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151.
Christopher Packham Keith L. Thompson Almudena Zurita Johan H. Knapen Ian Smail Robert Greimel Daniel F. M. Folha Chris Benn rew Humphrey Rene Rutten David Ciardi Matthieu Bec Richard Bingham Simon Craig Kevin Dee Derek Ives Paul Jolley Peter Moore Marti Pi i Puig Simon Rees Gordon Talbot Sue Worswick 《Monthly notices of the Royal Astronomical Society》2003,345(2):395-405
152.
The in vitro aryl hydrocarbon receptor (AhR) agonist potency of offshore produced water effluents, collected from the United Kingdom Continental Shelf, was determined using the dioxin responsive (DR)-chemically activated luciferase expression (CALUX) assay. Octadecylsilane (C18) solid phase extraction (SPE) extracts of produced water were exposed to DR-CALUX cells for 24 h in order to investigate the contribution in potency from compounds that are stable to metabolism by the CALUX cells during exposure. The stable AhR agonist potency determined over 24 h was highly variable and ranged from 1 to 430 ng TCDD TEQCALUX l−1. These data reflect the highly variable composition of produced water discharges from different production fields. It is recommended that further work be performed to characterise the full range of stable dioxin like AhR agonists present in offshore produced water discharges using techniques such as bioassay-directed analysis. 相似文献
153.
Pedoja Kevin 《中国科学D辑(英文版)》2005,48(11):1900-1912
The importance of calcimicrobes and microbialite in carbonate platform and reefal environments has been stressed in recent literature. Burne and Moore[1] introduced the term microbialite to describe the clotted, laminated and undifferentiated fabrics formed by mi-crobial communities. Microbialites are organosedi-mentary deposits that have accreted as a result of ben-thic (prokaryotic or eukaryotic) communities, trapping and binding detrital sediment[1]. Microbial organisms and microbialite are… 相似文献
154.
In the three decades since their discovery, the accumulated body of observational data from pulsar sources puts constraints on models that seek to explain their periodic radiation. This paper reviews this data, reports on a VLA search for haloes predicted by an early model, and reinvestigates a magnetospheric disk-field-aligned-current transmission line system as the origin of the observed radiation, with external wave excitation by as yet an unexplained source. Three dimensional, fully electromagnetic particle-in-cell simulations of the pulsar surface and magnetosphere are used to explore the waveshape and polarization properties of the observed radiation. 相似文献
155.
Eric?Rodriguez Kevin?A.?McGuinness Duke?U.?OphoriEmail author 《Environmental Geology》2004,45(5):623-632
An initial assessment of an old manufacturing site with groundwater impacted by trichloroethene (TCE) contamination in the metropolitan New York area showed that the TCE was being removed naturally by reductive dechlorination. However, complete dechlorination was not expected at the site because the process was progressing too slowly under transitional to aerobic conditions at a degradation constant of –0.0013 and a TCE half life of 533 days. A pilot test was conducted at the site in which a carbohydrate substrate (molasses) was injected into the groundwater to create an In-Situ Reactive Zone (IRZ). Post-pilot test groundwater sampling and analysis indicated that an IRZ was created successfully as the total organic carbon (TOC) content and conductivity increased significantly while oxidation-reduction (REDOX) potential and dissolved oxygen (DO) decreased. The created IRZ caused enhanced reductive dechlorination of TCE at the site, found to proceed with a degradation constant of –0.0158 and a TCE half life of 44 days. 相似文献
156.
William J. Green Brian R. Stage Bonnie Jo Bratina Shannon Wagers Adam Preston Kevin O’bryan Joseph Shacat Silvia Newell 《Aquatic Geochemistry》2004,10(3-4):303-323
Lake Vanda is a closed-basin, permanently ice-covered lake located in the Wright Valley of Antarctica. The lakes more important geochemical features include the fact that it is fed by a single glacial melt water stream for only 6–8weeks out of the year; that it has remained stratified for more than a millennium; and that, like other lakes in the region, it is remote from anthropogenic influence. These, together with the fact that it is among the least biologically productive lakes in the world, make it an ideal system for examining the transport, cycling and fate of trace metals in the aquatic environment. Like others before us, we view this lake as a natural geochemical laboratory, a flask in the desert. This paper presents the first set of closely spaced, vertical, profiles for dissolved and particulate Mn, Fe, Ni, Cu, Zn and Cd in the water column. Despite the absence of an outflow, metals in the fresh upper waters of the lake have extremely low concentrations, in the pico-molar to nano-molar range, and are partitioned largely into dissolved rather than particulate phases. Efficient metal scavenging by particles from these oxygen-rich waters is indicated. Significant increases in metal concentrations begin to appear at depth, between 57 and 60m, and these increases coincide with the onset of manganese oxide dissolution in oxic, but lower pH waters. Vertical profiles suggest that the entire suite of trace metals (Ni, Cu, Zn, and Cd) is being released from manganese oxide carrier phases. Thermodynamic analysis indicates that Mn3 O4 (i.e., the mineral hausmannite) may be important in metal sequestration and recycling in the deeper waters of Lake Vanda. Manganese-reducing organisms reported by Bratina etal. (1998) are active in the zone of metal release and these could also contribute to the observed cycling. 相似文献
157.
