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71.
F.A. Franklin 《Icarus》1979,40(3):329-334
A principal feature of the asteroidal distribution is the rapid truncation of its population outward from ~3.4 AU. This paper presents further evidence, based on the motion and distribution of certain minor planets with large semimajor axes, that this truncation cannot be strictly the result of gravitational perturbations of the major planets even acting over times of ~109 years. The motion of other outer asteroids sets a probable upper limit of 0.081 on Jupiter's eccentricity. 相似文献
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The interaction of Mn2+ with the surface of calcite in aqueous solutions is complex. In dilute solutions the Mn2+ is rapidly absorbed, MnCO33 nucleates on the calcite surface and then grows by a first order reaction with respect to the initial Mn2+ concentration. At higher ionic strengths in NaCl solutions, the rate of these processes is slower, but the same general pattern persists. In solutions containing Mg2+, at the concentration of seawater and in seawater, the nucleation phase of the uptake process does not appear to occur. The long-term uptake rate of Mn2+ on the surface of calcite in seawater is first order with respect to the dissolved Mn2+ concentration. The rate constant is over three orders of magnitude smaller than that found in dilute Mg2+-free solutions. A probable explanation for the slower growth rate in seawater is that MnCO3 is not nucleated on the calcite surface due to the presence of high Mg2+ concentrations. The Mg2+, through site competition, prevents enough Mn2+ from being adsorbed to reach a critical concentration for MnCO3 nucleation. This behavior is similar to that found for orthophosphate with calcite surfaces in dilute solutions and seawater. It indicates that rhodochrosite cannot nucleate in carbonate-rich recent sediments unless the Mg2+ concentration is lowered below that of seawater.Measurements of the solubility of rhodochrosite in seawater gave results from an undersaturation approach to equilibrium in excellent agreement with those found in previous studies in dilute solutions. When equilibrium was approached from supersaturation, approximately fifty times more calcium was precipitated than Mn2+. The measured solubility was over twice that determined from undersaturation. It is possible that a Mn—calcite containing 25 to 30 mol% MnCO3 formed on the rhodochrosite from the supersaturated solutions. Consequently, it is doubtful that pure rhodochrosite controls the concentration of Mn2+ even in calcium carbonate-poor marine environments. 相似文献
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Alves SR Severino PC Ibbotson DP da Silva AZ Lopes FR Sáenz LA Bainy AC 《Marine environmental research》2002,54(3-5):241-245
Furadan is a carbamate pesticide used widely to combat agricultural pests. However little information is available about the toxicity of furadan in aquatic macroinvertebrates. The in vivo effects of furadan were evaluated in mussels, Perna perna, and oysters, Crassostrea rhizophorae. Glutathione S-transferase (GST), catalase (CAT) and cholinesterase (ChE) activities were measured in the gills of both species exposed to furadan (100 microg/l) for 96 h. No changes were observed in GST activity in the exposed groups. CAT activity was higher (9%) in the oysters exposed to furadan. ChE activity was inhibited by 64 and 35%, respectively, in C. rhizophorae and P. perna exposed to furadan, suggesting that the former is more susceptible to the toxic effects of furadan. 相似文献
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Keewook Kim Gene Whelan S. Thomas Purucker Thomas F. Bohrmann Michael J. Cyterski Marirosa Molina Yin Gu Yakov Pachepsky Andrey Guber Dorcas H. Franklin 《水文研究》2014,28(20):5220-5235
Four seasonal rainfall simulations in 2009 and 2010 were applied to a field containing 36 plots (0.75 × 2 m each), resulting in 144 runoff events. In all simulations, a constant rate of rainfall was applied then halted 60 min after initiation of runoff, with plot‐scale monitoring of runoff every 5 min during that period. Runoff was simulated with the Kinematic Runoff and Erosion/Simulator of Transport with Infiltration and Runoff (KINEROS2/STWIR) field‐scale model, whose hydrodynamics are based on the kinematic wave equation. Because of the non‐linear nature of the model and a highly parameterized model with respect to the available data, several approaches were investigated to upscale nine runoff‐related parameters from a series of small monitored plots to the field scale. Inverse modeling was performed using the model‐independent Parameter ESTimation (PEST) algorithm to individually calibrate the nine KINEROS2/STWIR parameters on 36 plots. The parameters were averaged, and bootstrapping was used to assess uncertainty of the parameters via estimation of confidence intervals (CI). A Monte Carlo simulation using the bootstrap results showed reasonable field‐scale representation of flow rates. Median values of calibrated parameters were within the 95% CI obtained with bootstrapping. The simulated results for the median values associated with the 90% CI flow rates produced similar trends as those exhibited with the observed data, suggesting that median values of the calibrated parameters from the PEST inverse modeling could be used to represent the field scale. Copyright © 2013 John Wiley & Sons, Ltd. 相似文献
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Aidan Foley Gerd Cachandt Janine Franklin Fergus Willmore Tim Atkinson 《Hydrogeology Journal》2012,20(3):483-498
The Corallian limestone of northern England (UK) is widely exploited for water supplies and exhibits the karstic phenomena of sinking rivers, conduit development and groundwater velocities of several kilometres per day. To test a number of model-derived source protection zones and elucidate contaminant transport mechanisms in the aquifer, three tracer tests were conducted from a set of swallow-holes draining the River Derwent toward public water supply wells in the eastern part of the aquifer. Tracers used included: Enterobacter cloacae (bacteriophage), Photine C (optical brightener), sodium fluorescein (fluorescent dye) and sulphur hexafluoride (dissolved gas), the varying properties of which make them suitable analogues for different types of potential contaminant. Observed tracer transport times and arrival patterns indicate that tracer transport occurs through karstic channels embedded in a network of primary fissures which exert control over tracer concentrations once initial tracer plumes have passed. A dipole flow system is observed between the swallow-holes and the closest abstraction well, whilst previously modelled source protection zones do not accurately reflect either groundwater velocity or those areas of the aquifer supplying the wells. These findings imply that managing such aquifers for potential contamination should rely upon empirical tracer evidence for source-protection zone modelling. 相似文献
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