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The complex reactions between high saline solutions and toxic chemical wastes were investigated by means of laboratory experiments and geochemical modelling. The specific boundary conditions of an underground repository in salt formations were taken into account. In order to determine the chemical equilibrium compositions of the resulting solutions a new leaching procedure was developed and successfully employed with several toxic wastes. The results for a fly ash waste stemming from a glass smelting furnace are given in detail. Zinc and cadmium are the two most prominent heavy metals, that accumulate significantly in the leachates. In order to gain an insight into the complex dissolution and precipitation processes in such multi-component systems, geochemical modelling was performed using the program code EQ3/6 and the Pitzer formalism for calculating the activity coefficients. The thermodynamic database used was extended and Pitzer coefficients for Zn and Cd in high saline solutions were derived from literature data and added to the database. The results of the geochemical modelling of the investigated reactions were in good agreement with the experimental data. On this basis the maximum concentrations that can be leached from the investigated fly ash into a Mg-rich saline solution, that is typical for a salt repository in Northern Germany, are predicted to be 0,181 mol/kg H2O zinc and 0,00317 mol/kg H2O cadmium, respectively.  相似文献   
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BaAl2Ge2O8-Feldspar undergoes an order-disorder phase transition I2/c↔C2/m at T tr ≈1690 K. The thermodynamics of the Al,Ge cation ordering process is described in terms of the compressible Ising model in mean field approximation. The mean field potential predicts a first order character of the phase transition. This is compared to antiferromagnetic ordering in a two-dimensional square Ising model with NN-pair interactions and four-spin interactions on alternating squares. Calculated order parameters and short range ordering are in good agreement with the corresponding properties observed in BaAl2Ge2O8-feldspar by means of X-ray diffraction, hard mode infrared spectroscopy and TEM. Using known calorimetric data a similar model is postulated for Al,Si ordering in anorthite, CaAl2Si2O8, for which the derived potential describes a transition with slightly stronger first order character at T tr ≈1928 K. Received: 30 January 1998 / Revised, accepted: 29 August 1998  相似文献   
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The general purpose finite element code DYNA2D is used to calculate the response of an unlined tunnel in jointed rock, with sliding interfaces used to represent the joints. The model problem selected for analysis closely follows a calculation using the discrete element code UDEC. Results for two cases [(1) jointed rock with lubricated joints (no joint friction) and (2) jointed rock with frictional resistance to joint motion] are presented and compared with each other and the UDEC results.  相似文献   
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Simple evolutionary models of asteroids of various sizes and solar distances have been constructed assuming unipolar electrical induction heating due to passage of the Sun through a T Tauri phase with an increased magnetic field. Typical T Tauri conditions and an elementary solar wind model were used to calculate induced currents in modlels assuming electrical conductivities appropriate for carbonaceous material. Two restrictions with opposite dependence upon radius dominate the results. The electrical insulating tendency of a cold surface favors heating of larger bodies. The current-limiting backpressure of the induced magnetic field favors heating of smaller bodies. Thus it is found that maximum heating, in some cases sufficient for melting, occurs for model asteroids at the inner edge of the belt and with (model-dependent) radii from 25 to 250 km. This effect, if operant, would have produced a primordial distribution of metamorphosed asteroids primarily occurring at small solar distance and intermediate size. The observational evidence for such a distribution is unclear because the primordial distribution has likely been considerably modified by collisions, particularly at smaller sizes. There does seem to be some consistency with the model in the distribution of the largest asteroids, though data are sparse. In particular, this model seems relevant to the well-known dichotomy between Ceres and Vesta.Paper dedicated to Professor Hannes Alfvén on the occasion of his 70th birthday, 30 May, 1978Also Dept of Planetary Sciences  相似文献   
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The parameterization of the non-neutral atmospheric surface layer has been reexamined using the basic principles of small-scale energetics and thermodynamics. On the basis of this more complete treatment, the K- parameterization has been reformulated. It is found that the linear regression laws between fluxes and driving gradient forces of the turbulent heat and humidity exchanges in the surface layer can be derived in a much more comprehensive manner than by using the commonly used K-theory. With respect to stationary conditions and in the context of similarity concepts, a system of algebraic equations has been formulated which provides reasonable estimates of the distributions of the dimension-less rates of viscous energy dissipation as well as turbulent kinetic and thermal-diffusive energy transport as functions of the variable z/L. Quantitative calculations have been performed using the scaling height formulations of Takeuchi and Yokoyama, Prandtl, and von Kármán as closure conditions of the equations.  相似文献   
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