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101.
Mary Anne Carroll Leroy E. Heidt Ralph J. Cicerone Ronald G. Prinn 《Journal of Atmospheric Chemistry》1986,4(3):375-395
The diurnal-to-monthly behavior of the fluxes of OCS, H2S, and CS2 from a mixed-Spartina grass-covered site in a Wallops Island salt water marsh was determined through a series of experiments in August and September, 1982. Absolute flux values were determined for OCS and H2S, while only relative values were determined for CS2. The rates of emission of OCS and H2S were observed to vary diurnally and to be strongly influenced by tides. The time-averaged flux values show that such mixed-Spartina stands are insignificant ( 1%) global sources of H2S or CS2 and insignificant contributors to the global OCS cycle (< 1%). These results demonstrate that some marsh regions play a minor role in the global sulfur budget and, consequently, that the inclusion of such areas in extrapolations of measurements of more productive regions could lead to an overestimate of the role of salt water marshes in the global sulfur budget. 相似文献
102.
Samantha Dow Noah P. Snyder William B. Ouimet Anna M. Martini Brian Yellen Jonathan D. Woodruff Robert M. Newton Dorothy J. Merritts Robert C. Walter 《地球表面变化过程与地形》2020,45(10):2380-2393
Centuries-long intensive land-use change in the north-eastern United States provides the opportunity to study the timescale of geomorphic response to anthropogenic disturbances. In this region, forest-clearing and agricultural practices following EuroAmerican settlement led to deposition of legacy sediment along valley bottoms, including behind mill dams. The South River in western Massachusetts experienced two generations of damming, beginning with mill dams up to 6-m high in the eighteenth–nineteenth century, and followed by construction of the Conway Electric Dam (CED), a 17-m-tall hydroelectric dam near the watershed outlet in 1906. We use the mercury (Hg) concentration in upstream deposits along the South River to constrain the magnitude, source, and timing of inputs to the CED impoundment. Based on cesium-137 (137Cs) chronology and results from a sediment mixing model, remobilized legacy sediment comprised % of the sediment load in the South River prior to 1954; thereafter, from 1954 to 1980s, erosion from glacial deposits likely dominated (63 ± 14%), but with legacy sediments still a substantial source (37 ± 14%). We also use the CED reservoir deposits to estimate sediment yield through time, and find it decreased after 1952. These results are consistent with high rates of mobilization of legacy sediment as historic dams breached in the early twentieth century, and suggest rapid initial response to channel incision, followed by a long decay in the second half of the century, that is likely dependent on large flood events to access legacy sediment stored in banks. Identifying sources of sediment in a watershed and quantifying erosion rates can help to guide river restoration practices. Our findings suggest a short fluvial recovery time from the eighteenth–nineteenth century to perturbation during the first half of the twentieth century, with subsequent return to a dominant long-term signal from erosion of glacial deposits, with anthropogenic sediment persisting as a secondary source. © 2020 John Wiley & Sons, Ltd. 相似文献
103.
Environmental parameters (salinity, sediment concentration, equilibration time) affecting radionuclide partitioning between sediment and seawater were experimentally investigated for Kara Sea sediments collected from nuclear waste dumping sites in Abrosimov and Stepovogo Bays off Novaya Zemlya. Adsorption kinetics were examined and the influence of salinity and sediment concentration were evaluated over the range of concentrations expected in the bays for the following radionuclides: 110 mAg; 241Am; 109Cd; 60Co; 57Co-cobalamine; 134Cs; 152Eu; 54Mn; 133Ba; 106Ru; and 85Sr. The major findings of this investigation are that 1. radionuclide distribution coefficients (Kds) were most sensitive to variations in sediment character (241Am, 60Co, 109Cd) and concentration (57Co-cobalamine, 85Sr, and 133Ba), 2. distribution coefficients generally decreased with increasing sediment concentration and 3. fast adsorption kinetics (near equilibrium ≈1 day) were observed only for 137Cs and 110 mAg. The observed differences in Kds for sediments from the two dumpsites exemplifies the importance of undertaking site-specific determinations of Kds. For purposes of confining radioactive wastes to the dumpsites in Stepovogo and Abrosimov Bays, the findings of this study indicate that based on sediment character alone, Stepovogo Bay will be more effective at retaining radionuclides than Abrosimov Bay. This is unfortunate since less radioactive waste resides in Stepovogo Bay (0.6 PBq) than in Abrosimov Bay (1.4 PBq). 相似文献
104.
