastal waters having a mean TCO2 of 2007.2 μmol l?1 (0.05% CV). Sources of error and precautions are discussed. This method, which has been used successfully at sea, can be used to study a variety of marine phenomena involving TCO2. 相似文献
92.
Replicate portions of a Delaware salt marsh were enclosed in cylindrical microcosms and exposed to elevated levels of inorganic arsenic (arsenate). All biotic and abiotic components in dosed cylinders rapidly incorporated arsenic. Spartina blades showed the greatest arsenic enrichment, with dosed plants incorporating arsenic concentrations an order of magnitude higher than controls. Spartina detritus and sediments also exhibited greatly elevated arsenic concentrations. Virtually all of the arsenic was incorporated into plant tissue or strongly sorbed to cell surfaces. Thus, elevated arsenic concentrations in estuarine waters will be reflected in living and non-living components of a salt marsh ecosystem, implying that increased arsenic will be available to organisms within the marsh ecosystem. 相似文献
93.
94.
Surface waters of Alsea Bay, an unpolluted estuary on the Oregon coast, were analysed for nitrous oxide, nitrate and nitrite on a weekly or biweekly basis during the summer of 1979. The estuary was found to be a variable source of N2O to the atmosphere. Large and rapid increases in the concentrations of N2O, NO3?, and NO2? occurred at the beginning of the sampling period and are attributed to the influx of nutrient-rich upwelling water into the estuary with the tide. The subsequent decline in concentrations of nitrate, nitrite and nitrous oxide over the remainder of the summer is attributed to a decrease in upwelling intensity, a decline in nitrification rates and to assimilatory nitrate reduction. Measurements of nitrous oxide at six stations along the Alsea River were also made in September and October before and after the onset of the rainy season. Samples taken after flood conditions were established were systematically 50% higher than pre-flood samples. The data suggest that soil runoff results in elevated concentrations of N2O in rivers. 相似文献
95.
Alan M Bond Julie R Bradbury Henry A Hudson John S Garnham Peter J Hanna Stanley Strother 《Marine Chemistry》1985,16(1):1-9
Evidence was found that uptake of lead from seawater in both model and natural systems by the leaves of the seagrass Zostera muelleri does occur for live, dead and scraped leaves at all the lead concentrations tested. Positive uptake of lead was measured using the three analytical techniques of radio-tracer, differential pulse anodic stripping voltammetry and atomic absorption spectrometry; similar uptake profiles were obtained for each technique. Profiles always showed an initial rapid uptake phase followed by a gradual transition to a plateau phase at which an approximate equilibrium between lead attached to seagrass and free ionic lead in seawater was reached. The presence of active lead uptake processes was indicated in experiments which attempted to remove lead from leaves by a chelating agent. 相似文献
96.
The existence of prolonged periods of abnormally low solar activity (such as the Maunder minimum) is explained within the framework of Leighton's model of a solar cycle with a hypothetical internal magnetic field of the Sun taken into account. 相似文献
97.
The paper considers the random phase errors in the phase shifters which are used in an antenna array to steer the beam in the look direction, and analyzes the effect of these errors on the performance of the optimal processor which maximizes the output SNR by deriving the expressions for the output signal power, residual interference power, output SNR, and the array gain as a function of the variance of these errors. The paper also considers the phase quantization error which arises in the digital phase shifters and shows how the performance of the optimal processor depends on the number of bits of the digital phase shifters. 相似文献
98.
99.
G. Djurašević P. Rovithis H. Rovithis-Livaniou E. Fragoulopoulou 《Astrophysics and Space Science》2005,296(1-4):311-314
BV light curves of the eclipsing binary UV Leo obtained at the Kryonerion Astronomical Station of the National Observatory of
Athens, Greece, are analyzed. The analysis is based on a Roche configuration with two spots on the secondary surface. The
elements of the two components of the system are calculated and the spot characteristics are given. 相似文献
100.