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61.
Nicolas Seignez Arnaud Gauthier David Bulteel Denis Damidot Jean-Luc Potdevin 《Applied Geochemistry》2008,23(12):3699-3711
Lead metallurgical slags are partially vitrified materials containing residual amounts of Zn, Pb, Cr, Cd and As. These hazardous materials are generally buried on heaps exposed to weathering. In this study, leaching behavior of lead blast furnace slags has been tested using pure water and open flow experiments. It appears that in such far from equilibrium and slightly acidic conditions, the main phase to be altered is the vitreous phase. As for lunar, basaltic and nuclear glasses, alkalis/proton exchanges prevail and lead to the formation of a non-protective altered layer enriched in Si, Fe and Al. The composition of the altered layer is quite constant except for Si whose concentration decreases towards the leachate interface. Owing to their sizes, micrometric Pb droplets are not always totally dissolved at the slag surface. Nevertheless, nanometric Pb droplets are instantaneously dissolved while a surrounding altered layer is formed. This leads to high Pb releases in open flow systems. Leachate chemistry and dissolution rates of the vitreous phase are closely comparable to previous leaching tests with basaltic and nuclear glasses in conditions far from equilibrium. Moreover, this study confirms that Fe is a stable element in such conditions. 相似文献
62.
Rice is a major exposure route for arsenic in Chakdaha block,Nadia district,West Bengal,India: A probabilistic risk assessment 总被引:2,自引:0,他引:2
The importance or otherwise of rice as an exposure pathway for As ingestion by people living in Bengal and other areas impacted by hazardous As-bearing groundwaters is currently a matter of some debate. Here this issue is addressed by determining the overall increased cancer risk due to ingestion of rice in an As-impacted district of West Bengal. Human target cancer health risks have been estimated through the intake of As-bearing rice by using combined field, laboratory and computational methods. Monte Carlo simulations were run following fitting of model probability curves to measured distributions of (i) As concentration in rice and drinking water and (ii) inorganic As content of rice and fitting distributions to published data on (i) ingestion rates and (ii) body weight and point estimates on bioconcentration factors, exposure duration and other input variables. The distribution of As in drinking water was found to be substantially lower than that reported by previous authors for As in tube wells in the same area, indicating that the use of tube well water as a proxy for drinking water is likely to result in human health risks being somewhat overestimated. The calculated median increased lifetime cancer risk due to cooked rice intake was 7.62 × 10−4, higher than the 10−4–10−6 range typically used by the USEPA as a threshold to guide determination of regulatory values and similar to the equivalent risk from water intake. The median total risk from combined rice and water intake was 1.48 × 10−3. The contributions to this median risk from drinking water, rice and cooking of rice were found to be 48%, 44% and 8%, respectively. Thus, rice is a major potential source of As exposure in the As-affected study areas in West Bengal and the most important exposure pathway for groups exposed to low or no As in drinking water. 相似文献
63.
Estimation of Rn transfer from water to indoor air based on multi-day measurements may underestimate alpha exposure that occurs at short time scales in confined spaces, such as from showering, in houses with high Rn activities in the water supply. In order to examine one such incremental increase in exposure, variations in Rn in water and indoor air in 18 houses with private wells in western North Carolina (USA) were investigated. Radon in well water ranged from 158 to 811 Bq L−1 (median 239 Bq L−1). After 20-min showers in bathrooms with closed doors, peak Rn in air increases (above background) ranged from 71 to 4420 Bq m−3 (median 1170 Bq m−3). Calculated transfer coefficients at the scale of a 40-min closed bathroom (20-min shower plus 20 min post-shower) are described by a lognormal distribution whose geometric mean exceeds the widely-used ∼10−4 whole-house transfer coefficient by about one order of magnitude. As short-lived decay products grow from shower-derived Rn, short-term alpha energy exposure occurs in bathrooms in addition to the exposure caused by Rn mixed throughout the volume of the house. Due to the increasing ratio of Rn decay products to Rn, alpha energy exposure is greatest several minutes after the shower is turned off. For a 7.2-min shower with 10 min of additional exposure before opening the door, a geometric mean 5.6% increase in exposure over the ∼10−4 whole-house transfer coefficient derived from longer measurement periods was estimated. In addition to Rn activity in water, short-term shower exposure to Rn progeny depends on exposure time, ventilation, attachment and deposition, among other variable factors that characterize individual houses and residents. 相似文献
64.
