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991.
I. E. Paukov N. K. Moroz Yu. A. Kovalevskaya I. A. Belitsky 《Physics and Chemistry of Minerals》2002,29(4):300-306
The heat capacity of paranatrolite and tetranatrolite with a disordered distribution of Al and Si atoms has been measured
in the temperature range of 6–309 K using the adiabatic calorimetry technique. The composition of the samples is represented
with the formula (Na1.90K0.22Ca0.06)[Al2.24Si2.76O10]·nH2O, where n=3.10 for paranatrolite and n=2.31 for tetranatrolite. For both zeolites, thermodynamic functions (vibrational entropy, enthalpy, and free energy function)
have been calculated. At T=298.15 K, the values of the heat capacity and entropy are 425.1 ± 0.8 and 419.1 ±0.8 J K−1 mol−1 for paranatrolite and 381.0 ± 0.7 and 383.2 ± 0.7 J K−1 mol−1 for tetranatrolite.
Thermodynamic functions for tetranatrolite and paranatrolite with compositions corrected for the amount of extraframework
cations and water molecules have also been calculated. The calculation for tetranatrolite with two water molecules and two
extraframework cations per formula yields: C
p
(298.15)=359.1 J K−1 mol−1, S(298.15) −S(0)=362.8 J K−1 mol−1. Comparing these values with the literature data for the (Al,Si)-ordered natrolite, we can conclude that the order in tetrahedral
atoms does not affect the heat capacity. The analysis of derivatives dC/dT for natrolite, paranatrolite, and tetranatrolite has indicated that the water- cations subsystem within the highly hydrated
zeolite may become unstable at temperatures above 200 K.
Received: 30 July 2001 / Accepted: 15 November 2001 相似文献
992.
F. Ouchterlony M. Olsson I. Bergqvist 《Fragblast: International Journal for Blasting and Fragmentation》2002,6(2):235-261
A Swedish table of blast damage depths has, in one form or other, been in use since the late-1970s. Its history and the underlying theory are described. New experimental and theoretical findings that point out a number of shortcomings in the table and the underlying theory are presented and discussed. A revised version of the blast damage table was recently introduced in conjunction with new but incomplete recommendations for cautious perimeter blasting. The new table leaves the difficult task of taking into account factory like decoupling, water in the borehole, the rock properties, type of initiation, charge length and the actual bit diameter to the user. This paper discusses different ways of doing this, based on the experimental findings and a recent formula for the prediction of the lengths of radial cracks behind the half-casts. The material presented in this paper is meant to supplement and extend the new Swedish recommendations for cautious perimeter blasting of tunnels, shafts, pits and road cuts. 相似文献
993.
We have experimentally studied the formation of diamonds in alkaline carbonate–carbon and carbonate–fluid–carbon systems at 5.7–7.0 GPa and 1150–1700 °C, using a split-sphere multi-anvil apparatus (BARS). The starting carbonate and fluid-generating materials were placed into Pt and Au ampoules. The main specific feature of the studied systems is a long period of induction, which precedes the nucleation and growth of diamonds. The period of induction considerably increases with decreasing P and T, but decreases when adding a C–O–H fluid to the system. In the range of P and T corresponding to the formation of diamonds in nature, this period lasts for tens of hours. The reactivity of the studied systems with respect to the diamond nucleation and growth decreases in this sequence: Na2CO3–H2C2O4·2H2O–C>K2CO3–H2C2O4·2H2O–C>>Na2CO3–C>K2CO3–C. The diamond morphology is independent of P and T, and is mainly governed by the composition of the crystallization medium. The stable growth form is a cubo-octahedron in the Na2CO3 melt, and an octahedron in the K2CO3 melt. Regardless of the composition of the carbonate melt, only octahedral diamond crystals formed in the presence of the C–O–H fluid. The growth rates of diamond varied in the range from 1.7 μm/h at 1420 °C to 0.1–0.01 μm/h at 1150 °C, and were used to estimate, for the first time, the possible duration of the crystallization of natural diamonds. From the analysis of the experimental results and the petrological evidence for the formation of diamonds in nature, we suggest that fluid-bearing alkaline carbonate melts are, most likely, the medium for the nucleation and growth of diamonds in the Earth's upper mantle. 相似文献
994.