Meltwater from snow that falls in the Catskill/Delaware watershed in the Catskill Mountains in south-central New York contributes to reservoirs that supply drinking water to approximately nine million people in and near New York City (NYC). Using the Interactive Multisensor Snow and Ice Mapping System (IMS) 4-km snow maps from the National Oceanic and Atmospheric Administration’s National Ice Center, we identified and tracked 28 lake-effect (LE) storms that deposited snow in the Catskills (2004–2017). These storms, which generally originated from Lake Ontario, but sometimes from Lake Erie, represent an underestimate of the number of LE storms that contribute snowfall to the Catskills snowpack because snowstorms are not visible on IMS maps when they travel over already-snow-covered terrain. Using satellite, meteorological (including NEXRAD and National Weather Service Cooperative Observer Program), and reanalysis data, we identified conditions that contributed to the LE snowstorms and mapped snow-cover extent (SCE) following the storms. We show that LE snow makes an important contribution to the Catskills snowpack because of the frequency of events, even though the total amount of each event may, on average, be small. The IMS 4-km maps tend to overestimate SCE compared to MODerate-resolution Imaging Spectroradiometer and Landsat snow maps. Climate change could impact LE storms and the distribution of rain versus snow in the Catskills, which may affect future reservoir operations in the NYC Water Supply System and winter recreation in the Catskills. 相似文献
105.
Lake basin response to tectonic drainage diversion: Eocene Green River Formation, Wyoming 总被引:1,自引:0,他引:1
A previously unidentified major sequence boundary within the Eocene Green River Formation separates fluctuating profundal facies of the Tipton Shale Member from evaporative facies of the Wilkins Peak Member. During deposition of the Tipton Shale Member, rivers entered the basin from the north, across the subdued Wind River Mountains, and deposited the southward prograding deltaic complex of the Farson Sandstone Member. Boulder-rich alluvial fan deposits overlie the Farson Sandstone adjacent to the Continental Fault, and correlate basinward to hypersaline lacustrine deposits of the Wilkins Peak Member. The alluvial fan deposits record a period of reverse motion on the Continental Fault and uplift of the southeastern Wind River Range, which diverted drainage away from the greater Green River Basin. This decreased inflow caused Lake Gosiute to shrink, exposing its bed to desiccation and erosion, and contributed to hydrologically-closed conditions and periodic evaporite deposition thereafter. This study is one of the first to demonstrate a direct relationship between movement along a specific basin-bounding structure, and a change in the overall style of lacustrine sedimentation. The identification of similar relationships elsewhere may challenge conventional interpretations of climate as the dominant factor influencing the character of lake deposits, and provide an important, but previously unexploited, approach to interpreting continental deformation and regional drainage organization. 相似文献
106.
The Aurelia Metamorphosis Test System was devised to use simple Aurelia polyps as indicator organisms for the detection of subtle effects of petroleum-related hydrocarbons and of Alaskan crude petroleum oil (ACPO) on developmental processes involved in strobilation initiation, differentiation of ephyrae, and genetic modification expressed through cloning. Compounds tested were ACPO, aniline, anthracene, benzanthracene, benzene, benzo[a]pyrene, biphenyl, cresol, naphthalene, perylene, phenol and pyrene. Gross morphology of the ephyrae (patterning, numbers and appearance of structures), statolith and mematocyst numbers, and pulsing behavior were recorded using the light microscope. Selected ephyrae with teratological malformations were studied with the scanning electron microscope and swimming behavior was observed visually. The variety of subtle developmental, behavioral and genetic effects due to marine hydrocarbons detected using the Aurelia Metamorphosis Test System demonstrated that this test system could be used as an early warning system to detect subtle effects of other marine pollutants. 相似文献
107.
