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Spatial character of the gaseous and particulate state compound correlation of urban atmospheric pollution in winter and summer 总被引:1,自引:0,他引:1
XU Xiangde SHI Xiaohui XIE Lian DING Guoan MIAO Qiuju MA Jianzhong ZHENG Xiangdong 《中国科学D辑(英文版)》2005,48(Z2)
The spatial/temporal variation information of atmospheric dynamic-chemical processes at observation site points of the "canopy" boundary of Beijing urban building ensemble and over urban area "surface", as well as the seasonal correlation structure of the gaseous and particulate states of urban atmospheric pollution (UAP) and its seasonal conversion feature at observation points are investigated, using the comprehensive observation data of the Beijing City Air Pollution Observation Experiment (BECAPEX) in winter and summer 2003 with a "point-surface" combined research approach. By using "one dimension spatial empirical orthogonal function (EOF)" principal component analysis (PCA) mode, the seasonal change of gaseous and particulate states of atmospheric aerosols and the association feature of pollutant species under the background of the complicated structure of urban boundary layer (UBL) are analyzed. The comprehensive analyses of the principal components of particle concentrations,gaseous pollutant species, and meteorological conditions reveal the seasonal changes of the complex constituent and structure features of the gaseous and particulate states of UAP to further trace the impact feature of urban aerosol pollution surface sources and the seasonal difference of the component structure of UAP. Research results suggest that in the temporal evolution of the gaseous and particulate states of winter/summer UAP, NOx, CO, and SO2 showed an "in-phase" evolution feature, however, O3 showed an "inverse-phase" relation with other species,all possessing distinctive dependent feature. On the whole, summer concentrations of gaseous pollutants CO, SO2, and NOx were obviously lower than winter ones, especially, the reduction in CO concentration was most distinctive, and ones in SO2 and NOx were next. However, the summer O3 concentration was more than twice winter one. Winter/summer differences in PM10and PM2.5 particle concentrations were relatively not obvious, which indicates that responses of PM10 and PM2.5 particle concentrations to the difference of winter/summer heating period emission sources are far less distinctive than those of NOx, SO2, and CO. The correlation feature of winter/summer gaseous and particulate states depicts that both PM10 and PM2.5 particles were significantly correlated with NOx, and their correlations with NOx are more significant than those with other pollutants. Through PCA, it is found that there was a distinctive difference in the principal component combination structure of winter/summer PM10 and PM2.5 particles: SO2 and NOx dominated in the principal component of winter PM10 and PM2.5 particles; while CO and NOx played the major role in the principal component of summer PM10 and PM2.5 particles. For winter/summer PM10 and PM2.5 particles, there might exist the gaseous and particulate states correlation structures of different "combinations" of such dependent pollutant species. Research results also uncover that the interaction processes of gaseous and particulate states were also related with the vertical structure of UBL, that is to say, the low value layer of UBL O3 concentration was associated with the collocation of atmospheric vertical structures of the low level inversion,inverse humidity, and small wind, which depicts summer boundary layer atmospheric character, i.e.the compound impact of the dependent factor "combination" of wind, temperature, and humidity elements and their collocation structure on the variations of different gaseous pollutant concentrations. Such a depth structure of the extremely low value of O3 concentration in the UBL accords with its "inverse-phase" relation with other gaseous pollutant species. The PCA of meteorological factors associated with PM10 and PM2.5 concentrations also reveals the sensitivity of PM10 and PM2.5 concentration to the combinatory feature of local meteorological conditions. 相似文献
114.
XU Jianming XU Xiangde LIU Yu DING Guoan CHEN Huailiang HU Jiangkai ZHANG Jianchun WU Hao LI Weiliang HE Jinhai YANG Yuanqin WANG Jiahe 《中国科学D辑(英文版)》2005,48(Z2)
Based on analysis of the air pollution observational data at 8 observation sites in Beijing including outer suburbs during the period from September 2004 to March 2005, this paper reveals synchronal and in-phase characteristics in the spatial and temporal variation of air pollutants on a city-proper scale at deferent sites; describes seasonal differences of the pollutant emission influence between the heating and non-heating periods, also significantly local differences of the pollutant emission influence between the urban district and outer suburbs, i.e. the spatial and temporal distribution of air pollutant is closely related with that of the pollutant emission intensity. This study shows that due to complexity of the spatial and temporal distribution of pollution emission sources, the new generation Community Multi-scale Air Quality (CMAQ) model developed by the EPA of USA produced forecasts, as other models did, with a systematic error of significantly lower than observations, albeit the model has better capability than previous models had in predicting the spatial distribution and variation tendency of multi-sort pollutants. The reason might be that the CMAQ adopts average amount of pollutant emission inventory, so that the model is difficult to objectively and finely describe the distribution and variation of pollution emission sources intensity on different spatial and temporal scales in the areas, in which the pollution is to be forecast. In order to correct the systematic prediction error resulting from the average pollutant emission inventory in CMAQ, this study proposes a new way of combining dynamics and statistics and establishes a statistically correcting model CMAQ-MOS for forecasts of regional air quality by utilizing the relationship of CMAQ outputs with corresponding observations, and tests the forecast capability. The investigation of experiments presents that CMAQ-MOS reduces the systematic errors of CMAQ because of the uncertainty of pollution emission inventory and improves the forecast level of air quality. Also this work employed a way of combining point and area forecasting, i.e. taking the products of CMAQ for a center site to forecast air pollution for other sites in vicinity with the scheme of model products "reanalysis" and average over the "area". 相似文献
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116.