The Simpevarp area is one of the alternative sites being considered for the deep geological disposal of high level radioactive waste in Sweden. In this paper, a coupled regional groundwater flow and reactive solute transport model of the Simpevarp area is presented that integrates current hydrogeological and hydrochemical data of the area. The model simulates the current hydrochemical pattern of the groundwater system in the area. To that aim, a conceptual hydrochemical model was developed in order to represent the dominant chemical processes. Groundwater flow conditions were reproduced by taking into account fluid-density-dependent groundwater flow and regional hydrogeologic boundary conditions. Reactive solute transport calculations were performed on the basis of the velocity field so obtained. The model was calibrated and sensitivity analyses were carried out in order to investigate the effects of heterogeneities of hydraulic conductivity in the subsurface medium. Results provided by the reactive transport model are in good agreement with much of the measured hydrochemical data. This paper emphasizes the appropriateness of the use of reactive solute transport models when water-rock interaction reactions are involved, and demonstrates what powerful tools they are for the interpretation of hydrogeological and hydrochemical data from site geological repository characterization programs, by providing a qualitative framework for data analysis and testing of conceptual assumptions in a process-oriented approach. 相似文献
65.
David P. Bacon Nash’at N. Ahmad Thomas J. Dunn Michael C. Monteith Ananthakrishna Sarma 《Natural Hazards》2008,44(3):317-327
By definition, a crisis is a situation that requires assistance to be managed. Hence, response to a crisis involves the merging
of local and non-local emergency response personnel. In this situation, it is critical that each participant: (1) know the
roles and responsibilities of each of the other participants; (2) know the capabilities of each of the participants; and (3)
have a common basis for action. For many types of natural disasters, this entails having a common operational picture of the unfolding events, including detailed information on the weather, both current and forecasted, that may impact on either
the emergency itself or on response activities. The Consequences Assessment Tool Set (CATS) is a comprehensive package of
hazard prediction models and casualty and damage assessment tools that provides a linkage between a modeled or observed effect
and the attendant consequences for populations, infrastructure, and resources, and, hence, provides the common operational
picture for emergency response. The Operational Multiscale Environment model with Grid Adaptivity (OMEGA) is an atmospheric
simulation system that links the latest methods in computational fluid dynamics and high-resolution gridding technologies
with numerical weather prediction to provide specific weather analysis and forecast capability that can be merged into the
geographic information system framework of CATS. This paper documents the problem of emergency response as an end-to-end system
and presents the integrated CATS–OMEGA system as a prototype of such a system that has been used successfully in a number
of different situations. 相似文献
66.
67.
David King 《Natural Hazards》2008,47(3):497-508
The concept of a natural hazard is a human construct. It is the interaction with human communities and settlements that defines
a natural phenomenon as a natural hazard. Thus the end point of hazard mitigation and hazard vulnerability assessment must
involve an attempt to reduce, or mitigate, the impact of the natural hazard on human communities. The responsibility to mitigate
hazard impact falls primarily upon governments and closely connected non-government and private institutional agencies. In
particular, it is most often local government that takes the responsibility for safeguarding its own communities, infrastructure
and people. Hazard vulnerability of specific local communities is best assessed by the local government or council, which
then faces the responsibility to translate that assessment into community education and infrastructural safeguards for hazard
mitigation. This paper illustrates the process of local government engagement in hazard mitigation in Australia, through the
Natural Disaster Risk Management Studies, as a first step towards natural disaster reduction. 相似文献
68.
Alessandro Tarantino Andrew M. Ridley David G. Toll 《Geotechnical and Geological Engineering》2008,26(6):751-782
This paper presents a review of techniques for field measurement of suction, water content, and water hydraulic conductivity
(permeability). Main problems in the use of field tensiometers are addressed and hints on how to improve tensiometer performance
are given. Advantages and limitations of instruments for indirect measurement of suction including electrical conductivity
sensors, thermal conductivity sensors, dielectric permittivity sensors, filter paper, and psychrometer are discussed. Techniques
for water content measurement based on dielectric methods are then presented. These include time and amplitude domain reflectometry
and capacitance. Finally, a brief overview of methods for measurement of water permeability in the field is presented. 相似文献
69.
70.
