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201.
Jae-Seok Kim Anna Liza Bais Sun-hee Kang Jaehoon Lee Kihong Park 《Journal of Atmospheric Chemistry》2011,68(3):251-263
Ammonia has a short residence time in the atmosphere and rapidly neutralizes acid gases that occur near its source, requiring a rapid measurement system for ammonia and particulate ammonium concentrations to better understand their sources, temporal variation of ammonia emissions, and the formation of secondary ammonium aerosols. A semi-continuous measurement system, consisting of a diffusion scrubber, a particle growth chamber, an air-liquid separator, and a fluorescent detector, was developed to determine both gaseous ammonia (NH3) and particulate ammonium (NH 4 + ) in PM2.5 in the ambient atmosphere of Gwangju, South Korea, during the months of March, April, July, and September of 2007. During the sampling periods, the average concentrations of ammonia and ammonium were found to be 2.33?±?1.29 μg/m3 and 1.89?±?0.99 μg/m3, respectively. Although the average gaseous ammonia concentration was highest in March, the particulate ammonium concentration was higher during the warmer season, reaching 2.08?±?1.07 μg/m3 and 2.32?±?0.94 μg/m3 in April and July, respectively, while only 1.68?±?0.61 μg/m3 in March and 1.24?±?0.99 μg/m3 in September. It is proposed that the higher availability of acid species during the warmer months produced a significant amount of particulate ammonium sulfate. Diurnal fluctuation of ammonia and ammonium during the warmer months showed that their peak time occurred at approximately 10:00 am. Both ammonia and ammonium concentrations were better correlated during the warmer months than during the cooler months. Further, the data suggest that the ammonia and ammonium were measured under well dispersed conditions, and multiple sources contributed to the ammonia at the sampling site. 相似文献
202.
The aim of this study was to display distribution and relationships of heavy elements in the unconfined, shallow alluvial aquifers of the lower Jia Bharali catchment and adjoining areas in central part of North Brahmaputra Plain (NBP), India using hydrochemical as well as multivariate statistical techniques such as principal component analysis (PCA) and cluster analysis. The original matrix was made up of 10 trace elements (As, Cd, Cu, Co, Cr, Fe, Mn, Pb, Ni and Zn) estimated from 50 shallow alluvial dug wells in both the wet and the dry season for a duration of 3 hydrological years (2008–2011). Except As, Cu and Zn all the other toxic metals in the shallow aquifers were found exceeding the WHO maximum permissible limits for drinking water. PCA extracted five varimax factors as geogenic, agricultural and anthropogenic explaining about 71.2% of the total variance in the wet season and 69.3% total variance in the dry season. Hierarchical cluster analysis classified the dug wells into two groups in the wet season and three groups in the dry season with respect to the heavy elements. The results emphasized the need for routine monitoring and management in order to avoid contamination of groundwater sources in the NBP with respect to the dissolved trace elements. 相似文献
203.
Akhtar R. Mir V. Balaram Javid A. Ganai Shamim A. Dar A. Keshav Krishna 《中国地球化学学报》2016,35(4):428-436
The geochemical characteristics of two sections—the Permian–Triassic boundary (PTB) Guryul Ravine section, Kashmir Valley, Jammu and Kashmir, India; and the Attargoo section, Spiti Valley, Himachal Pradesh, India—have been studied in the context of provenance, paleo-weathering, and plate tectonic setting. These sections represent the siliciclastic sedimentary sequence from the Tethys Himalaya. The PTB siliciclastic sedimentary sequence in these regions primarily consists of sandstones and shales with variable thickness. Present studied sandstones and shales of both sections had chemical index of alteration values between 65 and 74; such values reveal low-to-moderate degree of chemical weathering. The chemical index of weathering in studied samples ranged from 71 to 94, suggesting a minor K-metasomatism effect on these samples. Plagioclase index of alteration in studied sections ranged from 68 to 92, indicating a moderate degree of weathering of plagioclase feldspars. The provenance discriminant function diagram suggests that the detritus involved in the formation of present studied siliciclastic sedimentary rocks fall in quartzose sedimentary and felsic igneous provenances. These sediments were deposited in a passive continental margin plate tectonic setting according to their location on a Si2O versus K2O/Na2O tectonic setting diagram. 相似文献
204.
