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1.
Alan M Bond Julie R Bradbury Henry A Hudson John S Garnham Peter J Hanna Stanley Strother 《Marine Chemistry》1985,16(1):1-9
Evidence was found that uptake of lead from seawater in both model and natural systems by the leaves of the seagrass Zostera muelleri does occur for live, dead and scraped leaves at all the lead concentrations tested. Positive uptake of lead was measured using the three analytical techniques of radio-tracer, differential pulse anodic stripping voltammetry and atomic absorption spectrometry; similar uptake profiles were obtained for each technique. Profiles always showed an initial rapid uptake phase followed by a gradual transition to a plateau phase at which an approximate equilibrium between lead attached to seagrass and free ionic lead in seawater was reached. The presence of active lead uptake processes was indicated in experiments which attempted to remove lead from leaves by a chelating agent. 相似文献
2.
Walter Dean Roger Anderson J. Platt Bradbury David Anderson 《Journal of Paleolimnology》2002,27(3):287-299
The deepest part (29.5 m) of Elk Lake, ClearwaterCounty, northwestern Minnesota, contains a complete Holocene section that iscontinuously varved. The varve components are predominantly autochthonous(CaCO3, organic matter, biogenic silica, and several iron andmanganese minerals), but the varves do contain a minor detrital-clastic(aluminosilicate) component that is predominantly wind-borne (eolian) andprovides an important record of atmospheric conditions. Singular spectrumanalysis (SSA) and wavelet analysis of varve thickness recognized significantperiodicities in the multicentennial and multidecadal bands that varied inpower (i.e., variable significance) and position (i.e., variable period) withinthe periodic bands. Persistent periodicities of about 10, 22, 40, and 90 years,and, in particular, multicentennial periodicities in varve thickness and otherproxy variables are similar to those in spectra of radiocarbon production, aproxy for past solar activity. This suggests that there may be a solar control,perhaps through geomagnetic effects on atmospheric circulation. Multicentennialand multidecadal periodicities also occur in wavelet spectra of relativegray-scale density. However, gray-scale density does not appear to correlatewith any of the measured proxy variables, and at this point we do not know whatcontrolled gray scale. 相似文献
3.
Richard L. Reynolds Joseph G. Rosenbaum Josh Rapp Michael W. Kerwin J. Platt Bradbury Steven Colman David Adam 《Journal of Paleolimnology》2004,31(2):217-233
Petrological and textural properties of lacustrine sediments from Upper Klamath Lake, Oregon, reflect changing input volumes of glacial flour and thus reveal a detailed glacial history for the southern Cascade Range between about 37 and 15 ka. Magnetic properties vary as a result of mixing different amounts of the highly magnetic, glacially generated detritus with less magnetic, more weathered detritus derived from unglaciated parts of the large catchment. Evidence that the magnetic properties record glacial flour input is based mainly on the strong correlation between bulk sediment particle size and parameters that measure the magnetite content and magnetic mineral freshness. High magnetization corresponds to relatively fine particle size and lower magnetization to coarser particle size. This relation is not found in the Buck Lake core in a nearby, unglaciated catchment. Angular silt-sized volcanic rock fragments containing unaltered magnetite dominate the magnetic fraction in the late Pleistocene sediments but are absent in younger, low magnetization sediments. The finer grained, highly magnetic sediments contain high proportions of planktic diatoms indicative of cold, oligotrophic limnic conditions. Sediment with lower magnetite content contains populations of diatoms indicative of warmer, eutrophic limnic conditions. During the latter part of oxygen isotope stage 3 (about 37–25 ka), the magnetic properties record millennial-scale variations in glacial-flour content. The input of glacial flour was uniformly high during the Last Glacial Maximum, between about 21 and 16 ka. At about 16 ka, magnetite input, both absolute and relative to hematite, decreased abruptly, reflecting a rapid decline in glacially derived detritus. The decrease in magnetite transport into the lake preceded declines in pollen from both grass and sagebrush. A more gradual decrease in heavy mineral content over this interval records sediment starvation with the growth of marshes at the margins of the lake and dilution of detrital material by biogenic silica and other organic matter. 相似文献
4.