Donald S. Burnett Amy J.G. Jurewicz Dorothy S. Woolum Jianhua Wang Julie M. Paque Larry R. Nittler Kevin D. McKeegan Munir Humayun Richard Hervig Veronika S. Heber Yunbin Guan 《Geostandards and Geoanalytical Research》2015,39(3):265-276
Ion microprobe elemental and isotopic determinations can be precise but difficult to quantify. Error is introduced when the reference material and the sample to be analysed have different compositions. Mitigation of such ‘matrix effects’ is possible using ion implants. If a compositionally homogeneous reference material is available which is ‘matrix‐appropriate’ (i.e., close in major element composition to the sample to be analysed, but having an unknown concentration of the element, E, to be determined) then ion implantation can be used to introduce a known amount of an E isotope, calibrating the E concentration and producing a matrix‐appropriate calibrator. Nominal implant fluences (ions cm?2) are inaccurate by amounts up to approximately 30%. However, ion implantation gives uniform fluences over large areas; thus, it is possible to ‘co‐implant’ an additional reference material of any bulk composition having known amounts of E, independently calibrating the implant fluence. Isotope ratio measurement standards can be produced by implanting two different isotopes, but permil level precision requires postimplant calibration of the implant isotopic ratio. Examples discussed include (a) standardising Li in melilite; (b) calibrating a 25Mg implant fluence using NIST SRM 617 glass and (c) using Si co‐implanted with 25Mg alongside NIST SRM 617 to produce a calibrated measurement of Mg in Si. 相似文献
108.
Late-type stars in general possess complicated magnetic surface fields which makes their detection and in particular their modeling and reconstruction challenging. In this work we present a new Zeeman-Doppler imaging code which is especially designed for the application to late-type stars. This code uses a new multi-line cross-correlation technique by means of a principal component analysis to extract and enhance the quality of individual polarized line profiles. It implements the full polarized radiative transfer equation and uses an inversion strategy that can incorporate prior knowledge based on solar analogies. Moreover, our code utilizes a new regularization scheme which is based on local maximum entropy to allow a more appropriate reproduction of complex surface fields as those expected for late-type stars. In a first application we present Zeeman-Doppler images of II Pegasi which reveal a surprisingly large scale surface structure with one predominant (unipolar) magnetic longitude which is mainly radially oriented. (© 2007 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim) 相似文献
109.
Angel A. Anaya Ingrid Padilla Raul Macchiavelli Dorothy J. Vesper John D. Meeker Akram N. Alshawabkeh 《Ground water》2014,52(4):584-596
Karst aquifers are highly productive groundwater systems often associated with conduit flow. These systems can be highly vulnerable to contamination, resulting in a high potential for contaminant exposure to humans and ecosystems. This work develops statistical models to spatially characterize flow and transport patterns in karstified limestone and determines the effect of aquifer flow rates on these patterns. A laboratory‐scale Geo‐HydroBed model is used to simulate flow and transport processes in a karstic limestone unit. The model consists of stainless steel tanks containing a karstified limestone block collected from a karst aquifer formation in northern Puerto Rico. Experimental work involves making a series of flow and tracer injections, while monitoring hydraulic and tracer response spatially and temporally. Statistical mixed models (SMMs) are applied to hydraulic data to determine likely pathways of preferential flow in the limestone units. The models indicate a highly heterogeneous system with dominant, flow‐dependent preferential flow regions. Results indicate that regions of preferential flow tend to expand at higher groundwater flow rates, suggesting a greater volume of the system being flushed by flowing water at higher rates. Spatial and temporal distribution of tracer concentrations indicates the presence of conduit‐like and diffuse flow transport in the system, supporting the notion of both combined transport mechanisms in the limestone unit. The temporal response of tracer concentrations at different locations in the model coincide with, and confirms the preferential flow distribution generated with the SMMs used in the study. 相似文献
110.
We have established a monitoring record of phosphate (PO43−) migration in the Long Point, ON campground septic system plume that now spans 26 years. Previously, at year 16 (2006), a P plume 16 m in length was documented and provided a good fit with an analytical advection dispersion model when a P migration velocity of 0.8 m/yr was used (retardation factor of 37) and when P behaved in an otherwise conservative manner (sorption only). However, between years 16 and 26 (2016), the P plume length expanded by only 2 m (0.2 m/yr) and increased in depth by only 0.5 m. The zone of abrupt P depletion at depth occurs close to the zone where SO42− concentrations increase in response to NO3− oxidation of pyrite. Scanning electron microscope images of sand grains from the nose of the P plume reveal abundant authigenic mineral coatings of considerable thickness (∼5 to 20 μm), with Fe as the dominant cation and containing 1 to 3 wt % P. This evidence suggests that P is now being attenuated along a reaction front that coincides with the zone where pyrite oxidation is occurring. P migration may now be controlled by the rate of migration of the pyrite oxidation front and this is several times slower than the previously indicated rate in the shallower, sorption-controlled portion of the plume. Monitoring at Long Point has demonstrated the danger of embracing an overly simplistic conceptual model when attempting to predict wastewater P migration in groundwater and also highlights the unique insight provided by a long-term monitoring record. 相似文献