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201.
Yousif K. Kharaka James J. Thordsen Susan D. Hovorka H. Seay Nance David R. Cole Tommy J. Phelps Kevin G. Knauss 《Applied Geochemistry》2009
Sedimentary basins in general, and deep saline aquifers in particular, are being investigated as possible repositories for large volumes of anthropogenic CO2 that must be sequestered to mitigate global warming and related climate changes. To investigate the potential for the long-term storage of CO2 in such aquifers, 1600 t of CO2 were injected at 1500 m depth into a 24-m-thick “C” sandstone unit of the Frio Formation, a regional aquifer in the US Gulf Coast. Fluid samples obtained before CO2 injection from the injection well and an observation well 30 m updip showed a Na–Ca–Cl type brine with ∼93,000 mg/L TDS at saturation with CH4 at reservoir conditions; gas analyses showed that CH4 comprised ∼95% of dissolved gas, but CO2 was low at 0.3%. Following CO2 breakthrough, 51 h after injection, samples showed sharp drops in pH (6.5–5.7), pronounced increases in alkalinity (100–3000 mg/L as HCO3) and in Fe (30–1100 mg/L), a slug of very high DOC values, and significant shifts in the isotopic compositions of H2O, DIC, and CH4. These data, coupled with geochemical modeling, indicate corrosion of pipe and well casing as well as rapid dissolution of minerals, especially calcite and iron oxyhydroxides, both caused by lowered pH (initially ∼3.0 at subsurface conditions) of the brine in contact with supercritical CO2. 相似文献
202.
Road-deposited sediment (RDS) is an accumulation of particulates upon street surfaces in urban centres. It is commonly highly contaminated and has major potential impacts upon surface water quality and human health, as well as becoming a waste material upon street sweeping. Although significant research has been undertaken upon the fine fraction within these systems, there is a lack of detailed, high-resolution grain-specific mineralogical and chemical data for the coarser fractions, which contain the bulk of the contamination by mass. The study reported here utilizes backscatter electron microscopic, electron microprobe and Raman spectroscopic analysis to provide novel data on RDS material from Manchester, UK, with significant implications for the improved understanding of source discrimination and contaminant metal speciation. The RDS samples studied are highly heterogeneous and the abundant nature of anthropogenic grains is particularly apparent. The RDS material has been found to be composed of a number of grain types: (i) silicate and alumino-silicate grains derived from a wide range of sources; (ii) iron oxide grains derived from the corrosion of galvanized steel; (iii) iron-rich glass grains derived as slag material from metal and waste processing activities and (iv) spherical Fe oxide and Fe-rich glass grains derived from high temperature combustion processes. Elemental metallic grains (Fe, Cu, Pb) are also present in minor amounts. 相似文献
203.
Variation in DOC and trace metal concentration along the heavily urbanized basin in Kathmandu Valley,Nepal 总被引:1,自引:0,他引:1
Water samples were analyzed for DOC and trace metals from Bagmati River within Kathmandu valley, Nepal, to understand the
variation trends of DOC and trace metals and their relationship along the drainage network. The variability in organic matter
and wastewater input within the Bagmati drainage basin appeared to control DOC and most of the trace metal concentration.
The large input of organic matter and wastewater creates anoxic condition by consuming dissolved oxygen and releasing higher
concentrations of DOC, trace elements such as nickel, arsenic, barium, cadmium, and copper with downstream distance. Concentrations
of DOC and trace metals like barium and zinc showed strong relationships with human population density and suggest that human
activities have strong control on these parameters along the drainage network. The DOC and most of the trace metal concentration
increased with downstream distance and appeared to be directly associated with human activities. The variation trends of most
of the trace metals appeared to be the same; however, concentration varied widely. Inputs of organic matter and wastewater
due to human activities appeared directly to be associated for the variation of DOC and trace metals along the Bagmati drainage
network within Kathmandu valley. 相似文献
204.
