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41.
42.
Significant petrogenetic processes governing the geochemicalevolution of magma bodies include magma Recharge (includingformation of quenched inclusions or enclaves),heating and concomitant partial melting of country rock withpossible contamination of the evolving magma body(Assimilation), and formation and separation of cumulates byFractional Crystallization (RAFC). Although the importance ofmodeling such open-system magma chambers subject to energy conservationhas been demonstrated, the effects of concurrent removal ofmagma by eruption and/or variable assimilation (involving imperfectextraction of anatectic melt from wall rock) have not been considered.In this study, we extend the EC-RAFC model to include the effectsof Eruption and variable amounts of assimilation, A. This model,called EC-E'RAFC, tracks the compositions (trace elements andisotopes), temperatures, and masses of magma body liquid (melt),eruptive magma, cumulates and enclaves within a composite magmaticsystem undergoing simultaneous eruption, recharge, assimilationand fractional crystallization. The model is formulated as aset of 4 + t + i + s coupled nonlinear differential equations,where the number of trace elements, radiogenic and stable isotoperatios modeled are t, i and s, respectively. Solution of theEC-E'RAFC equations provides values for the average temperatureof wall rock (Ta), mass of melt within the magma body (Mm),masses of cumulates (Mct), enclaves (Men) and wall rock () and the masses of anatectic melt generated () and assimilated (). In addition, t trace element concentrations and i + s isotopic ratios inmelt and eruptive magma (Cm, m, m), cumulates (Cct, m, m), enclaves(Cen, , ) and anatectic melt (Ca, , ) as a function of magma temperature (Tm) are also computed. Input parametersinclude the (user-defined) equilibration temperature (Teq),a factor describing the efficiency of addition of anatecticmelt () from country rock to host magma, the initial temperatureand composition of pristine host melt (, , , ), recharge melt (, , , ) and wall rock (, , , ), distribution coefficients (Dm, Dr, Da) and their temperaturedependences (Hm, Hr, Ha), latent heats of transition (meltingor crystallization) for wall rock (ha), pristine magma (hm)and recharge magma (hr) as well as the isobaric specific heatcapacity of assimilant (Cp,a), pristine (Cp,m) and recharge(Cp,r) melts. The magma recharge mass and eruptive magma massfunctions, Mr(Tm) and Me(Tm), respectively, are specified apriori. Mr(Tm) and Me(Tm) are modeled as either continuous orepisodic (step-like) processes. Melt productivity functions,which prescribe the relationship between melt mass fractionand temperature, are defined for end-member bulk compositionscharacterizing the local geologic site. EC-E'RAFC has potentialfor addressing fundamental questions in igneous petrology suchas: What are intrusive to extrusive ratios (I/E) for particularmagmatic systems, and how does this factor relate to rates ofcrustal growth? How does I/E vary temporally at single, long-livedmagmatic centers? What system characteristics are most profoundlyinfluenced by eruption? What is the quantitative relationshipbetween recharge and assimilation? In cases where the extractionefficiency can be shown to be less than unity, what geologiccriteria are important and can these criteria be linked to fieldobservations? A critical aspect of the energy-constrained approachis that it requires integration of field, geochronological,petrologic, and geochemical data, and, thus, the EC-ERAFC systemsapproach provides a means for answering broad questions whileunifying observations from a number of disciplines relevantto the study of igneous rocks. KEY WORDS: assimilation; energy conservation; eruption; open system; recharge 相似文献
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44.
Magmatic Evolution of the Skye Igneous Centre, Western Scotland: Modelling of Assimilation, Recharge and Fractional Crystallization 总被引:3,自引:2,他引:1
The Skye igneous centre, forming part of the British Tertiarymagmatic province, developed over a 7 Myr period (6154Ma) and is characterized by a complex suite of lavas, hypabyssaland intrusive rocks of picritic to granitic composition. Theintrusion of magma from mantle to crust at 2x103km3/yr(6 Mt/yr) advected magmatic heat of roughly 0·2 GW averagedover the period of magmatism supporting an excessheat flux of about 130 mW/m2, or about twice the present-dayaverage continental heat flow. The volume of new crust generatedat Skye (15000 km3) spread over the present-day area of Skyecorresponds to 9 km of new crust. The geochemical evolutionof the Skye magmatic system is constrained using the Energy-ConstrainedRecharge, Assimilation, and Fractional Crystallization (EC-RAFC)model to understand variations in the Sr- and Pb-isotopic andSr trace-element composition of the exposed magmatic rocks withtime. The character (composition and specific enthalpy) of bothassimilant and recharge magma appears to change systematicallyup-section, suggesting that the magma reservoirs migrated toprogressively shallower levels as the system matured. The modelof the magma transport system that emerges is one in which magmabatches are stored initially at lower-crustal levels, wherethey undergo RAFC evolution. Residual magma from this stagethen migrates to shallower levels, where mid-crustal wall rockis assimilated; the recharge magma at this level is characterizedby an increasingly crustal signature. For some of the stratigraphicallyyoungest rocks, the data suggest that the magma reservoirs ascendedinto, and interacted with, upper-crustal Torridonian metasediments. KEY WORDS: assimilation; EC-RAFC model; geochemical modelling; magma recharge; Skye magmatism 相似文献
45.
