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41.
The structures of sodium silicate and aluminosilicate glasses quenched from melts at high pressure (6-10 GPa) with varying degrees of polymerization (fractions of nonbridging oxygen) were explored using solid-state NMR [17O and 27Al triple-quantum magic-angle spinning (3QMAS) NMR]. The bond connectivity in melts among four and highly coordinated network polyhedra, such as [4]Al, [5,6]Al, [4]Si, and [5,6]Si, at high pressure is shown to be significantly different from that at ambient pressure. In particular, in the silicate and aluminosilicate melts, the proportion of nonbridging oxygen (NBO) generally decreases with increasing pressure, leading to the formation of new oxygen clusters that include 5- and 6-coordinated Si and Al in addition to 4-coordinated Al and Si, such as [4]Si-O-[5,6]Si, [4]Si-O-[5,6]Al and Na-O-[5,6]Si. While the fractions of [5,6]Al increase with pressure, the magnitude of this increase diminishes with increasing degrees of ambient-pressure polymerization under isobaric conditions. Incorporating the above structural information into models of melt properties reproduces the anomalous pressure-dependence of O2− diffusivity and viscosity often observed in silicate melts. 相似文献
42.
Andesite and dacite genesis via contrasting processes: the geology and geochemistry of El Valle Volcano,Panama 总被引:3,自引:0,他引:3
Mare J. Defant Lee F. Clark Robert H. Stewart Mark S. Drummond Jelle Z. de Boer René C. Maury Hervé Bellon Thomas E. Jackson Juan F. Restrepo 《Contributions to Mineralogy and Petrology》1991,106(3):309-324
The easternmost stratovolcano along the Central American arc is El Valle volcano, Panama. Several andesitic and dacitic lava
flows, which range in age 5–10 Ma, are termed the old group. After a long period of quiescence (approximately 3.4 Ma), volcanic
activity resumed approximately 1.55 Ma with the emplacement of dacitic domes and the deposition of dacitic pyroclastic flows
0.9–0.2 Ma. These are referred to as the young group. All of the samples analyzed are calc-alkaline andesites and dacites.
The mineralogy of the two groups is distinct; two pyroxenes occur in the old-group rocks but are commonly absent in the young
group. In contrast, amphibole has been found only in the young-group samples. Several disequilibrium features have been observed
in the minerals (e.g., oscillatory zoning within clinopyroxenes). These disequilibrium textures appear to be more prevalent
among the old- as compared with the young-group samples and are most likely the result of magma-mixing, assimilation, and/or
polybaric crystallization. Mass-balance fractionation models for major and trace elements were successful in relating samples
from the old group but failed to show a relationship among the young-group rocks or between the old- and young-group volcanics.
We believe that the old-group volcanics were derived through differentiation processes from basaltic magmas generated within
the mantlewedge. The young group, however, does not appear to be related to more primitive magmas by differentiation. The
young-group samples cannot be related by fractionation including realistic amounts of amphibole. Distinctive geochemical features
of the young group, including La/Yb ratios〉15, Yb〈1, Sr/Y〉150, and Y〈6, suggest that these rocks were derived from the partial
melting of the subducted lithosphere. These characteristics can be explained by the partial melting of a source with residual
garnet and amphibole. Dacitic material with the geochemical characteristics of subducted-lithosphere melting is generated
apparently only where relatively hot crust is subducted, based on recent work. The young dacite-genesis at El Valle volcano
is related to the subduction of relatively hot lithosphere. 相似文献
43.
The vegetated urban canopy model (VUCM) is implemented in a meteorological model, the Regional Atmospheric Modeling System (RAMS), for urban atmospheric modeling. The VUCM includes various urban physical processes such as in-canyon radiative transfer, turbulent energy exchanges, substrate heat conduction, and in-canyon momentum drag. The coupled model RAMS/VUCM is evaluated and then used to examine its impacts on the dynamic and thermodynamic structure of the urban boundary layer (UBL) in the Seoul metropolitan area. The spatial pattern of the nocturnal urban heat island (UHI) in Seoul is quite well simulated by the RAMS/VUCM. A statistical evaluation of 2-m air temperature reveals a significant improvement in model performance, especially in the nighttime. The RAMS/VUCM simulates the diurnal variations of surface energy balance fluxes realistically. This contributes to a reasonable UBL formation. A weakly unstable UBL is formed in the nighttime with UBL heights of about 100–200 m. When urban surfaces are represented in the RAMS using a land surface model of the Land Ecosystem-Atmosphere Feedback (LEAF), the RAMS/LEAF produces strong cold biases and thus fails to simulate UHI formation. This is due to the poor representation or absence of important urban physical processes in the RAMS/LEAF. This study implies that urban physical processes should be included in numerical models in order to reasonably simulate meteorology and air quality in urban areas and that the VUCM is one of the promising urban canopy models. 相似文献
44.
