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881.
The Preparation and Preliminary Characterisation of Eight Geological MPI-DING Reference Glasses for In-Situ Microanalysis 总被引:13,自引:4,他引:9
Klaus Peter Jochum Donald B. Dingwell Alexander Rocholl Brigitte Stoll Albrecht W. Hofmann S. Becker A. Besmehn D. Bessette H.-J. Dietze P. Dulski J. Erzinger E. Hellebrand P. Hoppe I. Horn K. Janssens G.A. Jenner M. Klein W.F. McDonough M. Maetz K. Mezger C. Müker I.K. Nikogosian C. Pickhardt I. Raczek D. Rhede H.M. Seufert S.G. Simakin A.V. Sobolev B. Spettel S. Straub L. Vincze A. Wallianos G. Weckwerth S. Weyer D. Wolf M. Zimmer 《Geostandards and Geoanalytical Research》2000,24(1):87-133
Eight silicate glasses were prepared by directly fusing and stirring 50-100 g each of basalt, andesite, komatiite, peridotite, rhyolite, and quartz-diorite. These are referred to as MPI-DING glasses and were made for the purpose of providing reference materials for geochemical, in-situ microanalytical work. Results from various analytical techniques indicate that individual glass fragments are well homogenised with respect to major and trace elements at the μm to mm scale. Heterogeneities due to quench crystallisation of olivine have been observed in small and limited areas of the two komatiitic glasses. In order to obtain concentration values for as many elements as possible, the glasses were analysed by a variety of bulk and microanalytical methods in a number of laboratories. The analytical uncertainties of most elements are estimated to be between 1% and 10%. From the analytical data, preliminary reference values for more than sixty elements were calculated. The analytical uncertainties of most elements are estimated to be between 1% and 10%. 相似文献
882.
Cristina?PulidoEmail author Kaj?Sand-Jensen Esther?C.?H.?E.?T.?Lucassen Jan?G.?M.?Roelofs Klaus?P.?Brodersen Ole?Pedersen 《Aquatic Sciences - Research Across Boundaries》2012,74(2):351-360
Isoetids, as indicators of near-pristine softwater lakes, have a high priority in national and international (European Water
Directive Framework) assessments of ecological lake quality. Our main goal was to identify the most important environmental
factors that influence the composition of plant communities and specifically determine the presence and abundance of the isoetid
Lobelia dortmanna in NW European softwater lakes. Geographical position and composition of surface water, porewater, sediment and plant communities
were examined in 39 lakes in four regions (The Netherlands, Denmark, West Norway and East Norway) distributed over a 1,200-km
long distance. We confirmed that lake location was accompanied by significant changes in environmental variables between NW
European lakes. Lake location was the single most important determinant of vegetation composition and it had significant individual
contributions independent of the coupling to environmental variables. This influence of location was supported by a significant
decline of community similarity with geographical distance between pairs of lakes at regional, inter-regional and international
scales. Combining the geographical position with environmental variables for surface water, porewater and sediment significantly
improved prediction of vegetation composition. Specifically, the combination of latitude, surface water alkalinity, porewater
phosphate and redox potential offered the highest correlation (BIO ENV correlation 0.66) to vegetation composition. This complex
analysis can also account for high sediment variability in the littoral zone of individual lakes, by using site-specific physico-chemical
sediment factors, and offer better predictions of vegetation composition when lake water chemistry is relatively homogeneous
among lakes within regions. 相似文献
883.
Much attention has recently been devoted to the fate and effects of pharmaceuticals in the water cycle. Removal of antibiotics in effluents by photo‐treatment or biodegradation is a topic currently under discussion. Degradation and removal efficiencies of sulfisomidine (SUI) by photodegradation and aerobic biodegradability were studied. SUI behavior was monitored during photolysis and photocatalysis (catalyst titanium dioxide) using 150‐W medium‐pressure Hg lamp. Also an aerobic bacterial degradation test from the OECD series (closed bottle test (CBT, OECD 301 D)) was performed. The primary elimination of SUI was monitored. Structures of photo‐degradation products were assessed by chromatographic separation on a C18 column with ultraviolet detection at 270 nm and ion trap MS. The results demonstrate that SUI is not readily biodegradable in CBT. Photo catalysis was more is effective than photolysis. SUI underwent photodegradation and several SUI photoproducts were identified. Accordingly, the photodegradation pathway of SUI was postulated. When reaching the aquatic environment, SUI and its photo products can constitute a risk to the environment. 相似文献
884.