Leigh N. Fletcher Kevin H. Baines Adam P. Showman Glenn S. Orton C. Merlet 《Icarus》2011,214(2):510-533
The latitudinal variation of Saturn’s tropospheric composition (NH3, PH3 and AsH3) and aerosol properties (cloud altitudes and opacities) are derived from Cassini/VIMS 4.6-5.1 μm thermal emission spectroscopy on the planet’s nightside (April 22, 2006). The gaseous and aerosol distributions are used to trace atmospheric circulation and chemistry within and below Saturn’s cloud decks (in the 1- to 4-bar region). Extensive testing of VIMS spectral models is used to assess and minimise the effects of degeneracies between retrieved variables and sensitivity to the choice of aerosol properties. Best fits indicate cloud opacity in two regimes: (a) a compact cloud deck centred in the 2.5-2.8 bar region, symmetric between the northern and southern hemispheres, with small-scale opacity variations responsible for numerous narrow light/dark axisymmetric lanes; and (b) a hemispherically asymmetric population of aerosols at pressures less than 1.4 bar (whose exact altitude and vertical structure is not constrained by nightside spectra) which is 1.5-2.0× more opaque in the summer hemisphere than in the north and shows an equatorial maximum between ±10° (planetocentric).Saturn’s NH3 spatial variability shows significant enhancement by vertical advection within ±5° of the equator and in axisymmetric bands at 23-25°S and 42-47°N. The latter is consistent with extratropical upwelling in a dark band on the poleward side of the prograde jet at 41°N (planetocentric). PH3 dominates the morphology of the VIMS spectrum, and high-altitude PH3 at p < 1.3 bar has an equatorial maximum and a mid-latitude asymmetry (elevated in the summer hemisphere), whereas deep PH3 is latitudinally-uniform with off-equatorial maxima near ±10°. The spatial distribution of AsH3 shows similar off-equatorial maxima at ±7° with a global abundance of 2-3 ppb. VIMS appears to be sensitive to both (i) an upper tropospheric circulation (sensed by NH3 and upper-tropospheric PH3 and hazes) and (ii) a lower tropospheric circulation (sensed by deep PH3, AsH3 and the lower cloud deck). 相似文献
205.
Chemistry on the icy surface of Europa is heavily influenced by the incident energetic particle flux from the jovian magnetosphere. The majority (>75%) of this energy is in the form of high energy electrons (extending to >10 MeV). We have simulated the electron irradiation environment of Europa with a vacuum system containing a high-energy electron gun for irradiation of ice samples formed on a gold mirror cooled with a cryostat. Pure water films of ∼2.6 μm thickness were grown at 100 K and then either cooled (to 80 K), warmed (to 120 K) or left at 100 K and subsequently irradiated with 10 keV electrons. The production of hydrogen peroxide (H2O2) was monitored by observation of the 2850 cm−1 (3.5 μm) band. Equilibrium concentrations of H2O2, in units of percent by number H2O2 relative to water, were found to be 0.043% (80 K), 0.029% (100 K), and 0.0063% (120 K). These values are 33%, 22%, and 5%, respectively, that of the reported surface concentration on the leading hemisphere of Europa (Carlson, R.W., Anderson, M.S., Johnson, R.E., Smythe, W.D., Hendrix, A.R., Barth, C.A., et al. [1999]. Science 283(5410), 2062-2064) and less than the equilibrium concentrations formed by ion irradiation. In addition to the ice film temperature, the current of electrons was varied between different experiments to determine the production and destruction of H2O2 as a function of both electron flux and ice temperature. Variation in current was found to have little effect on the results other than accelerating arrival at radiolytic equilibrium. 相似文献
206.
The distribution of adult Trichoptera in light traps was investigated alongside nine streams draining catchments under native forest, pine forest, or pasture near Hamilton, Waikato, New Zealand. The aim of the study was to determine the relationship between abundance, taxonomic richness, and community composition with respect to land use during summer, and to evaluate the use of adult Trichoptera compared with benthic invertebrates as potential bio‐indicators of the effectiveness of land‐management changes. Adult Trichoptera faunas alongside the native streams were dominated by Hydrobiosidae, Conoesucidae, and Helicopsychidae (each >10% of total Trichoptera numbers for at least two of the three sites), whereas Leptoceridae, Oeconescidae, and Hydrobiosidae were relatively abundant alongside at least two of the pine sites. Adult Trichoptera faunas at the pasture sites were strongly dominated by Hydroptilidae which made up 47–85% of numbers caught at all sites. The mean number of individuals and taxa caught in light traps increased from November to January and then declined in February for all land‐use types. Overall, total numbers and taxonomic richness of adult Trichoptera were significantly lower at the pine sites compared to the pasture or native sites. TWINSPAN classification of benthic invertebrates collected in November clearly differentiated sites based on land use for presence/absence and percentage abundance data. A similar pattern was evident for most sites when adult Trichoptera faunas were used for the four sampling dates combined, suggesting that light trapping has potential as a tool for bio‐monitoring. 相似文献
207.
Applying Bayesian belief networks to health risk assessment 总被引:1,自引:0,他引:1
Kevin Fong-Rey Liu Che-Fan Lu Cheng-Wu Chen Yung-Shuen Shen 《Stochastic Environmental Research and Risk Assessment (SERRA)》2012,26(3):451-465
The health risk of noncarcinogenic substances is usually represented by the hazard quotient (HQ) or target organ-specific
hazard index (TOSHI). However, three problems arise from these indicators. Firstly, the HQ overestimates the health risk of
noncarcinogenic substances for non-critical organs. Secondly, the TOSHI makes inappropriately the additive assumption for
multiple hazardous substances affecting the same organ. Thirdly, uncertainty of the TOSHI undermines the accuracy of risk
characterization. To address these issues, this article proposes the use of Bayesian belief networks (BBN) for health risk
assessment (HRA) and the procedure involved is developed using the example of road constructions. According to epidemiological
studies and using actual hospital attendance records, the BBN-HRA can specifically identify the probabilistic relationship
between an air pollutant and each of its induced disease, which can overcome the overestimation of the HQ for non-critical
organs. A fusion technique of conditional probabilities in the BBN-HRA is devised to avoid the unrealistic additive assumption.