Mass and energy fluxes between the atmosphere and vegetation are driven by meteorological variables, and controlled by plant
water status, which may change more markedly diurnally than soil water. We tested the hypothesis that integration of dynamic
changes in leaf water potential may improve the simulation of CO2 and water fluxes over a wheat canopy. Simulation of leaf water potential was integrated into a comprehensive model (the ChinaAgrosys)
of heat, water and CO2 fluxes and crop growth. Photosynthesis from individual leaves was integrated to the canopy by taking into consideration the
attenuation of radiation when penetrating the canopy. Transpiration was calculated with the Shuttleworth-Wallace model in
which canopy resistance was taken as a link between energy balance and physiological regulation. A revised version of the
Ball-Woodrow-Berry stomatal model was applied to produce a new canopy resistance model, which was validated against measured
CO2 and water vapour fluxes over winter wheat fields in Yucheng (36°57′ N, 116°36′ E, 28 m above sea level) in the North China
Plain during 1997, 2001 and 2004. Leaf water potential played an important role in causing stomatal conductance to fall at
midday, which caused diurnal changes in photosynthesis and transpiration. Changes in soil water potential were less important.
Inclusion of the dynamics of leaf water potential can improve the precision of the simulation of CO2 and water vapour fluxes, especially in the afternoon under water stress conditions. 相似文献
45.
Il-Sung Zo Joon-Bum Jee Kyu-Tae Lee Bu-Yo Kim 《Asia-Pacific Journal of Atmospheric Sciences》2016,52(4):405-412
Preliminary analysis with a solar radiation model is generally performed for photovoltaic power generation projects. Therefore, model accuracy is extremely important. The temporal and spatial resolutions used in previous studies of the Korean Peninsula were 1 km × 1 km and 1-h, respectively. However, calculating surface solar radiation at 1-h intervals does not ensure the accuracy of the geographical effects, and this parameter changes owing to atmospheric elements (clouds, aerosol, ozone, etc.). Thus, a change in temporal resolution is required. In this study, one-year (2013) analysis was conducted using Chollian geostationary meteorological satellite data from observations recorded at 15-min intervals. Observation data from the intensive solar site at Gangneung-Wonju National University (GWNU) showed that the coefficient of determination (R²), which was estimated for each month and season, increased, whereas the standard error (SE) decreased when estimated in 15-min intervals over those obtained in 1-h intervals in 2013. When compared with observational data from 22 solar sites of the Korean Meteorological Administration (KMA), R2 was 0.9 or higher on average, and over- or under-simulated sites did not exceed 3 sites. The model and 22 solar sites showed similar values of annual accumulated solar irradiation, and their annual mean was similar at 4,998 MJ m?2 (3.87 kWh m?2). These results show a difference of approximately ± 70 MJ m?2 (± 0.05 kWh m?2) from the distribution of the Korean Peninsula estimated in 1-h intervals and a higher correlation at higher temporal resolution. 相似文献
46.
A monotonic transport algorithm for a high-order time integration scheme is described in this paper. The algorithm is a modified version of an existing high-order time integration scheme, and is tested using a simple one-dimensional pulse and two-dimensional deformational flows. It is found that the new formulation can remove the error, caused by new maxima/minima and excessive smoothing, which occurs in scalar transport using the original extrapolation scheme. The results show that there may be potential for the high-order time integration scheme to be applied in numerical weather prediction models. 相似文献
47.
雷达拼图资料上中尺度对流系统的跟踪与预报 总被引:1,自引:2,他引:1
在中尺度对流系统(Mesoscale Convective Systems,MCSs)自动识别基础上,利用相关法跟踪雷达回波(Tracking Radar Echoes by Cross-correlation,TREC)和面积重叠法完成新的跟踪预报方法.新方法利用TREC得到MCSs移动矢量,利用该矢量外推对应MCSs雷达回波.根据外推回波与相应回波实况,采用面积重叠法完成跟踪,同时利用移动矢量完成预报.采用4次强天气过程对算法进行检验,分析结果表明:(1)新方法能够有效实现MCSs跟踪与预报;(2)新方法得到MCSs移动速度相对稳定,不因为系统合并、分裂和生消出现速度大幅度波动现象,有效减小预报误差,6~60 min预报误差相对于原方法减小20%以上;(3)新方法虽然能提取得到较为稳定的系统移动速度,但不能得到系统的传播速度.原方法能得到系统的移动速度和传播速度合成,但提取速度不稳定,容易受到质心偏移的影响,预报误差较大.新方法在系统消亡期提取移动速度不稳定,导致跟踪丢失现象的发生,而原方法在系统合并与分裂时易出现跟踪丢失现象. 相似文献
48.
