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71.
Two chemical processes can remove Mg2+ from suspensions containing amorphous silica (am-SiO2) at low temperatures: adsorption and precipitation of a Mg-hydroxysilicate resembling sepiolite. Mg2+ removal from am-SiO2 suspensions was investigated, and the relative role of the two removal processes evaluated, as a function of: pH, ionic strength, Mg2+ concentration, and temperature.The extent of Mg2+ adsorption onto am-SiO2 decreases with increasing NaCl concentration due to displacement of Mg2+ by Na+. At NaCl concentrations of 0.05 M and above, adsorption occurs only at pH values above 8.5, where rapid dissolution of am-SiO2 gives rise to high concentrations of dissolved silica, resulting in supersaturation with respect to sepiolite. Removal of Mg2+, at concentrations of 40 to 650 μM, from am-SiO2 suspensions in 0.70 M NaCl at 25 °C occurs at pH 9.0 and above. Experiments show that under these conditions adsorption and Mg-hydroxysilicate precipitation remove Mg2+ at similar rates. For 0.05 M Mg2+, at 0.70 M ionic strength and 25 °C, measurable Mg2+ removal occurs down to ca. pH 7.5 but is primarily due to Mg-hydroxysilicate precipitation. For the same solution conditions at 5°C, Mg2+ removal occurs above pH 8.0 and is primarily due to adsorption.Assuming that increasing pressure does not greatly enhance adsorption, Mg2+ adsorption onto am-SiO2 is an insignificant process in sea water. The surface charge of pristine am-SiO2 in sea water is primarily controlled by interactions with Na+. The principal reaction between Mg2+ and am-SiO2 in marine sediments is sepiolite precipitation.The age distribution of sepiolite in siliceous pelagic sediments is influenced by temperatures of bottom waters and by geothermal gradients. 相似文献
72.
D. S. Coombs Y. Kawachi B. F. Houghton G. Hyden I. J. Pringle J. G. Williams 《Contributions to Mineralogy and Petrology》1977,63(3):229-246
Almost pure andradite and intermediate members of the andradite-grossular series (gros40–49, and 47–54, py0–3, alm0–3, spess0–2, hydrogarnet0–3), often framboidal in habit, are widespread in metabasites including lavas, minor intrusions, and volcanic sandstones and
breccias metamorphosed under prehnite-pumpellyite and pumpellyite-actinolite facies conditions, possibly extending into the
zeolite facies. Coexisting phases include iron-rich epidotes (100 Fe*/Fe*+Al=22–34), pumpellyite, prehnite, actinolite, and
chlorite, electron microprobe analyses of which are given, as well as quartz, albite, and calcite. Zoisite (100 Fe*/Fe*+Al=1–5)
and iron-poor epidote (100 Fe*/Fe*+Al=11–18) occur in 2 rocks in pseudomorphs after plagioclase together with more iron-rich
epidote, but not in close association with the garnets. Coexisting pumpellyite is iron-rich (FeO* 9–14%) in the prehnite-pumpellyite
facies and iron-poor (FeO* 5%) in the pumpellyiteactinolite facies. Chlorites and actinolites vary widely and sympathetically
in FeO/MgO+FeO ratio. Andradite is also described from a stilpnomelane-actinolite-hematite-bearing andradite quartzite of
the pumpellyite-actinolite facies.
Conditions of formation involved temperatures of 300 to 400 ° or less, at pressures up to a few kilobars. A wide range of
oxygen fugacities is possible, but
in the fluid phase was low. Grandite and chlorite are incompatible in the pumpellyite-actinolite and greenschist facies in
the presence of quartz but the 2 minerals occur together in some pumpellyite-actinolite facies assemblages as a result of
incomplete reaction and/or local deficiency in silica. In the greenschist facies the association is replaced by epidote-actinolite±hematite
and sodic amphibole.
Whereas at medium to high grades of metamorphism andradite and grandite are characteristic of skarns irrespective of
, at very low grades they are found in mafic volcanic rocks and volcanogenic sediments as well as in certain cherty rocks
of unusual composition, rodingites, and serpentinites, where
was very low. 相似文献
73.
