Weathering process at the natural fission reactor of Bangombé

 The uranium deposits in the basin of Franceville (Gabon) host the only natural fission reactors known in the world. Unique geological conditions favoured a natural fission reaction 2 Ga ago. This was detected by anomalous isotopic compositions of uranium and rare earth elements (REE), which are produced by the fission reaction. In total, 16 reactor zones were found. Most of them are mined out. The reactor zone of Bangombé, is only 10–11 m below the surface. This site has been influenced by surface weathering processes. Six drill cores have been sampled at the site of the reactor zone of Bangombé during the course of the study and only one drill core (BAX 08) hit the core of the reactor. From these data and previous drilling campaigns, the reactor size is estimated to be 10 cm thick, 2–3 m wide and 4–6 m long. The migration of fission products can be traced by the anomalous isotope ratios of REE because of the fission process. The ¹⁴⁹Sm/¹⁴⁷Sm ratio close to the reactor zone is only 0.28 (normal: 0.92) because of the intense neutron capture of ¹⁴⁹Sm and subsequent transmutation, whereas ¹⁴⁷Sm is enriched by the fission reaction. Similar changes in isotopic patterns are detectable on other REE. The isotope ratios of Sm and Nd of whole rock and fracture samples surrounding the reactor indicate that fission-genic REE migrated only a few decimetres above and mainly below the reactor zone. Organic matter (bitumen) seems to act as a trap for fission-genic REE. Additional REE-patterns show less intense weathering with increasing depth in the log profile and support a simple weathering model. Received: 26 November 1999 · Accepted: 2 May 2000     

Microboudin structures of piemontite along the Sambagawa metamorphic belt, Japan: implications for lateral variation of differential stress during regional metamorphism

Evidence is presented of a lateral variation in differential stress during metamorphism along a regional metamorphic belt on the basis of the proportion of microboudinaged piemontite grains (p) in a quartz matrix in metacherts. It is proposed that p is a practical indicator of relative differential stress. Analysis of 123 metacherts from the 800 km long Sambagawa metamorphic belt, Japan, reveals that p‐values range from < 0.01 to 0.7 in this region. Most samples from Wakayama in the mid‐belt area have p‐values of 0.4–0.6, whereas those from western Shikoku have p‐values of < 0.1. This difference cannot be explained by variations in metamorphic temperature, and is instead attributed to a regional, lateral variation in differential stress during metamorphism.     

Hot stars in old stellar populations: a continuing need for intermediate ages

We present numerical investigations into the formation of massive stars from turbulent cores of density structure  ρ∝ r ^−1.5  . The results of five hydrodynamical simulations are described, following the collapse of the core, fragmentation and the formation of small clusters of protostars. We generate two different initial turbulent velocity fields corresponding to power-law spectra   P ∝ k ⁻⁴  and   P ∝ k ^−3.5  , and we apply two different initial core radii. Calculations are included for both completely isothermal collapse, and a non-isothermal equation of state above a critical density  (10⁻¹⁴ g cm⁻³)  . Our calculations reveal the preference of fragmentation over monolithic star formation in turbulent cores. Fragmentation was prevalent in all the isothermal cases. Although disc fragmentation was largely suppressed in the non-isothermal runs due to the small dynamic range between the initial density and the critical density, our results show that some fragmentation still persisted. This is inconsistent with previous suggestions that turbulent cores result in the formation of a single massive star. We conclude that turbulence cannot be measured as an isotropic pressure term.     

Effects of clumping on temperature – I. Externally heated clouds

We present a study of radiative transfer in dusty, clumpy star-forming regions. A series of self-consistent, 3D, continuum radiative transfer models are constructed for a grid of models parametrized by central luminosity, filling factor, clump radius and face-averaged optical depth. The temperature distribution within the clouds is studied as a function of this parametrization. Among our results, we find that: (i) the effective optical depth in clumpy regions is less than in equivalent homogeneous regions of the same average optical depth, leading to a deeper penetration of heating radiation in clumpy clouds, and temperatures higher by over 60 per cent; (ii) penetration of radiation is driven by the fraction of open sky (FOS) – which is a measure of the fraction of solid angle along which no clumps exist; (iii) FOS increases as clump radius increases and as filling factor decreases; (iv) for values of   FOS >0.6–0.8  the sky is sufficiently 'open' that the temperature distribution is relatively insensitive to FOS; (v) the physical process by which radiation penetrates is preferentially through streaming of radiation between clumps as opposed to diffusion through clumps; (vi) filling factor always dominates the determination of the temperature distribution for large optical depths, and for small clump radii at smaller optical depths; (vii) at lower face-averaged optical depths, the temperature distribution is most sensitive to filling factors of 1–10 per cent, in accordance with many observations; (viii) direct shadowing by clumps can be important for distances approximately one clump radius behind a clump.     