The use of the BBN-HRA is easy even for those without HRA knowledge. The input of pollution concentrations into the model
will bring more concrete information on the morbidity and mortality rates of all the related diseases rather than a single
score, which can reduce the uncertainty of the TOSHI. 相似文献
208.
Kevin Leleu Frédérique AlbanDominique Pelletier Eric CharbonnelYves Letourneur Charles F. Boudouresque 《Marine Policy》2012,36(2):414-422
How users perceive the performance of Marine Protected Areas (MPAs) is fundamental for the social acceptance of these zones. Moreover, their perceptions may be relevant for monitoring the effects of MPAs on extractive activities. This study analyzes artisanal fishers' perceptions of the performance of a north-western Mediterranean coastal MPA, which encompasses two no-take zones (NTZs). Three viewpoints have been considered: the effect on the personal activity of fishers, the effect on the local fishery and the effect on the ecosystem. In order to test the hypothesis that biomass export (spillover) - which had previously been evidenced from the two NTZs - may influence fishers' perceptions of NTZ effects, fishers' perceptions were compared with both declared and observed fishing activity over an one-year period.The results show that negative perceptions of NTZs are either nil or are negligible. Most fishers are aware of the beneficial effects of NTZs on ecosystems and fisheries. However, they remain to be convinced of the beneficial effects of the NTZs on their own activity. For instance, the proximity of a NTZ appears never to be involved in the choice of a fishing spot. This partial lack of correspondence between scientific expectation and fishers' perceptions is discussed in the light of fishing habits in the zone adjacent to NTZs, and takes into account fishing grounds, targeted species and seniority (defined as the number of years the fisher has been fishing within the MPA). All three factors appear to influence fishers' perceptions. For example, having a positive perception about a NTZ and spending more time fishing in the adjacent zone are habits that can be associated with fishers with less seniority. Fishers' perceptions obviously indicate the social acceptance of the MPA and are an essential monitoring tool for MPA managers. However, perceptions cannot be seen as a substitute for scientific monitoring, as both approaches are clearly complementary. 相似文献
209.
A model problem of the flow under an air-cushion vessel is studied. Two different numerical techniques are used to determine the solution of the free-surface elevation and the wave resistance for a range of Froude number, Reynolds number, value of the pressure applied in the cushion, and depth of the water. The first numerical technique uses a velocity potential that satisfies linearized free-surface boundary conditions, whereas the second employs a finite-volume method to find a solution that satisfies the fully nonlinear free-surface boundary conditions. The results clearly show that for high Froude number and practical values of the cushion pressure, the linear-theory solution is in excellent agreement with the more exact nonlinear prediction. For lower Froude number the solution becomes unsteady, and the disagreement between the two methods is larger. 相似文献
210.
Variability of suspended particulate matter in the Bohai Sea from the geostationary Ocean Color Imager (GOCI) 总被引:2,自引:0,他引:2
Kevin Ruddick Quinten Vanhellemont Jing Yan Griet Neukermans Guomei Wei Shaoling Shang 《Ocean Science Journal》2012,47(3):331-345
This study assesses the performance of the Geostationary Ocean Imager (GOCI) for mapping of suspended particulate matter in the Bohai Sea, a turbid water region. GOCI imagery for remote sensing reflectance and Total Suspended Solids (TSS) is analysed in detail for two days in June 2011 (8 images per day). Both instantaneous and daily composite maps are considered and a comparison is made with corresponding reflectance and TSS products from MODIS-AQUA. Results show TSS distributions corresponding to previous studies of the region. The advantage of the higher acquisition frequency (8 images/day instead of 1) offered by GOCI is clearly demonstrated in the daily composite which is more complete during this period of scattered but moving clouds. Consideration of temporal variation over the day indicates low natural variability but some artificial variability from processing errors ?? this analysis provides a first indication of how the higher frequency of data from geostationary ocean colour could lead to improved data quality control via temporal coherency outlier detection. While there is room for improvement on the GOCI calibration, atmospheric correction and retrieval algorithms, the current study suggests that the GOCI data can already be used now to study qualitatively sediment dynamics except in the extremely turbid waters which are masked out of the current dataset. In a wider context, it is considered that the technical challenges of geostationary ocean colour have been met by the GOCI concept, and, notwithstanding potential improvements on the concept and data processing methods, it is recommended that this mission serve as a model for future geostationary ocean colour sensors over Europe/Africa and the Americas. 相似文献