We investigate how well the variability of extreme daily precipitation events across the United Kingdom is represented in a set of regional climate models and the E-OBS gridded data set. Instead of simply evaluating the climatologies of extreme precipitation measures, we develop an approach to validate the representation of physical mechanisms controlling extreme precipitation variability. In part I of this study we applied a statistical model to investigate the influence of the synoptic scale atmospheric circulation on extreme precipitation using observational rain gauge data. More specifically, airflow strength, direction and vorticity are used as predictors for the parameters of the generalised extreme value (GEV) distribution of local precipitation extremes. Here we employ this statistical model for our validation study. In a first step, the statistical model is calibrated against a gridded precipitation data set provided by the UK Met Office. In a second step, the same statistical model is calibrated against 14 ERA40 driven 25?km resolution RCMs from the ENSEMBLES project and the E-OBS gridded data set. Validation indices describing relevant physical mechanisms are derived from the statistical models for observations and RCMs and are compared using pattern standard deviation, pattern correlation and centered pattern root mean squared error as validation measures. The results for the different RCMs and E-OBS are visualised using Taylor diagrams. We show that the RCMs adequately simulate moderately extreme precipitation and the influence of airflow strength and vorticity on precipitation extremes, but show deficits in representing the influence of airflow direction. Also very rare extremes are misrepresented, but this result is afflicted with a high uncertainty. E-OBS shows considerable biases, in particular in regions of sparse data. The proposed approach might be used to validate other physical relationships in regional as well as global climate models. 相似文献
74.
Summary Lovozero, the largest of the world’s layered peralkaline intrusions, includes gigantic deposits of Nb + REE-loparite ore.
Loparite, (Na,Ce,Ca)2(Ti,Nb)2O6, became a cumulus phase after crystallisation of about 35% of the ‘Differentiated Complex’, and its compositional evolution
has been investigated through a 2.35 km section of the intrusion. The composition of the cumulus loparite changes systematically
upwards through the intrusion with an increase in Na, Sr, Nb and Th and decrease in REE and Ti. This main trend of loparite
evolution records differentiation of the peralkaline magma through crystallisation of 1600 m of the intrusion. The formation
of the loparite ores was the result of several factors including the chemical evolution of the highly alkaline magma and mechanical
accumulation of loparite at the base of a convecting unit. At later stages of evolution, when concentrations of alkalis and
volatiles reached very high levels, loparite reacted with the residual melt to form a variety of minerals including barytolamprophyllite,
lomonosovite, steenstrupine-(Ce), vuonnemite, nordite, nenadkevichite, REE, Sr-rich apatite, vitusite-(Ce), mosandrite, monazite-(Ce),
cerite and Ba, Si-rich belovite. The absence of loparite ore in the “Eudialyte complex” is likely to be a result of the wide
crystallisation field of lamprophyllite, which here became a cumulus phase.
Received November 6, 2000; revised version accepted January 18, 2001 相似文献
75.
Saline water from a storm surge can flow down storm-damaged submerged water supply wells and contaminate boreholes and surrounding aquifers. Using data from conventional purging techniques, aquifer test response analysis, chemical analysis, and regression analysis of chloride/silica (Cl/Si) ratio, equations were derived to estimate the volume of saline water intrusion into a well and a porous media aquifer, the volume of water needed to purge a well shortly following an intrusion event, and the volume of water needed after delay of several or more months, when the saline plume has expanded. Purging time required is a function of volume of water and pumping rate. The study site well is located within a shoreline community of Lake Pontchartrain, St. Tammany Parish, in southeastern Louisiana, United States, which was impacted by two hurricane storm surges and had neither been rehabilitated nor chlorinated prior to our study. Chemical analysis of water samples in fall 2005 and purging of well and aquifer in June 6, 2006, indicated saline water had intruded the well in 2005 and the well and aquifer in 2006. The volume of water needed to purge the study well was approximately 200 casing volumes, which is significantly greater than conventionally used during collection of water samples for water quality analyses. 相似文献
76.
The spectacular fossils of the ‘water margin’: the Cambrian biota of Chengjiang,Yunnan, China
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Mark Williams David J. Siveter Derek J. Siveter Sarah E. Gabbott Xiaoya Ma Mark A. Purnell Peiyun Cong 《Geology Today》2016,32(6):233-237
Shi Nai'an's fourteenth century Chinese epic ‘Water Margin’ tells of the release of 36 heavenly spirits and 72 baleful stars from their captivity beneath a tablet of stone at Mount Longhu in Jiangxi Province. They are reincarnated as the 108 heroes of the Liangshan marsh in Shandong Province, who rise against an unjust world. The virtuous exploits of the ‘108’ were brought to life through the cathode‐ray screens of 1970s television sets, as the TV series The Water Margin introduced heroes like Lin Chong battling his evil nemesis Gao Qiu. Far to the west of Jiangxi Province and several hundred years after the Water Margin during the summer of 1984, a young scientist from Nanjing was working amongst the hills and lakes of southern Yunnan Province. He too overturned a stone slab, releasing from their half‐billion year captivity a cornucopia of new Chinese legends. His name was Xianguang Hou and he had made one of the most momentous fossil discoveries in history, uncovering the exceptionally preserved marine fossils of the Chengjiang biota from the ancient water margin of Cambrian seas. 相似文献
77.