Numerical Modeling of Basin-Range Tectonics Related to Continent-Continent Collision 总被引:1,自引:0,他引:1
CUI Junwen SHI Jinsong LI Pengwu ZHANG Xiaowei GUO Xianpu DING Xiaozhong Institute of Geology Chinese Academy of Geological Sciences Beijing Hehai University Nanjing Jiangsu 《《地质学报》英文版》2005,79(1):24-35
Continent-continent collision is the most important driving mechanism for the occurrence of various geological processes in the continental lithosphere. How to recognize and determine continent-continent collision,especially its four-dimensional temporal-spatial evolution, is a subject that geological communities have long been concerned about and studied. Continent-continent collision is mainly manifested by strong underthrnsting (subduction) of the underlying block along an intracontinental subduction zone and continuous obduction (thrusting propagation) of the overlying block along the intracontinental subduction zone, the occurrence of a basin-range tectonic framework in a direction perpendicular to the subduction zone and the flexure and disruption of the Moho. On the basis of numerical modeling, the authors discuss in detail the couplings between various amounts and rates of displacement caused by basin subsidence, mountain uplift and Moho updoming and downflexure during obduction (thrusting propagation) and subduction and the migration pattern of basin centers. They are probably indications or criteria for judgment or determination of continent-continent collision. 相似文献
117.
The aim of this paper is to investigate the feasibility of using Landsat TM data to retrieve leaf area index (LAI). To get a LAI retrieval model based ground reflectance and vegetation index, detailed field data were collected in the study area of eastern China, dominated by bamboo, tea plant and greengage. Plant canopy reflectance of Landsat TM wavelength bands has been inversed using software of 6S. LAI is an important ecological parameter. In this paper, atmospheric corrected Landsat TM imagery was utilized to calculate different vegetation indices (VI), such as simple ratio vegetation index (SR), shortwave infrared modified simple ratio (MSR), and normalized difference vegetation index (NDVI). Data of 53 samples of LAI were measured by LAI-2000 (LI-COR) in the study area. LAI was modeled based on different reflectances of bands and different vegetation indices from Landsat TM and LAI samples data. There are certainly correlations between LAI and the reflectance of Tm3, TM4, TM5 and TM7. The best model through analyzing the results is LAI = 1.2097*MSR + 0.4741 using the method of regression analysis. The result shows that the correlation coefficient R2 is 0.5157, and average accuracy is 85.75%. However, whether the model of this paper is suitable for application in subtropics needs to be verified in the future. 相似文献
118.
Sedimentation rates in the Wanggang salt marshes, Jiangsu 总被引:1,自引:0,他引:1
WANGAijun GAOShu JIAJianjun PANShaoming 《地理学报(英文版)》2005,15(2):199-209
1 IntroductionLand-ocean interaction in coastalzone is one of the key m atters of the International G eosphereand Biosphere Program (IG BP). The key problem s of the second phase in the next decadeinclude the m aterial cycle, the system evolution process … 相似文献
119.
Element mobility during pyrite weathering: implications for acid and heavy metal pollution at mining-impacted sites 总被引:1,自引:0,他引:1
Long Lu Rucheng Wang Fanrong Chen Jiyue Xue Peihua Zhang Jianjun Lu 《Environmental Geology》2005,49(1):82-89
Based on back scattered electron images and electron micro-probe analysis results, four alteration layers, including a transition layer, a reticulated ferric oxide layer, a nubby ferric oxide layer and a cellular ferric oxide layer, were identified in the naturally weathering products of pyrite. These layers represent a progressive alteration sequence of pyrite under weathering conditions. The cellular ferric oxide layer correlates with the strongest weathering phase and results from the dissolution of nubby ferric oxide by acidic porewater. Leaching coefficient was introduced to better express the response of element mobility to the degree of pyrite weathering. Its variation shows that the mobility of S, Co and Bi is stronger than As, Cu and Zn. Sulfur in pyrite is oxidized to sulfuric acid and sulfate that are basically released into to porewater, and heavy metals Co and Bi are evidently released by acid dissolution. As, Cu and Zn are enriched in ferric oxide by adsorption and by co-precipitation, but they would re-release to the environment via desorption or dissolution when porewater pH becomes low enough. Consequently, Co, Bi, As, Cu and Zn may pose a substantial impact on water quality. Considering that metal mobility and its concentration in mine waste are two important factors influencing heavy metal pollution at mining-impacted sites, Bi and Co are more important pollutants in this case. 相似文献
120.
江苏王港盐沼的现代沉积速率 总被引:35,自引:0,他引:35
江苏海岸湿地总面积超过5000km^2,但围垦活动的加剧使盐沼湿地面积迅速减少;为了达到海岸防护、保滩促淤的目的,先后引种了大米草和互花米草。通过采集江苏王港潮滩盐沼湿地9处柱状样和挖取探槽剖面,以及对沉积剖面样品进行^210Pb和^137Cs测年分析,探讨了^210Pb的本底及影响^210Pb富集的因素,估算了王港盐沼湿地的现代沉积速率。王港潮滩盐沼沉积物对^210Pb的吸附作用较弱;受风暴潮、生物扰动、物源变化及实验误差等因素的影响,在^210Pbex剖面上出现了数据异常点,将这些数据点剔除后计算得到的沉积速率为33cm yr^-1,^137Cs测年显示,该地区1963年以来的平均沉积速率3.1cm yr^-1,与^210Pb法及前人研究结果相一致。根据一个典型剖面的^137Cs测年数据分析,王港潮滩盐沼的沉积过程根据地貌特征的不同可分3个阶段,大米草覆盖阶段滩面高程迅速增加,互花米草的生长提高了滩面淤积速率。 相似文献