Anis Gasmi Cécile Gomez Hédi Zouari Antoine Masse Danielle Ducrot 《Arabian Journal of Geosciences》2016,9(20):753
The purpose of this study was to examine the efficiency of Advanced Space Borne Thermal Emission and Reflection Radiometer (ASTER) data in the discrimination of geological formations and the generation of geological map in the northern margin of the Tunisian desert. The nine ASTER bands covering the visible (VIS), near-infrared (NIR) and short-wave infrared (SWIR) spectral regions (wavelength range of 400–2500 nm) have been treated and analyzed. As a first step of data processing, crosstalk correction, resampling, orthorectification, atmospheric correction, and radiometric normalization have been applied to the ASTER radiance data. Then, to decrease the redundancy information in highly correlated bands, the principal component analysis (PCA) has been applied on the nine ASTER bands. The results of PCA allow the validation and the rectification of the lithological boundaries already published on the geologic map, and gives a new information for identifying new lithological units corresponding to superficial formations previously undiscovered. The application of a supervised classification on the principal components image using a support vector machine (SVM) algorithm shows good correlation with the reference geologic map. The overall classification accuracy is 73 % and the kappa coefficient equals to 0.71. The processing of ASTER remote sensing data set by PCA and SVM can be employed as an effective tool for geological mapping in arid regions. 相似文献
205.
Irina N. Plotnikova 《International Journal of Earth Sciences》2008,97(5):1131-1142
The study area is the South Tatarstan Arch located in the Volgo-Ural Region, which is an enigmatic crustal segment occupying
one third of the East European Platform. Monitoring studies have shown that fluid discharge processes are still active and
time-dependent. This paper presents an integrated review of the geological, geophysical, hydrochemical and geochemical studies
of the crystalline basement of Tatarstan. These studies are based on the stratigraphic and compositional schemes within the
crystalline basement, the drilling of deep wells, the geodynamic activity of the fractured zones of the crystalline basement
and the presence of fluids therein. Furthermore, the changes in the chemical composition of the basement waters are taken
into account. 相似文献
206.
Chemistry of major and minor elements, 87Sr/86Sr, δD, δ18O and δ34S of brines were measured from Tertiary strata and Quaternary salt lakes in the western Qaidam Basin. The water chemistry
data show that all oilfield brines are CaCl2 type. They were enriched in Ca2+, B3+, Li+, Sr2+, Br−, and were depleted in Mg2+, SO4
2−, which indicated that these brines had the characteristics of deeply circulated water. The relationship between δD and δ18O shows that all data of these brines decline towards the Global Meteoric Water Line (GWL) and Qaidam Meteoric Water Line
(QWL), and that the intersection between oilfield brines and Meteoric Water Lines was close to the local spring and fresh
water in the piedmont in the western Qaidam Basin. The results suggest that oilfield brines has initially originated from
meteoric water, and then might be affected by water-rock metamorphose, because most oilfield brines distribute in the range
of metamorphosing water. The 87Sr/86Sr values of most oilfield brines range from 0.71121 to 0.71194, and was less than that in salt lake water (>0.712), but close
to that of halite in the study area. These imply that salt dissolution occurred in the process of migration. In addition,
all oilfield brines have obviously much positive δ34S values (ranging from 26.46‰ to 54.57‰) than that of salt lake brines, which was caused by bacterial sulfate reduction resulting
in positive shift of δ34S value and depleteed SO4
2− in oilfield brines. Combined with water chemical data and δD, δ18O, 87Sr/86Sr, δ34S values, we concluded that oilfield brines mainly originate from the deeply circulated meteoric waters, and then are affected
by salt dissolution, water-rock metamorphose, sulfate reduction and dolomitization during the process of migration. These
processes alter the chemical compositions of oilfield brines and accumulate rich elements (such as B, Li, Sr, Br, K and so
on) for sustainable utilization of salt lake resources in the Qaidam Basin. 相似文献
207.
A method for the prediction of ocean waves was developed on the basis of the single-parameter growth equation of wind waves, proposed byToba (1978) on the basis of similarity in growing wind waves. The applicability of the method to actual problems was tested by hindcasting the wave characteristics with the method, for two cases with differing time and space scales, one in Kii Channel Approach, Japan, and the other in the North Atlantic Ocean. The results showed that the present method can predict waves within an error of 1.3 m in wave heights, which ranged from 3 to 12 m. 相似文献
208.