THORSTEN HOFFMANN JAY R. ODUM FRANK BOWMAN DONALD COLLINS DIETER KLOCKOW RICHARD C. FLAGAN JOHN H. SEINFELD 《Journal of Atmospheric Chemistry》1997,26(2):189-222
Measurements of aerosol formation during thephotooxidation of -pinene, -pinene,d-3-carene, d-limonene, ocimene, linalool, terpinene-4-ol, andtrans-caryophyllene were conducted in anoutdoor smog chamber. Daylight experiments in thepresence of
and dark experiments withelevated ozone concentrations were performed. Theevolution of the aerosol was simulated by theapplication of a gas/particle absorption model inconnection with a chemical reaction mechanism. Thefractional aerosol yield is shown to be a function ofthe organic aerosol mass concentration andtemperature. Ozone and, for selected hydrocarbons, theNO3 reaction of the compounds were found torepresent efficient routes to the formation ofcondensable products. For initial hydrocarbon mixingratios of about 100 ppb, the fractional aerosol yieldsfrom daylight runs have been estimated to be 5%for open-chain hydrocarbons, such as ocimene andlinalool, 5–25% for monounsaturated cyclicmonoterpenes, such as -pinene, d-3-carene, orterpinene-4-ol, and 40% for a cyclic monoterpenewith two double bonds like d-limonene. For the onlysesquiterpene investigated, trans-caryophyllene, afractional aerosol yield of close to 100% wasobserved. The majority of the compounds studied showedan even higher aerosol yield during dark experimentsin the presence of ozone. 相似文献
46.
ANDREAS DEHNERT FRANK PREUSSER JAN D. KRAMERS NAKI AKÇAR PETER W. KUBIK REGINA REBER CHRISTIAN SCHLÜCHTER 《Boreas: An International Journal of Quaternary Research》2010,39(3):620-632
Dehnert, A., Preusser, F., Kramers, J. D., Akçar, N., Kubik, P. W., Reber, R. & Schlüchter, C. 2010: A multi‐dating approach applied to proglacial sediments attributed to the Most Extensive Glaciation of the Swiss Alps. Boreas, Vol. 39, pp. 620–632. 10.1111/j.1502‐3885.2010.00146.x. ISSN 0300‐9483. The number and the timing of Quaternary glaciations of the Alps are poorly constrained and, in particular, the age of the Most Extensive Glaciation (MEG) in Switzerland remains controversial. This ice advance has previously been tentatively correlated with the Riss Glaciation of the classical alpine stratigraphy and with Marine Isotope Stage (MIS) 6 (186–127 ka). An alternative interpretation, based on pollen analysis and stratigraphic correlations, places the MEG further back in the Quaternary, with an age equivalent to MIS 12 (474–427 ka), or even older. To re‐evaluate this issue in the Swiss glaciation history, a multi‐dating approach was applied to proglacial deltaic ‘Höhenschotter’ deposits in locations outside the ice extent of the Last Glacial Maximum. Results of U/Th and luminescence dating suggest a correlation of the investigated deposits with MIS 6 and hence with the Riss Glaciation. Cosmogenic burial dating suffered from large measurement uncertainties and unusually high 26Al/10Be ratios and did not provide robust age estimates. 相似文献
47.
48.
