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21.
Silke Merchel Ulrich Ott Siegfried Herrmann Thomas Faestermann Gunther Korschinek Anton Wallner 《Geochimica et cosmochimica acta》2003,67(24):4949-4960
We have developed a procedure that allows extraction of clean nanodiamond samples from primitive meteorites for isotopic analyses of trace elements on a timescale of just a week. This procedure includes microwave digestion and optimization of existing isolation techniques for further purification. Abundances of trace elements that are difficult to dissolve using standard procedures (e.g., Ir) are lower in the diamond residues prepared using the new technique. Accelerator mass spectrometry (AMS) was explored as a means for isotopic measurements. Results obtained on diamond fractions from Allende and Murchison show the need for suitable matrix-adjusted standards to correct for fractionation effects; nevertheless they allow putting an upper limit on the abundance of 198Pt-H in nanodiamonds of ∼1 × 1014 atoms/g. This limit is on the order of what can be expected from predictions of competing nucleosynthesis models and extrapolation of the apparently mass dependent abundance trend of the associated noble gases.Unfortunately, and unexpectedly, presolar silicon carbide is almost quantitatively dissolved during microwave digestion with HCl/HF/HNO3. Re-evaluation of the standard extraction technique, however, shows that it also may lead to severe loss of fine-grained SiC, a fact not commonly appreciated. A lower limit to SiC abundance in Murchison is 20 ppm, and previous conclusions that Murchison SiC is unusually coarse-grained compared to SiC in other primitive meteorites seem not to be warranted. Graphite and silicon nitride may survive and possibly can be separated after this step as suggested by a simulation experiment using terrestrial analog material, but the detailed behavior of meteoritic graphite requires further study. 相似文献
22.
Gunther Kletetschka Petr Pruner Daniela Venhodova Jaroslav Kadlec 《Geochemical transactions》2007,8(1):2
A magnetic signature of tree rings was tested as a potential paleo-climatic indicator. We examined wood from sequoia tree,
located in Mountain Home State Forest, California, whose tree ring record spans over the period 600 – 1700 A.D. We measured
low and high-field magnetic susceptibility, the natural remanent magnetization (NRM), saturation isothermal remanent magnetization
(SIRM), and stability against thermal and alternating field (AF) demagnetization. Magnetic investigation of the 200 mm long
sequoia material suggests that magnetic efficiency of natural remanence may be a sensitive paleoclimate indicator because
it is substantially higher (in average >1%) during the Medieval Warm Epoch (700–1300 A.D.) than during the Little Ice Age
(1300–1850 A.D.) where it is <1%. Diamagnetic behavior has been noted to be prevalent in regions with higher tree ring density.
The mineralogical nature of the remanence carrier was not directly detected but maghemite is suggested due to low coercivity
and absence of Verwey transition. Tree ring density, along with the wood's magnetic remanence efficiency, records the Little
Ice Age (LIA) well documented in Europe. Such a record suggests that the European LIA was a global phenomenon. Magnetic analysis
of the thermal stability reveals the blocking temperatures near 200 degree C. This phenomenon suggests that the remanent component
in this tree may be thermal in origin and was controlled by local thermal condition. 相似文献
23.
The deep groundwater in the quaternary gravel sequence of the southern Upper Rhine Graben locally contains high chloride concentrations near the river Rhine between Fessenheim (France) in the South and Breisach (Germany) in the North. This historical pollution is mainly due to past infiltration from the former brine storage basins of the French potash mines on the Fessenheim Island and—to a lesser extent—from the leaching of the salt dumps of the German potash mines in Buggingen and Heitersheim. The spreading of the salt plume was investigated by means of a groundwater model. The aim of the model was to understand the brine movement, the present distribution of chloride as defined by recent hydrochemical investigations, and to select locations for new reconnaissance boreholes. The geological structure was reproduced by a three layer model, which was calibrated for steady state flow conditions. The hydraulic conductivity of the first layer was determined by comparing measured and calculated heads in the model area. The vertical resolution was refined to simulate the density-dependent salt transport processes. The transport of the salt plumes was simulated over a 40-year period, starting at the beginning of brine storage in the 1950s. The relevant transport parameters have been estimated in a sensitivity analysis, where the simulated breakthrough curves of chloride concentration have been compared with the measured data. The results of the groundwater model indicate that brines containing approximately 1 million tons of chloride are still present at the bottom of the aquifer. These highly concentrated salt brines mix with fresh water from the upper part of the aquifer. This dispersive process leads to the formation of a plume of chloride-rich water extending downstream, where pumping wells for several local water supplies are located. 相似文献
24.