Sorption edges and isotherms for Eu(III) uptake on Ca-montmorillonite and Na-illite in 0.066 mol/L Ca(ClO4)2 and 0.1 mol/L NaClO4 background electrolytes, respectively, were modelled using a quasi-mechanistic sorption model (the two site protolysis non electrostatic surface complexation and cation exchange (2SPNE SC/CE) model). For both clay minerals the Eu sorption edges could be quantitatively modelled in the pH range ∼3 to ∼10 using cation exchange reactions for Eu3+/Na+ and Eu3+/Ca2+ and three surface complexation reactions on the strong sorption sites forming ≡SSOEu2+, ≡SSOEuOH+ and ≡SSOEu(OH)2° inner sphere complexes which appear successively with increasing pH. Time resolved laser fluorescence spectroscopy (TRLFS) measurements of Cm(III) loaded Ca-montmorillonite and Na-illite were available from Part 1 of this work. De-convolution of the normalised fluorescence spectra measured at different pH values indicated three distinct Cm surface complexes, Cm complexes 1, 2 and 3 for both clay minerals, in agreement with model predictions, but with different distribution functions for the individual species. Under the assumption that Eu and Cm exhibit essentially the same hydrolysis and sorption behaviour, the Eu surface complexation constants were used to predict surface species distribution functions for Cm under the same experimental conditions used in the TRLFS measurements. Comparison of modelled and experimentally deduced species distributions indicated that for both clay minerals peak heights and widths of the three peaks did not correspond particularly well. It is shown that the calculated species distribution functions are sensitive to the values of the hydrolysis constants used in the calculations, whereas modelling the sorption edge measurements by applying the 2SPNE SC/CE approach is much less sensitive. By modifying the values of the hydrolysis constants within their uncertainty range and re-modelling the sorption edges, considerably better correspondence between the modelled and TRLFS species distribution functions was found. In particular, peak positions, heights and widths for the model predicted peaks for the ≡SSOCm2+ and ≡SSOCmOH+ species distribution, and those for Cm complexes 1 and 2 derived from TRLFS, were found to be very close for both clay minerals. However, discrepancies were still apparent between the profile for the calculated ≡SSOEu(OH)2° surface species and the Cm complex 3 species, especially in the case of Na-illite. 相似文献
5.
6.
This study integrated surface and subsurface stratigraphic data with geophysical logs and hydrogeologic data in order to
characterize the hydraulic properties of the Silurian dolomite in northeastern Wisconsin. Silurian stratigraphy consists of
predictable alternations of characteristic facies associations. A vertical profile of hydraulic conductivity, obtained from
short-interval packer tests in a core hole that penetrates a majority of the Silurian section, indicates that hydraulic conductivity
ranges over five orders of magnitude (10–1 to 10–6 cm/s). Matrix conductivity is generally low and varies with texture; the finer-grained restricted-marine and transitional
facies being less permeable than the coarser-grained open-marine facies. High-conductivity values are generally associated
with bedding-plane fractures, and fracture frequency is greater in the restricted-marine facies.
High-flow features in 16 wells were identified using fluid-temperature/resistivity and heat-pulse flowmeter logs. Natural-gamma
logs were used to identify the stratigraphic position of flow features in each well and to correlate flow features to specific
stratigraphic horizons. By combining stratigraphic, geophysical, and hydrogeologic data, 14 high-permeability zones within
the Silurian aquifer have been identified and correlated in wells more than 16 km apart. These zones parallel bedding, appear
most pronounced at contacts between contrasting lithologies, and are most abundant in restricted-marine lithologies.
Electronic Publication 相似文献
7.
There are few studies on the hydrogeology of sedimentary rock aquitards although they are important controls in regional ground water flow systems. We formulate and test a three-dimensional (3D) conceptual model of ground water flow and hydrochemistry in a fractured sedimentary rock aquitard to show that flow dynamics within the aquitard are more complex than previously believed. Similar conceptual models, based on regional observations and recently emerging principles of mechanical stratigraphy in heterogeneous sedimentary rocks, have previously been applied only to aquifers, but we show that they are potentially applicable to aquitards. The major elements of this conceptual model, which is based on detailed information from two sites in the Maquoketa Formation in southeastern Wisconsin, include orders of magnitude contrast between hydraulic diffusivity (K/S(s)) of fractured zones and relatively intact aquitard rock matrix, laterally extensive bedding-plane fracture zones extending over distances of over 10 km, very low vertical hydraulic conductivity of thick shale-rich intervals of the aquitard, and a vertical hydraulic head profile controlled by a lateral boundary at the aquitard subcrop, where numerous surface water bodies dominate the shallow aquifer system. Results from a 3D numerical flow model based on this conceptual model are consistent with field observations, which did not fit the typical conceptual model of strictly vertical flow through an aquitard. The 3D flow through an aquitard has implications for predicting ground water flow and for planning and protecting water supplies. 相似文献
8.
