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441.
Jos C. Aponte Hannah L. McLain Danielle N. Simkus Jamie E. Elsila Daniel P. Glavin Eric T. Parker Jason P. Dworkin Dolores H. Hill Harold C. Connolly Dante S. Lauretta 《Meteoritics & planetary science》2020,55(7):1509-1524
Evaluating the water‐soluble organic composition of carbonaceous chondrites is key to understanding the inventory of organic matter present at the origins of the solar system and the subsequent processes that took place inside asteroid parent bodies. Here, we present a side‐by‐side analysis and comparison of the abundance and molecular distribution of aliphatic amines, aldehydes, ketones, mono‐ and dicarboxylic acids, and free and acid‐releasable cyanide species in the CM2 chondrites Aguas Zarcas and Murchison. The Aguas Zarcas meteorite is a recent fall that occurred in central Costa Rica and constitutes the largest recovered mass of a CM‐type meteorite after Murchison. The overall content of organic species we investigated was systematically higher in Murchison than in Aguas Zarcas. Similar to previous meteoritic organic studies, carboxylic acids were one to two orders of magnitude more abundant than other soluble organic compound classes investigated in both meteorite samples. We did not identify free cyanide in Aguas Zarcas and Murchison; however, cyanide species analyzed after acid digestion of the water‐extracted meteorite mineral matrix were detected and quantified at slightly higher abundances in Aguas Zarcas compared to Murchison. Although there were differences in the total abundances of specific compound classes, these two carbonaceous chondrites showed similar isomeric distributions of aliphatic amines and carboxylic acids, with common traits such as a complete suite of structural isomers that decreases in concentration with increasing molecular weight. These observations agree with their petrologic CM type‐2 classification, suggesting that these meteorites experienced similar organic formation processes and/or conditions during parent body aqueous alteration. 相似文献
442.
443.
Peter Jenniskens Jason Utas Qing‐Zhu Yin Robert D. Matson Marc Fries J. Andreas Howell Dwayne Free Jim Albers Hadrien Devillepoix Phil Bland Aaron Miller Robert Verish Laurence A. J. Garvie Michael E. Zolensky Karen Ziegler Matthew E. Sanborn Kenneth L. Verosub Douglas J. Rowland Daniel R. Ostrowski Kathryn Bryson Matthias Laubenstein Qin Zhou Qiu‐Li Li Xian‐Hua Li Yu Liu Guo‐Qiang Tang Kees Welten Marc W. Caffee Matthias M. M. Meier Amy A. Plant Colin Maden Henner Busemann Mikael Granvik 《Meteoritics & planetary science》2019,54(4):699-720
It has been proposed that all L chondrites resulted from an ongoing collisional cascade of fragments that originated from the formation of the ~500 Ma old asteroid family Gefion, located near the 5:2 mean‐motion resonance with Jupiter in the middle Main Belt. If so, L chondrite pre‐atmospheric orbits should be distributed as expected for that source region. Here, we present contradictory results from the orbit and collisional history of the October 24, 2015, L6 ordinary chondrite fall at Creston, CA (here reclassified to L5/6). Creston's short 1.30 ± 0.02 AU semimajor axis orbit would imply a long dynamical evolution if it originated from the middle Main Belt. Indeed, Creston has a high cosmic ray exposure age of 40–50 Ma. However, Creston's small meteoroid size and low 4.23 ± 0.07° inclination indicate a short dynamical lifetime against collisions. This suggests, instead, that Creston originated most likely in the inner asteroid belt and was delivered via the ν6 resonance. The U‐Pb systematics of Creston apatite reveals a Pb‐Pb age of 4,497.1 ± 3.7 Ma, and an upper intercept U‐Pb age of 4,496.7 ± 5.8 Ma (2σ), circa 70 Ma after formation of CAI, as found for other L chondrites. The K‐Ar (age ~4.3 Ga) and U,Th‐He (age ~1 Ga) chronometers were not reset at ~500 Ma, while the lower intercept U‐Pb age is poorly defined as 770 ± 320 Ma. So far, the three known L chondrites that impacted on orbits with semimajor axes a <2.0 AU all have high (>3 Ga) K‐Ar ages. This argues for a source of some of our L chondrites in the inner Main Belt. Not all L chondrites originate in a continuous population of Gefion family debris stretching across the 3:1 mean‐motion resonance. 相似文献
444.
445.