995.
996.
A. K. Varma R. M. Gairola A. K. Mathur B. S. Gohil Vijay K. Agarwal 《Journal of Earth System Science》2002,111(3):247-256
In this paper, MSMR geophysical products like Integrated Water Vapour (IWV), Ocean Surface Wind Speed (OWS) and Cloud Liquid
Water (CLW) in different grids of 50, 75 and 150 kms are compared with similar products available from other satellites like
DMSP-SSM/I and TRMMTMI. MSMR derived IWV, OWS and CLW compare well with SSM/I and TMI finished products. Comparison of MSMR
derived CLW with that derived from TMI and SSM/I is relatively in less agreement. This is possibly due to the use of 37 GHz
in SSM/I and TMI that is highly sensitive to CLW, while 37 GHz channels are not available on MSMR. Monthly comparison of MSMR
geophysical products with those from TMI is all carried out for climatological purpose. The monthly comparisons were much
better compared to instantaneous comparisons. In this paper, details of the data analysis and comparison results are presented.
The usefulness of the MSMR vis-à-vis other sensors is also discussed. 相似文献
997.
Hydraulic Characteristics of Rough Fractures in Linear Flow under Normal and Shear Load 总被引:19,自引:3,他引:19
Summary
A hydro-mechanical testing system, which is capable of measuring both the flow rates and the normal and shear displacement
of a rock fracture, was built to investigate the hydraulic behaviour of rough tension fractures. Laboratory hydraulic tests
in linear flow were conducted on rough rock fractures, artificially created using a splitter under various normal and shear
loading. Prior to the tests, aperture distributions were determined by measuring the topography of upper and lower fracture
surfaces using a laser profilometer. Experimental variograms of the initial aperture distributions were classified into four
groups of geostatistical model, though the overall experimental variograms could be well fitted to the exponential model.
The permeability of the rough rock fractures decayed exponentially with respect to the normal stress increase up to 5 MPa.
Hydraulic behaviours during monotonic shear loading were significantly affected by the dilation occurring until the shear
stress reached the peak strength. With the further dilation, the permeability of the rough fracture specimens increased more.
However, beyond shear displacement of about 7 to 8 mm, permeability gradually reached a maximum threshold value. The combined
effects of both asperity degradation and gouge production, which prohibited the subsequent enlargement of mean fracture aperture,
mainly caused this phenomenon. Permeability changes during cyclic shear loading showed somewhat irregular variations, especially
after the first shear loading cycle, due to the complex interaction from asperity degradations and production of gouge materials.
The relation between hydraulic and mechanical apertures was analyzed to investigate the valid range of mechanical apertures
to be applied to the cubic law.
Received June 12, 2001; accepted February 26, 2002 Published online September 2, 2002 相似文献
998.
999.
Poroelastic analysis of cover-collapse sinkhole formation by piezometric surface drawdown 总被引:1,自引:0,他引:1
T. Tharp 《Environmental Geology》2002,42(5):447-456
Where the water table is above the soil-rock contact in karst regions, cover-collapse sinkholes in the soil and soft sediment above the rock commonly occur as a result of drawdown of the piezometric surface in the karst aquifer. Transient stresses and pore pressures around soil voids at the soil-rock contact can cause hydraulic fracturing of the soil near the wall of the void. After the first such fracture, successive sloughing of soil propagates the soil void rapidly to the surface, resulting in a cover-collapse sinkhole. Sinkhole formation by this mechanism should be strongly a function of rate and magnitude of piezometric surface drawdown, permeability and tensile strength of the soil, and the size, depth, and geometry of the initial soil void. Large soil voids and those with walls that are partly planar or of low curvature are most susceptible to hydraulic fracture and the resulting progression to sinkhole formation. 相似文献
1000.
Heavy metal concentrations in surficial sediments from accreting and eroding areas along the coast of Guyana 总被引:1,自引:0,他引:1