DANIEL VERES ELISABETH LALLIER-VERGÈS BARBARA WOHLFARTH TERRI LACOURSE DIDIER KÉRAVIS SVANTE BJÖRCK FRANK PREUSSER VALéRIE ANDRIEU-PONEL LINDA AMPEL 《Boreas: An International Journal of Quaternary Research》2009,38(2):230-243
A new set of geochemical data obtained from a long sediment sequence from the Les Echets basin provides a new record of palaeoenvironmental change for western Europe. The sequence covers the late part of Marine Isotope Stage (MIS) 3 and MIS 2 ( c . 46.1–15.0 cal. kyr BP) and extends over 30 m of sediment, allowing for high sampling resolution. Distinct cyclic fluctuations in aquatic productivity proxies suggest a tempo of environmental change at Les Echets that resembles the one established for Dansgaard-Oeschger cycles and Heinrich events. Increases in organic carbon are paralleled by high hydrogenous contents and enriched δ13 Corg and Corg /Ntot ratios, implying a mixture of aquatic and land-derived constituents. The stable isotope values are directly linked to primary aquatic productivity and the input of terrestrial organic matter, enriched during warm, productive, periods, and drastically depleted during cold periods, particularly Heinrich events. Phases of relatively high productivity correlate with Dansgaard-Oeschger interstadials 8–2, while Heinrich events 3 and 2 are also clearly delineated by distinct lithological horizons with very low organic contents, high dry densities and enhanced organic matter oxidation. A large hiatus occurring about the time of Heinrich event 4 suggests that the cold and dry climate reconstructed for this event in the North Atlantic region also greatly affected Les Echets and its catchment. 相似文献
49.
Pressure, Temperature, and Structural Evolution of West-Central New Hampshire: Hot Thrusts over Cold Basement 总被引:2,自引:0,他引:2
KOHN MATTHEW J.; ORANGE DANIEL L.; SPEAR FRANK S.; RUMBLE DOUGLAS III; HARRISON T. MARK 《Journal of Petrology》1992,33(3):521-556
Pressure-temperature (P-T) paths have been calculated from pelitesand amphibolites of several major Acadian structures in west-centralNew Hampshire by using both inclusion thermobarometry and differentialthermodynamics (the Gibbs method). P-T paths calculated forrocks exposed in the Orfordville and Bronson Hill anticlinoriaare clockwise and show 12.5 kb of exhumationwith 30100 C of heating. Because this type of path ischaracteristic of the lower plate of overthrust terranes, theserocks are interpreted to be (para)autochthonous. P-T paths forrocks exposed in an intervening synclinorium (the Hardscrabblesynclinorium) show isothermal loading of 13 kb followedby possible isobaric cooling. This behavior is characteristicof rocks occupying a middle-plate structural position withina multiple thrust package, and so these rocks are interpretedto be allochthonous. The interpretation that the Hardscrabblerocks are allochthonous differs from previous models, but betterexplains the petrologic data and is consistent with the stratigraphicand structural data on which other models have been based. Correlation of the P-T paths with deformational events throughkinematic and textural analysis indicates that during nappestage deformation, the synclinorial rocks were transported westward,and that the anticlinorial and synclinorial rocks were buriedto depths of 2530 and 2025 km respectively. Theexhumation with heating recorded by the anticlinorial samplesoccurred during the dome stage of deformation, and differentiallyuplifted the anticlinorial rocks relative to the synclinorialrocks; this differential uplift may have been accommodated throughreactivation of early thrust faults with normal movement sense.P-T paths of the Hardscrabble synclinorium rocks are suggestiveof a relatively elevated initial geothermal gradient for theirpre-nappe source terrane, which is interpreted to have beenbetween the Kearsarge-Central Maine basin and the Bronson Hillparautochthon. 相似文献
50.
A new, detailed tectonic model is presented for the Acadianorogenic belt of central New England (Vermont and New Hampshire)that accounts for a wide range of petrological and structuralobservations. Three belts are considered: the Eastern Vermont,Merrimack, and intervening Bronson Hill belts. Specific observationsin eastern Vermont that are accounted for in the model includethe following. PT paths are clockwise with maximum pressuresnear the Athens, Chester, and Strafford domes of 811kbar, but with maximum pressures decreasing to 35 kbarat the boundary with the Bronson Hill belt. Differential exhumationof the Vermont domes relative to the rocks in easternmost Vermontis required by the recorded differences in maximum pressure(56 kbar; 1520 km) and the present-day geographicalseparation (710 km). Specific observations in New Hampshirethat are explained include the following. PT paths inthe Merrimack belt are counter-clockwise with maximum pressuresof 45 kbar and are related to high regional heat flowand heat transfer by early Acadian plutons. PT pathsin the Bronson Hill belt are intimately associated with structuralposition. An early contact metamorphism is evidenced in theSkitchewaug and Fall Mountain nappes near contacts with theearly Acadian Bethlehem gneiss ( 相似文献