Joan A. Browder Victor R. Restrepo Jason K. Rice Michael B. Robblee Zoula Zein-Eldin 《Estuaries and Coasts》1999,22(2):484-499
Two modeling approaches were used to explore the basis for variation in recruitment of pink shrimp,Farfantepenaeus duorarum, to the Tortugas fishing grounds. Emphasis was on development and juvenile densities on the nursery grounds. An exploratory
simulation modeling exercise demonstrated large year-to-year variations in recruitment contributions to the Tortugas pink
shrimp fishery may occur on some nursery grounds, and production may differ considerably among nursery grounds within the
same year, simply on the basis of differences in temperature and salinity. We used a growth and survival model to simulate
cumulative harvests from a July-centered cohort of early-settlementstage postlarvae from two parts of Florida Bay (western
Florida Bay and northcentral Florida Bay), using historic temperature and salinity data from these areas. Very large year-to-year
differences in simulated cumulative harvests were found for recruits from Whipray Basin. Year-to-year differences in simulated
harvests of recruits from Johnson Key Basin were much smaller. In a complementary activity, generalized linear and additive
models and intermittent, historic density records were used to develop an uninterrupted multi-year time series of monthly
density estimates for juvenile pink shrimp in the Johnson Key Basin. The developed data series was based on relationships
of density with environmental variables. The strongest relationship was with sea-surface temperature. Three other environmental
variables (rainfall, water level at Everglades National Park Well P35, and mean wind speed) also contributed significantly
to explaining variation in juvenile densities. Results of the simulation model and two of the three statistical models yielded
similar interannual patterns for Johnson Key Basin. While it is not possible to say that one result validates the other, the
concordance of the annual patterns from the two models is supportive of both approaches. 相似文献
446.
Sean P Healey Jock A Blackard Todd A Morgan Dan Loeffler Greg Jones Jon Songster Jason P Brandt Gretchen G Moisen Larry T DeBlander 《Carbon balance and management》2009,4(1):1-11
The issues surrounding 'Reduced Emissions from Deforestation and Forest Degradation' (REDD) have become a major component of continuing negotiations under the United Nations Framework Convention on Climate Change (UNFCCC). This paper aims to address two key requirements of any potential REDD mechanism: first, the generation of measurable, reportable and verifiable (MRV) REDD credits; and secondly, the sustainable and efficient provision of emission reductions under a robust financing regime. To ensure the supply of MRV credits, we advocate the establishment of an 'International Emission Reference Scenario Coordination Centre' (IERSCC). The IERSCC would act as a global clearing house for harmonized data to be used in implementing reference level methodologies. It would be tasked with the collection, reporting and subsequent processing of earth observation, deforestation- and degradation driver information in a globally consistent manner. The IERSCC would also assist, coordinate and supervise the computation of national reference scenarios according to rules negotiated under the UNFCCC. To overcome the threats of "market flooding" on the one hand and insufficient economic incentives for REDD on the other hand, we suggest an 'International Investment Reserve' (IIR) as REDD financing framework. In order to distribute the resources of the IIR we propose adopting an auctioning mechanism. Auctioning not only reveals the true emission reduction costs, but might also allow for incentivizing the protection of biodiversity and socio-economic values. The introduced concepts will be vital to ensure robustness, environmental integrity and economic efficiency of the future REDD mechanism. 相似文献
447.
Jason M.E. Ahad Johannes A.C. Barth Raja S. Ganeshram Robert G.M. Spencer Günther Uher 《Estuarine, Coastal and Shelf Science》2008,78(4):685-693
In order to evaluate the respiration–photosynthesis dynamics in two contrasting North Sea estuaries, pH, temperature, alkalinity, chlorophyll-a (chl-a), and isotopic ratios of dissolved inorganic carbon (δ13CDIC) and dissolved oxygen (δ18ODO) were measured in the Tyne (July 2003) and Tweed (July 2003 and December 2003) estuaries. Using a concentration-dependent isotope mixing line, δ13CDIC values in the Tweed (July 2003) demonstrated mostly conservative behaviour across the estuary, reflecting mixing between riverine and marine sources, although some samples were slightly more 13C-enriched than predicted δ13CDIC values. Low pCO2 (less than 2 times atmospheric pressure) and 18O-depleted δ18ODO signatures below equilibrium with the atmosphere provided further evidence for net autotrophy in the Tweed estuary in summer 2003. Conversely, in the Tyne during the summer and in the Tweed during the winter higher pCO2 (up to 6.5 and 14.4 times atmospheric partial pressure in the Tweed and Tyne, respectively), slightly 13C-depleted δ13CDIC and 18O-enriched δ18ODO values indicated heterotrophy as the dominant process. The relatively large releases of CO2 observed during these two estuarine surveys can be attributed to significant oxidation of terrigenous organic matter (OM). This study therefore demonstrates the usefulness of combined δ18ODO and δ13CDIC isotopes in examining the relationship between respiration–photosynthesis dynamics and the fate of terrestrially derived OM during estuarine mixing. 相似文献
448.