Taus R. C. Jrgensen Douglas K. Tinkham C. Michael Lesher 《Journal of Metamorphic Geology》2019,37(2):271-313
Low‐pressure and high‐temperature (LP–HT) metamorphism of basaltic rocks, which occurs globally and throughout geological time, is rarely constrained by forward phase equilibrium modelling, yet such calculations provide valuable supplementary thermometric information and constraints on anatexis that are not possible to obtain from conventional thermometry. Metabasalts along the southern margin of the Sudbury Igneous Complex (SIC) record evidence of high‐grade contact metamorphism involving partial melting and melt segregation. Peak metamorphic temperatures reached at least ~925°C at ~1–3 kbar near the SIC contact. Preservation of the peak mineral assemblage indicates that most of the generated melt escaped from these rocks leaving a residuum characterized by a plagioclase–orthopyroxene–clinopyroxene–ilmenite‐magnetite±melt assemblage. Peak temperatures reached ~875°C up to 500 m from the SIC lower contact, which marks the transition to metabasalts that only experienced incipient partial melting without melt loss. Metabasalts ~500 to 750 m from the SIC contact are characterized by a similar two‐pyroxene mineral assemblage, but typically contain abundant hornblende that overgrew clino‐ and orthopyroxene along an isobaric cooling path. Metabasalts ~750 to 1,000 m from the SIC contact are characterized by a hornblende–plagioclase–quartz–ilmenite assemblage indicating temperatures up to ~680°C. Mass balance and phase equilibria calculations indicate that anatexis resulted in 10–20% melt generation in the inner ~500 m of the aureole, with even higher degrees of melting towards the contact. Comparison of multiple models, experiments, and natural samples indicates that modelling in the Na2O–CaO–FeO–MgO–Al2O3–SiO2–H2O–TiO2–O2 (NCFMASHTO) system results in the most reliable predictions for the temperature of the solidus. Incorporation of K2O in the most recent amphibole solution model now successfully predicts dehydration melting by the coexistence of high‐Ca amphibole and silicate melt at relatively low pressures (~1.5 kbar). However, inclusion of K2O as a system component results in prediction of the solidus at too low a temperature. Although there are discrepancies between modelling predictions and experimental results, this study demonstrates that the pseudosection approach to mafic rocks is an invaluable tool to constrain metamorphic processes at LP–HT conditions. 相似文献
78.
79.
Understory and small trees contribute importantly to stemflow of a lower montane cloud forest
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Teresa Margarita González‐Martínez Guadalupe Williams‐Linera Friso Holwerda 《水文研究》2017,31(5):1174-1183
Stemflow (Sf) measurements in tropical rain and montane forests dominated by large trees rarely include the understory and small trees. In this study, contributions of lower (1‐ to 2‐m height) and upper (>2‐m height and <5‐cm diameter at breast height [DBH]) woody understory, small trees (5 < DBH < 10 cm), and canopy trees (>10‐cm DBH) to Sf per unit ground area (Sfa) of a Mexican lower montane cloud forest were quantified for 32 days with rainfall (P) during the 2014 wet season. Rainfall, stemflow yield (Sfy), vegetation height, density, and basal area were measured. Subsequently, stemflow funneling ratios (SFRs) were calculated, and three common methods to scale up Sfy from individual trees to the stand level (tree‐Sfy correlation, P‐Sfy correlation, and mean‐Sfy extrapolation) were used to calculate Sfa. Understory woody plants, small trees, and upper canopy trees represented 96%, 2%, and 2%, respectively, of the total density. Upper canopy trees had the lowest SFRs (1.6 ± 0.5 Standard Error (SE) on average), although the lower understory had the highest (36.1 ± 6.4). Small trees and upper understory presented similar SFRs (22.9 ± 5.4 and 20.2 ± 3.9, respectively). Different Sf scaling methods generally yielded similar results. Overall Sfa during the study period was 22.7 mm (4.5% of rainfall), to which the understory contributed 70.1% (15.9 mm), small trees 10.6% (2.4 mm), and upper canopy trees 19.3% (4.4 mm). Our results strongly suggest that for humid tropical forests with dense understory of woody plants and small trees, Sf of these groups should be measured to avoid an underestimation of overall Sf at the stand level. 相似文献