Rosen G Rivera-Duarte I Chadwick DB Ryan A Santore RC Paquin PR 《Marine environmental research》2008,66(3):327-336
Critical tissue copper (Cu) residues associated with adverse effects on embryo-larval development were determined for the Mediterranean mussel (Mytilus galloprovincialis) and purple sea urchin (Strongylocentrotus purpuratus) following laboratory exposure to Cu-spiked seawater collected from San Diego Bay, California, USA. Whole body no-observed-effect-residues (NOER) were similar, with means of 21 and 23mugg(-1)dw, for M. galloprovincialis and S. purpuratus, respectively. Mean whole body median effect residues (ER50) were 49 and 142mugg(-1)dw for M. galloprovincialis and S. purpuratus, respectively. The difference in ER50s between species was reduced to a factor of <2 when expressed as soft tissue residues. Coefficients of variation among whole body-ER50s were 3-fold lower than median waterborne effect concentrations (EC50) for both species exposed to samples varying in water quality characteristics. This suggests that tissue concentrations were a better predictor of toxicity than water concentrations. The CBRs described herein do not differentiate between the internal Cu concentrations that are metabolically available and those that are accumulated and then detoxified. They do appear, however, to be well enough related to the level of accumulation at the site of action of toxicity that they serve as useful surrogates for the copper concentration that affects embryonic development of the species tested. Results presented have potentially important implications for a variety of monitoring and assessment strategies. These include regulatory approaches for deriving saltwater ambient water quality criteria for Cu, contributions towards the development of a saltwater biotic ligand model, the conceptual approach of using CBRs, and ecological risk assessment. 相似文献
25.
Gregory F. HERZOG Marc W. CAFFEE Thomas FAESTERMANN R. HERTENBERGER Gunther KORSCHINEK Ingo LEYA Robert C. REEDY J. M. SISTERSON 《Meteoritics & planetary science》2011,46(10):1427-1446
Abstract– Cross sections were measured for the nuclear reactions natMg(3He,x)26Al, 27Al(3He,x)26Al, natCa(3He,x)41Ca, and natCa(3He,x)36Cl in the energy region from approximately 5–35 MeV. The rates of these reactions are important for studies of early solar system irradiation scenarios. The 26Al, 36Cl, and 41Ca were separated chemically, and the numbers of atoms produced in each reaction channel were measured using accelerator mass spectrometry (AMS). From these results, 26 cross sections were determined and compared with predictions of the TALYS code. Agreement is within 40% for most cross sections. Our measurements were used to model the production of 7Be, 10Be, 26Al, and 41Ca in the early solar system. For projectiles 1H, 3He, and 4He, we assumed energy spectra of the general form E?α. For a wide range of parameterizations, the modeled ratios of 7Be/Be and 10Be/Be on the one hand and of 26Al/27Al and 41Ca/Ca on the other are coupled because the excitation functions for the relevant nuclear reactions have similar shapes. Modeling of a closed system with the constraint that 10Be/9Be = 0.001 fails to reproduce simultaneously the range of 7Be/9Be, 26Al/27Al, and 41Ca/Ca ratios inferred for the early solar system from studies of meteorites. 相似文献
26.