David Drew Houghton 《Meteorology and Atmospheric Physics》1962,12(4):407-425
Summary The large scale three-dimensional diabatic heating in the atmosphere is computed at 12 isentropic surfaces for a particular twelve hour time period. Using a method due toErtel, the continuity equation is combined with the equations of motion to give an explicit relation between diabatic heating and changes in potential vorticity and stability along isentropic surface trajectories. The results are barely of useful accuracy and reliability and this only under favorable conditions. The distribution of diabatic heating is qualitatively reasonable in the regions near the tropopause, close to the ground, above a cloud or moist layer, and within an area of general condensation. Errors and approximations make the computed values completely unreliable in areas of large anticyclonic vorticity or large baroclinity. Comparison of magnitudes with those computed from rainfall observations and with those measured directly at the earth's surface shows agreement in sign and within a factor of three in the areas of best data. The results emphasize that there are regions and periods where diabatic heating in the free atmosphere may be important in controlling atmospheric behavior. Sample calculations in one of these regions using values of diabatic heating computed by this study illustrate that this process is of comparable importance with the adiabatic process in determining vertical velocity.
With 7 Figures 相似文献
Zusammenfassung Die großräumige nichtadiabatische Erwärmung der Atmosphäre in 12 isentropen Flächen während eines 12stündigen Zeitabschnittes wird berechnet. Unter Verwendung einer Methode vonErtel liefert eine Kombination der Kontinuitätsgleichung mit den Bewegungsgleichungen eine explizite Beziehung zwischen der nichtadiabatischen Erwärmung, der potentiellen Vorticity und der Stabilität entlang der isentropen Trajektorien. Das Resultat ist von beschränkter Genauigkeit — und auch dies nur unter günstigen Bedingungen. Qualitativ brauchbare Verteilungen der nichtadiabatischen Erwärmung erhält man nahe der Tropopause, in Bodennähe, über einer Schicht von Wolken oder feuchter Luft und innerhalb der Zonen mit verbreiteter Kondensation. In Gebieten mit großer antizyklonaler Vorticity oder großer Baroklinität werden die berechneten Werte infolge von Meß- und Approximationsfehlern völlig ungenau. In den Gebieten mit optimalen Voraussetzungen stimmen die berechneten Werte mit den aus Niederschlagsmessungen abgeleiteten oder am Boden direkt beobachteten im Vorzeichen und innerhalb eines Faktors von 3 überein. Die Ergebnisse der vorliegenden Untersuchung weisen erneut darauf hin, daß in manchen Gebieten bzw. Zeitabschnitten das Verhalten der freien Atmosphäre durch nichtadiabatische Erwärmung wesentlich beeinflußt sein kann. Stichprobenweise Berechnungen für eines dieser Gebiete zeigen, daß die theoretisch ermittelte nichtadiabatische Erwärmung für die resultierende Vertikalgeschwindigkeit der Luft quantitativ von ähnlicher Bedeutung ist wie der adiabatische Prozeß.
Résumé L'auteur a calculé le réchauffement non adiabatique, à grande échelle, de l'atmosphère à 12 niveaux isentropes pendant un intervalle de 12 heures. Une méthode établie parErtel combine l'équation de continuité et les équations de mouvement et aboutit à une relation explicite entre le réchauffement non adiabatique, la vorticity potentielle et la stabilité le long de trajectoires isentropes. Le résultat n'a qu'une exactitude approchée, et cela dans des conditions favorables seulement. On obtient une répartition utilisable du réchauffement non adiabatique au voisinage de la tropopause, du sol, au-dessus d'une couche de nuages ou d'air humide, ainsi qu'à l'intérieur des zones à forte condensation. Dans les régions à grande vorticity anticyclonique et à grande baroclinité, les valeurs calculées deviennent tout à fait inexactes par suite d'une approximation insuffisante et d'erreurs de mesure. Dans les régions à conditions favorables par contre, les valeurs calculées correspondent à celles que l'on peut tirer de la mesure des précipitations ou de celles que l'on mesure au sol, cela au signe et à un facteur 3 près. Le résultat de cette étude montre à nouveau que dans certaines régions ou certains laps de temps l'état de l'atmosphère peut être notablement conditionné par un réchauffement non adiabatique. Des épreuves faites pour l'une de ces régions montrent que le réchauffement non adiabatique obtenu par calcul est quantitativement aussi important pour la vitesse verticale résultante de l'air que le processus adiabatique.
With 7 Figures 相似文献