A field study was conducted using a combination of intrinsic and artificial tracers to estimate travel times and dilution during transport of infiltrate from a reclaimed water infiltration basin to nearby monitoring wells. A major study objective was to validate boric acid enriched in (10)B as an artificial tracer. Basin 10E at the Rio Hondo Spreading Grounds in Whittier, California, was the site of the test. The basin normally receives a mixture of treated municipal waste water, purchased State Project water, and local runoff from the San Gabriel River. Approximately 3.5 kg of (10)B-enriched boric acid was dispersed among 2.05 x 10(5) m(3) of basin water to initiate the experiment. The resultant median delta(11)B in the infiltration basin was -71 per thousand. Prior to tracer addition, the basin water had an intrinsic delta(11)B of +2 per thousand. Local monitoring wells that were used to assess travel times had delta(11)B values of +5 per thousand and +8 per thousand at the time of tracer addition. Analytic results supported an assumption that boron is conserved during ground water transport and that boron enriched in (10)B is a useful artificial tracer. Several intrinsic tracers were used to reinforce the boric acid tracer findings. These included stable isotopes of oxygen (delta(18)O) and hydrogen (deltaD), sulfate concentration, and the boron to chloride ratio. Xenon isotopes, (136)Xe and (124)Xe, also supported boron isotope results. Xenon isotopes were added to the recharge basin as dissolved gases by investigators from the Lawrence Livermore National Laboratory. 相似文献
158.
Matthew J. Wooller John W. Pohlman Benjamin V. Gaglioti Peter Langdon Miriam Jones Katey M. Walter Anthony Kevin W. Becker Kai-Uwe Hinrichs Marcus Elvert 《Journal of Paleolimnology》2012,48(1):27-42
Atmospheric contributions of methane from Arctic wetlands during the Holocene are dynamic and linked to climate oscillations. However, long-term records linking climate variability to methane availability in Arctic wetlands are lacking. We present a multi-proxy ~12,000?year paleoecological reconstruction of intermittent methane availability from a radiocarbon-dated sediment core (LQ-West) taken from a shallow tundra lake (Qalluuraq Lake) in Arctic Alaska. Specifically, stable carbon isotopic values of photosynthetic biomarkers and methane are utilized to estimate the proportional contribution of methane-derived carbon to lake-sediment-preserved benthic (chironomids) and pelagic (cladocerans) components over the last ~12,000?years. These results were compared to temperature, hydrologic, and habitat reconstructions from the same site using chironomid assemblage data, oxygen isotopes of chironomid head capsules, and radiocarbon ages of plant macrofossils. Cladoceran ephippia from ~4,000?cal?year BP sediments have ??13C values that range from ~?39 to ?31??, suggesting peak methane carbon assimilation at that time. These low ??13C values coincide with an apparent decrease in effective moisture and development of a wetland that included Sphagnum subsecundum. Incorporation of methane-derived carbon by chironomids and cladocerans decreased from ~2,500 to 1,500?cal?year BP, coinciding with a temperature decrease. Live-collected chironomids with a radiocarbon age of 1,640?cal?year BP, and fossil chironomids from 1,500?cal?year BP in the core illustrate that ??old?? carbon has also contributed to the development of the aquatic ecosystem since ~1,500?cal?year BP. The relatively low ??13C values of aquatic invertebrates (as low as ?40.5??) provide evidence of methane incorporation by lake invertebrates, and suggest intermittent climate-linked methane release from the lake throughout the Holocene. 相似文献
159.
160.
Well before President Putin ratified the Kyoto Protocol, the debate had begun as to the appropriate form of any post-Kyoto agreement. Amongst the emission reduction regimes being considered is that of Contraction and Convergence; conceived by Global Commons Institute (GCI) as a practical interpretation of the philosophy that “every adult on the planet has an equal right to emit greenhouse gases”. To support the Contraction and Convergence regime, the GCI have developed a computer model, CCOptions, to correlate CO2 stabilisation levels with global, regional and national carbon reduction targets. This paper analyses the model, concluding that, whilst the aim of CCOptions is laudable, the application of the model in its current form is unnecessarily ambitious and as a consequence potentially misleading to all but the well-informed user. 相似文献