Inverted echo sounder measurement of dynamic height through an ENSOcycle in the central equatorial Pacific

A four-year record from an inverted echo sounder deployed near Palmyra Island at 6°N in the central Pacific Ocean is compared with a simultaneous record of subsurface pressure from this island lagoon. A factor m, converting round-trip acoustic travel time to surface dynamic height relative to a deep pressure level, was estimated from the ratio of the spectra of the two records in the energetic synoptic oscillation band. Year-to-year variation in m was not statistically significant. For the overall record, m was found to be -70±8 dynamic m/s, where the error bounds represent a 90% confidence interval. This is consistent with first-baroclinic-mode excitation     

Circumstellar Silicate Mineralogy

This paper reviews spectra obtained with the SWS on board of ISO of dust shells around O-rich objects. These spectra reveal the presence of many new emission features between 10 and 45 μm. These bands are generally much narrower than the well-known 10 and 20 μm silicates features. The strength of these features relative to the underlying broad continuum varies from source to source (≅ 5-50%). The 10 μm region shows evidence for the presence of Al2O3 grains. At longer wavelength, the spectra are dominated by features due to crystalline olivine and pyroxene. The exact peak position of these features shows that the emitting grains consist of the Mg-rich end-members of these minerals with an Fe-content of < 10%. The underlying continuum is attributed to amorphous silicate grains. These observations of aluminum-rich and magnesium-rich compounds compare well with the thermodynamic condensation sequence of minerals expected for O-rich outflows. The observations also imply that freeze out (ie., kinetics) of this condensation sequence at different temperatures is an important characteristic of dust formation in these objects. It is suggested that the absence of Fe-rich silicates is a natural consequence of the low temperature at which gaseous Fe reacts with Mg-rich silicates in these outflows, resulting in amorphous grains with little characterizing spectral detail. This revised version was published online in August 2006 with corrections to the Cover Date.     

Exposure history of the Torino meteorite

Abstract— We determined He, Ne, Ar, ¹⁰Be, ²⁶Al, ³⁶Cl, and ¹⁴C concentrations, as well as cosmic-ray track densities and halogen concentrations in different specimens of the H6 chondrite Torino, in order to constrain its exposure history to cosmic radiation. The Torino meteoroid had a radius of ～20 cm and travelled in interplanetary space for 2.5–10 Ma. Earlier, Torino was part of a larger body. The smallest possible precursor had a radius of 55 cm and a journey through space longer than ～65 Ma. If the first-stage exposure took place in a body with a radius of >3 m or in the parent asteroid, then it lasted nearly 300 Ma. The example of Torino shows that it is easy to underestimate first-stage exposure ages when constructing two-stage histories.     

Evolution of 2:1 layered silicates in low-grade metamorphosed Liassic shales of Central Switzerland

White mica from the Liassic black shales and slates in Central Switzerland was analysed by transmission electron microscopy (TEM) and electron microprobe to determine its textural and compositional evolution during very low-grade prograde metamorphism. Samples were studied from the diagenetic zone, anchizone and epizone (T ≈100°–450 °C). Phyllosilicate minerals analysed include illite/smectite (I/S), phengite, muscovite, brammallite, paragonite, margarite and glauconite. Textural evolution primarily is towards larger, more defect-free grains with compositions that approach those of their respective end-members. The smectite-to-illite transformation reduced the amounts of the exchange components SiK_?1Al_?1, MgSiAl_?2, and Fe³⁺Al_?1. These trends continue to a lesser degree in the anchizone and epizone. Correlations between the proportion of smectite in I/S and the composition of I/S indicate that smectite layers may contain a high layer charge. Illite in I/S bears a compositional resemblance to macrocrystalline phengite in some samples, but is different in others. Paragonite first appears in the upper diagenetic zone or lower anchizone as an interlayer-deficient brammallite, and it may be mixed with muscovite on the nanometre scale. Owing to the small calculated structure factor for paragonite-muscovite superstructures, conventional X-ray powder diffraction cannot distinguish between mixed-layer structures and a homogeneous compositionally intermediate solid solutions. However, indirect TEM evidence shows that irregularly shaped domains of Na- and K-rich mica exist below 10 nm. Subsequent coarsening of domains at higher grades produced discrete paragonite grains at the margins of muscovite crystals or in laths parallel to the basal plane of the host muscovite. Margarite appears in the epizone and follows a textural evolution similar to paragonite in that mixtures of margarite, paragonite, and muscovite may initially occur on the nanometre scale. However, no evidence of interlayer-poor margarite has been found.