A. Smith R. W. Atkins S. Bradbury O. Celik Y. C. K. Chow P. Cogan C. Dowdall S. J. Fegan P. Fortin D. Gall G. H. Gillanders J. Grube K. J. Gutierrez T. A. Hall D. Hanna J. Holder D. Horan S. B. Hughes T. B. Humensky I. Jung P. Kaaret G. Kenny M. Kertzman D. B. Kieda A. Konopelko H. Krawczynski F. Krennrich M. J. Lang S. Le Bohec G. Maier J. Millis P. Moriarty R. A. Ong J. S. Perkins K. Ragan G. H. Sembroski J. A. Toner L. Valcarcel V. V. Vassiliev R. G. Wagner S. P. Wakely T. C. Weekes R. J. White D. A. Williams 《Astrophysics and Space Science》2007,309(1-4):299-303
In this paper we present the results of the past two years observations on the galactic microquasar LS I +61 303 with the
Whipple 10 m gamma-ray telescope. The recent MAGIC detection of the source between 200 GeV and 4 TeV suggests that the source
is periodic with very high energy (VHE) gamma-ray emission linked to its orbital cycle. The entire 50-hour data set obtained
with Whipple from 2004 to 2006 was analyzed with no reliable detection resulting. The upper limits obtained in the 2005–2006
season covered several of the same epochs as the MAGIC Telescope detections, albeit with lower sensitivity. Upper limits are
placed on emission during the orbital phases of 0→0.1 and 0.8→1, phases which are not included in the MAGIC data set.
相似文献
9.
A climatic-limnologic model of diatom succession for paleolimnological interpretation of varved sediments at Elk Lake,Minnesota 总被引:1,自引:0,他引:1
J. Platt Bradbury 《Journal of Paleolimnology》1988,1(2):115-131
Sediment traps placed in the profundal region of Elk Lake, north central Minnesota during the 1979 spring and 1983–84 fall and spring seasons monitored seasonal diatom production for two climatically distinctive periods. The spring of 1979 was one of the coldest and wettest on record. Ice out at Elk Lake was 10 days later than average, and spring circulation was short. Fragilaria crotonensis dominated the late spring and early summer diatom production in association with Synedra and Cyclotella species, perhaps because rates of phosphorus supply were low compared to silica. The winter of 1983–84 was drier than usual, and the early but cold spring of 1984 caused ice out at Elk Lake to be about 1 week earlier than normal. Spring storms promoted a long and full circulation that allowed Stephanodiscus minulutus to bloom, presumably in response to increased phosphorus loading related to deep and vigorous circulation. The two dominant diatoms in Elk Lake, F. crotonensis and S. minutulus may reflect climatic patterns that control lake circulation. The climatically regulated occurrence of these diatoms is generally, but not specifically, comparable to their distribution in lake surface sediments throughout Minnesota. A combination of regional and lake-specific studies on the controls of diatom succession and distribution provides climatic insights for interpreting paleolimnogical records of diatoms. 相似文献
10.
The spatial and temporal variability of groundwater recharge in a forested basin in northern Wisconsin 总被引:1,自引:0,他引:1
Recharge varies spatially and temporally as it depends on a wide variety of factors (e.g. vegetation, precipitation, climate, topography, geology, and soil type), making it one of the most difficult, complex, and uncertain hydrologic parameters to quantify. Despite its inherent variability, groundwater modellers, planners, and policy makers often ignore recharge variability and assume a single average recharge value for an entire watershed. Relatively few attempts have been made to quantify or incorporate spatial and temporal recharge variability into water resource planning or groundwater modelling efforts. In this study, a simple, daily soil–water balance model was developed and used to estimate the spatial and temporal distribution of groundwater recharge of the Trout Lake basin of northern Wisconsin for 1996–2000 as a means to quantify recharge variability. For the 5 years of study, annual recharge varied spatially by as much as 18 cm across the basin; vegetation was the predominant control on this variability. Recharge also varied temporally with a threefold annual difference over the 5‐year period. Intra‐annually, recharge was limited to a few isolated events each year and exhibited a distinct seasonal pattern. The results suggest that ignoring recharge variability may not only be inappropriate, but also, depending on the application, may invalidate model results and predictions for regional and local water budget calculations, water resource management, nutrient cycling, and contaminant transport studies. Recharge is spatially and temporally variable, and should be modelled as such. Copyright © 2009 John Wiley & Sons, Ltd. 相似文献