Qingchao Li Yuanfang Cheng Qiang Li Ubedullah Ansari Yuwen Liu Chuanliang Yan Chuang Lei 《Arabian Journal of Geosciences》2018,11(12):325
Natural gas hydrate is widely distributed all over the world and may be a potential resource in the near future, whereas hydrate dissociation during the development affects wellbore stability and drilling safety. However, the present modeling of hydrate reservoir parameters ignored the influence of effective stress and only considered the hydrate saturation. In this paper, a series of stress sensitivity experiments for the unconsolidated sandstone were carried out, and the influence of mean effective stress on physical parameters was obtained; a comprehensive model for the physical parameters of hydrate reservoir was developed subsequently. With the help of ABAQUS finite element software, the established comprehensive model was verified by the use of the wellbore stability numerical model of hydrate reservoir. The verification results show that ignoring the effect of mean effective stress on the parameters of hydrate formation aggravates the invasion of drilling fluid into the hydrate formation. Besides, ignoring the stress sensitivity of reservoir physical parameters will underestimate the wellbore instability during hydrate drilling, which will be a threat to the safety of gas hydrate drilling. At the end of the drilling operation, the maximum plastic strain of the model for considering and not considering stress sensitivity was 0.0145 and 0.0138, respectively. Therefore, the established comprehensive model will provide a theoretical support for accurately predicting the engineering geological disasters in hydrate development process. 相似文献
209.
Nivedita Sanwlani Prakash Chauhan Ranganath R. Navalgund 《Journal of the Indian Society of Remote Sensing》2010,38(4):617-626
Space-borne ocean-colour remote sensor-detected radiance is heavily contaminated by solar radiation backscattered by the atmospheric
air molecules and aerosols. Hence, the first step in ocean-colour data processing is the removal of this atmospheric contribution
from the sensor-detected radiance to enable detection of optically active oceanic constituents e.g. chlorophyll-a, suspended sediment etc. In standard atmospheric correction procedure for OCEANSAT-1 Ocean Colour Monitor (OCM) data, NIR
bands centered at 765 and 865 nm wavelengths were used for aerosol characterization. Due to high absorption by water molecules,
ocean surface in these two wavelengths acts as dark background, therefore, sensor detected radiance can be assumed to have
major contribution from atmospheric scattering. For coastal turbid waters this assumption of dark surface fails due to the
presence of highly scattering sediments which causes sufficient water-leaving radiance in NIR bands and lead to over-estimation
of aerosol radiance resulting in negative water leaving radiance for λ < 700 nm. In the present study, for the turbid coastal
waters in the northern Bay of Bengal, the concept of spatial homogeneity of aerosol and water leaving reflectance has been
applied to perform atmospheric correction of OCAEANSAT-1 OCM data. The results of the turbid water atmospheric correction
have also been validated using in-situ measured water-leaving radiance. Comparison of satellite derived water-leaving radiance for five coastal stations with in-situ measured radiance spectra, indicates an improvement over the standard atmospheric correction algorithm giving physically
realistic and positive values. Root Mean Square Error (RMSE) between the in-situ measured and satellite derived water leaving radiance for wavelengths 412 nm, 443 nm, 490 nm, 512 nm and 555 nm was found
to be 1.11, 0.718, 0.575, 0.611 and 0.651%, respectively, using standard atmospheric correction procedure. By the use of spatial
homogeneity concept, this error was reduced to 0.125, 0.173, 0.176, 0.225, and 0.290 and the correlation coefficient arrived
at 0.945, which is an improvement over the standard atmospheric correction procedure. 相似文献
210.
Michio J. Kishi Shin-ichi Ito Bernard A. Megrey Kenneth A. Rose Francisco E. Werner 《Journal of Oceanography》2011,67(1):3-16
The evolution of the North Pacific Ecosystem Model for Understanding Regional Oceanography (NEMURO) family of models to study
marine ecosystems is reviewed. Applications throughout the North Pacific have shown the models to be robust and to be able
to reproduce 1D, 2D and 3D components of nutrient, carbon cycle and biogeochemical cycles as well as aspects of the lower
trophic levels ecosystem (phyto- and zooplankton). NEMURO For Including Saury and Herring, an extension that includes higher
trophic levels, can be run uncoupled or coupled to NEMURO. In the uncoupled mode, the growth and weight of an individual fish
is computed using plankton densities simulated by NEMURO but with no feedback between fish consumption and plankton mortality.
In the coupled mode, the feeding, growth and weight of a representative fish are computed, and prey removals due to feeding
by fish appear as mortality terms on the prey. The NEMURO family of models continues to evolve, including effects of the microbial
loop and iron limitation at lower trophic levels, and full life cycle, multi-species and multi-generational simulations at
higher trophic levels. We outline perspectives for future end-to-end modeling efforts that can be used to study marine ecosystems
in response to global environmental change. 相似文献