Kenneth S. Davis Niall C. Slowey Ingo H. Stender Hannelore Fiedler William R. Bryant Gunther Fechner 《Geo-Marine Letters》1996,16(3):273-278
The relationship between spatial variations of the properties of sea-floor sediments and acoustic backscatter from the surface of the sea floor on the continental shelf off of Panama City, Florida, USA, is investigated using surficial sediment grab samples and digital side-scan sonar data. Acoustic backscatter strength has a high, direct correlation with the mean grain size of the sediments. Acoustic backscatter strength also correlates directly with the carbonate content of the sediments, particularly in medium-and coarse-sand facies, because large, irregularly shaped, carbonate particles affect both the mean grain size of the sediments and the roughness of the surface of the sea floor. 相似文献
27.
The injection of CO2 into depleted natural gas reservoirs has been proposed as a promising new technology for combining enhanced gas recovery and geological storage of CO2. During the injection, application of suitable techniques for monitoring of the induced changes in the subsurface is required. Observing the movement and the changes in saturation of the fluids contained in the reservoir and the confining strata is among the primary aims here. It is shown that under conditions similar to the Altmark site, Germany, pulsed neutron-gamma logging can be applied with limitations. The pulsed neutron-gamma method can be applied for detection and quantification of changes in brine saturation and water content, whereas changes in the gas composition are below the detection limit. A method to account for the effects of salt precipitation resulting from evaporation of residual brine is presented. 相似文献
28.
Casey Bosse Gunther Rosen Marienne Colvin Patrick Earley Robert Santore Ignacio Rivera-Duarte 《Marine pollution bulletin》2014
The bioavailability and toxicity of copper (Cu) in Shelter Island Yacht Basin (SIYB), San Diego, CA, USA, was assessed with simultaneous toxicological, chemical, and modeling approaches. Toxicological measurements included laboratory toxicity testing with Mytilus galloprovincialis (Mediterranean mussel) embryos added to both site water (ambient) and site water spiked with multiple Cu concentrations. Chemical assessment of ambient samples included total and dissolved Cu concentrations, and Cu complexation capacity measurements. Modeling was based on chemical speciation and predictions of bioavailability and toxicity using a marine Biotic Ligand Model (BLM). Cumulatively, these methods assessed the natural buffering capacity of Cu in SIYB during singular wet and dry season sampling events. Overall, the three approaches suggested negligible bioavailability, and isolated observed or predicted toxicity, despite an observed gradient of increasing Cu concentration, both horizontally and vertically within the water body, exceeding current water quality criteria for saltwater. 相似文献
29.
Masumi Zaiki Gunther P. Können Keiji Kimura Takehiko Mikami Togo Tsukahara 《Climatic change》2009,95(1-2):231-248
The temperature and pressure differences between Tokyo and Nagasaki were used to reconstruct past climate conditions. January and July in each available year since the 1820s were classified into several types with characteristic sea level atmospheric pressure patterns. This results in 18 years of pre-1881 data and a continuous series thereafter. The series indicate that the warming after 1900 (after the end of the so-called Little Ice Age) and again after 1960 can at least partly be attributed to an increase in the frequency of warm circulation pattern types at the expense of cold types. The difference in nature of the shifts in circulation types that occurred in the late nineteenth century compared with that in the late twentieth centuries suggests that the mechanism behind the warming in the late nineteenth century differs from that in the late twentieth century. 相似文献
30.
Thomas M. Gunther 《Natural Resources Research》1992,1(4):267-280
Quantitative assessments and analyses of mineral resources can provide important input to decisions affecting public lands. This article, a companion article to Spanski, 1992, presents an application of resource assessment and analysis tools developed by the U.S. Bureau of Mines and the U.S. Geological Survey to U.S. Forest Service lands in northwest Montana. The analytical system described here integrates mineral deposit models, mine and mill cost-estimation models, and relevant economic and policy assumptions to estimate potential mineral production and the associated direct and indirect mineral-related economic impacts that could follow development of minerals. Finally, the impacts of land-use policies are estimated using the model. 相似文献