Fetch and Footprint of Turbulent Fluxes over Vegetative Stands with Elevated Sources 总被引:1,自引:0,他引:1
Xuhui Lee 《Boundary-Layer Meteorology》2003,107(3):561-579
In this study, Raupach's localized near-field (LNF)theory is combined with appropriate parameterizations ofthe turbulence inside a canopy to investigate how airstability and source configuration influence the fluxfootprint and flux adjustment with fetch in theroughness sublayer. The model equations are solvednumerically. The flux footprint from the LNF predictionis in general more contracted than the prediction basedon the inertial sublayer similarity functions. Invery unstable conditions, the near-field effect causes thefootprint of the elevated canopy source to locatefurther upwind than that of the ground-level source, andthe combined footprint can become negative in situationswhere the two sources are of opposite sign. The fluxfootprint and flux adjustment with fetch in theroughness sublayer are sensitive to source configurationand the parameters specifying wind speed and theLagrangian time scale inside the canopy. 相似文献
49.
The climate–population relationship has long been conceived. Although the topic has been repeatedly investigated, most of
the related works are Eurocentric or qualitative. Consequently, the relationship between climate and population remains ambiguous.
In this study, fine-grained temperature reconstructions and historical population data sets have been employed to statistically
test a hypothesized relationship between temperature change and population growth (i.e., cooling associated with below average
population growth) in China over the past millennium. The important results were: (1) Long-term temperature change significantly
determined the population growth dynamics of China. However, spatial variation existed, whilst population growth in Central
China was shown to be responsive to both long- and short-term temperature changes; in marginal areas, population growth was
only sensitive to short-term temperature fluctuations. (2) Temporally, the temperature–population relationship was obscured
in some periods, which was attributable to the factors of drought and social buffers. In summary, a temperature–population
relationship was mediated by geographic factors, the aridity threshold, and social factors. Given the upcoming threat posed
by climate change to human societies, this study seeks to improve our knowledge and understanding of the climate–society relationship. 相似文献
50.
Seong-Joong Kim Thomas J. Crowley David J. Erickson Bala Govindasamy Phillip B. Duffy Bang Yong Lee 《Climate Dynamics》2008,31(1):1-16
The climate of the last glacial maximum (LGM) is simulated with a high-resolution atmospheric general circulation model, the
NCAR CCM3 at spectral truncation of T170, corresponding to a grid cell size of roughly 75 km. The purpose of the study is
to assess whether there are significant benefits from the higher resolution simulation compared to the lower resolution simulation
associated with the role of topography. The LGM simulations were forced with modified CLIMAP sea ice distribution and sea
surface temperatures (SST) reduced by 1°C, ice sheet topography, reduced CO2, and 21,000 BP orbital parameters. The high-resolution model captures modern climate reasonably well, in particular the distribution
of heavy precipitation in the tropical Pacific. For the ice age case, surface temperature simulated by the high-resolution
model agrees better with those of proxy estimates than does the low-resolution model. Despite the fact that tropical SSTs
were only 2.1°C less than the control run, there are many lowland tropical land areas 4–6°C colder than present. Comparison
of T170 model results with the best constrained proxy temperature estimates (noble gas concentrations in groundwater) now
yield no significant differences between model and observations. There are also significant upland temperature changes in
the best resolved tropical mountain belt (the Andes). We provisionally attribute this result in part as resulting from decreased
lateral mixing between ocean and land in a model with more model grid cells. A longstanding model-data discrepancy therefore
appears to be resolved without invoking any unusual model physics. The response of the Asian summer monsoon can also be more
clearly linked to local geography in the high-resolution model than in the low-resolution model; this distinction should enable
more confident validation of climate proxy data with the high-resolution model. Elsewhere, an inferred salinity increase in
the subtropical North Atlantic may have significant implications for ocean circulation changes during the LGM. A large part
of the Amazon and Congo Basins are simulated to be substantially drier in the ice age—consistent with many (but not all) paleo
data. These results suggest that there are considerable benefits derived from high-resolution model regarding regional climate
responses, and that observationalists can now compare their results with models that resolve geography at a resolution comparable
to that which the proxy data represent. 相似文献