Abstract— We present a numerical simulation technique for the retrieval of the electric properties relative permittivity and conductivity of planetary, asteroid, and cometary regolith. Our simulation techniques aim at accompanying hardware development and conducting virtual experiments, e.g., to assess the response of arbitrary heterogeneous conductivity and permittivity distributions or to scrutinize possibilities for spatial reconstruction methods using inverse schemes. In a first step, we have developed a finite element simulation code on the basis of unstructured, adaptive triangular grids for arbitrary two‐dimensional axisymmetric distributions of conductivity and permittivity. The code is able to take into account the spatial geometry of the probe and allows for possible inductive effects. In previous studies, the non‐inductive approach has been used to convert potential and phase data into apparent material properties. By our simulations, we have shown that this approach is valid for the frequency range from 102 Hz to 107 Hz and electric conductivities of 10?8 S/m that are typical for the near‐surface region of asteroids and comets composed of chondritic materials and/or frozen volatiles such as H2O and CO2 ice. We prove the accuracy of our code to be better than 10%, using mixed types of boundary conditions and present a simulated vertical log through a horizontally stratified subsurface layer as a representative example of a heterogeneous distribution of the electrical properties. Resolution studies for the given electrode separation reveal that the material parameters of layers having thicknesses of less than about half the electrode spread are not reconstructible if only apparent quantities are considered. Therefore, spatial distributions of the complex sensitivity are presented having in mind a future data inversion concept that will permit the multi‐dimensional reconstruction of material parameters in heterogeneous environments. 相似文献
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888.
It is well known that the neutral component of the local interstellar medium can effectively pass through the plasma interface ahead of the solar system and can penetrate deeply into the inner heliosphere. Here we present a newly-developed theoretical approach to describe the distribution function of LISM neutral hydrogen in the heliosphere, also taking into account time-dependent solar and interstellar boundary conditions. For this purpose we start from a Boltzmann-Vlasov equation, Fourier-transformed with respect to space and time coordinates, in connection with correspondingly transformed solar radiation forces and ionization rates, and then arrive at semi-analytic solutions for the transformed hydrogen velocity distribution function. As interstellar boundary conditions we allow for very general, non-Maxwellian and time-dependent distribution functions to account for the case that some LISM turbulence patterns or nonlinear wave-like shock structures pass over the solar system. We consider this theoretical approach to be an ideal instrument for the synoptic interpretation of huge data samples on interplanetary Ly- resonance glow intensities registered from different celestial directions over extended periods of time. In addition we feel that the theoretical approach presented here, when applied to interplanetary resonance glow data, may permit the detection of genuine fluctuations in the local interstellar medium. 相似文献
889.
Authors Index
Author Index Volume 56 相似文献890.
Andreas?M?llerEmail author Bas?J.?Hensen Richard?A.?Armstrong Klaus?Mezger Michel?Ballèvre 《Contributions to Mineralogy and Petrology》2003,145(4):406-423
The age of Proterozoic granulite facies metamorphism and deformation in the Strangways Metamorphic Complex (SMC) of central Australia is determined on zircon grown in syn-metamorphic and syn-deformational orthopyroxene-bearing, enderbitic, veins. SHRIMP zircon studies suggest that M 1–M 2 and the correlated periods of intense deformation (D 1–D 2) are part of a single tectonothermal event between 1,717±2 and 1,732±7 Ma. It is considered unlikely that the two metamorphic phases (M 1, M 2) suggested by earlier work represent separate events occurring within 10–25 Ma of each other. Previous higher estimates for the age of M 1 granulite metamorphism in the SMC (Early Strangways event at ca. 1,770 Ma) based on U–Pb zircon dating of granitic, intrusive rocks, are not believed to relate to the metamorphism, but to represent pre-metamorphic intrusion ages. Conventional multi-grain U–Pb monazite analyses on high-grade metasediments from three widely spaced localities in the western SMC yield 207Pb/ 235U ages between 1,728±11 and 1,712±2 Ma. The age range of the monazites corresponds to the SHRIMP zircon ages in the granulitic veins and is interpreted to record monazite growth (prograde in the metasedimentary rocks). The data imply a maximum time-span of 30 Ma for high-grade metamorphism and deformation in the SMC. There is, thus, no evidence for an extremely long period of continuous high-temperature conditions from 1,770 to ca. 1,720 Ma as previously proposed. The results firmly establish that the SMC has a very different high-grade metamorphic history than the neighbouring Harts Range, where upper amphibolite facies metamorphism in the Palaeozoic caused widespread growth or recrystallization of monazite. 相似文献