Sources and fate of nutrients in a subtropical reservoir 总被引:1,自引:0,他引:1
Michele?A.?BurfordEmail author Susanne?A.?Green Andrew?J.?Cook Suzanne?A.?Johnson Jason?G.?Kerr Katherine?R.?O’Brien 《Aquatic Sciences - Research Across Boundaries》2012,74(1):179-190
This study examined the sources and fate of nutrient inputs from two principal tributaries to the eutrophic subtropical Wivenhoe
reservoir: an unregulated river and a dammed river with regular releases, during a period of declining reservoir water levels.
Nutrient budgets were constructed over a period of 6 years, and combined with short-term data on nutrient concentrations and
forms, and δ15N stable isotope data. Our study found that over a 6 year period, there was net retention of phosphorus (P) in the reservoir,
with 60% of inputs retained. Most of the P input load came from the unregulated river, with an agricultural catchment, during
periods of high flow. During one event half of the total TP load from the unregulated river in the study period was delivered
in only 12 days. Much of the P was dissolved inorganic P (DIP) and was derived from high P concentrations in soils and sediments.
This highlights the importance of appropriate catchment management practices to reduce P losses from terrestrial systems because
retention of P in reservoir sediments reduces the availability of this nutrient for agricultural production. In contrast,
there was negligible retention of nitrogen (N). The unregulated river was an important source of N derived from N fixation
in the river and adjacent soils, while the source from the dammed river was mostly reprocessed N. The high retention of P
relative to N is consistent with relatively higher accumulation of P in sediments. 相似文献
449.
Simulation of Meteorological Fields Within and Above Urban and Rural Canopies with a Mesoscale Model 总被引:3,自引:4,他引:3
Accurate simulation of air quality at neighbourhood scales (on order of 1-km horizontal grid spacing) requires detailed meteorological fields inside the roughness sub-layer (RSL). Since the assumptions of the roughness approach, used by most of the mesoscale models, are unsatisfactory at this scale, a detailed urban and rural canopy parameterisation, called DA-SM2-U, is developed inside the Penn State/NCAR Mesoscale Model (MM5) to simulate the meteorological fields within and above the urban and rural canopies. DA-SM2-U uses the drag-force approach to represent the dynamic and turbulent effects of the buildings and vegetation, and a modified version of the soil model SM2-U, called SM2-U(3D), to represent the thermodynamic effects of the canopy elements. The turbulence length scale is also modified inside the canopies. SM2-U(3D) assesses the sensible and latent heat fluxes from rural and urban surfaces in each of the computational layers inside the canopies by considering the shadowing effect, the radiative trapping by the street canyons, and the storage heat flux by the artificial surfaces. DA-SM2-U is tested during one simulated day above the city of Philadelphia, U.S.A. It is shown that DA-SM2-U is capable of simulating the important features observed in the urban and rural RSL, as seen in the vertical profiles of the shear stress, turbulent kinetic energy budget components, eddy diffusivity, potential air temperature, and specific humidity. Within the canopies, DA-SM2-U simulates the decrease of the wind speed inside the dense canopies, the skirting of the flow around the canopy blocks, warmer air inside the vegetation canopy than above open areas during the night and conversely during the day, and constantly warmer air inside the urban canopy. The comparison with measurements shows that the surface air temperature above rural and urban areas is better simulated by DA-SM2-U than by the `standard version' of MM5. 相似文献
450.
Acacia S. Pepler Lisa V. Alexander Jason P. Evans Steven C. Sherwood 《Climate Dynamics》2016,46(1-2):123-133
Southeast Australia is a region of high rainfall variability related to major climate drivers, with a long-term declining trend in cool-season rainfall. Projections of future rainfall trends are uncertain in this region, despite projected southward shifts in the subtropical ridge and mid-latitude westerlies. This appears to be related to a poor representation of the spatial relationships between rainfall variability and zonal wind patterns across southeast Australia in the latest Coupled Model Intercomparison Project ensemble, particularly in the areas where weather systems embedded in the mid-latitude westerlies are the main source of cool-season rainfall. Downscaling with regional climate models offers improvements in the mean rainfall climatology, and shows some ability to correct for poor modelled relationships between rainfall and zonal winds along the east coast of Australia. However, it provides only minor improvements to these relationships in southeast Australia, despite the improved representation of topographic features. These results suggest that both global and regional climate models may fail to translate projected circulation changes into their likely rainfall impacts in southeast Australia. 相似文献