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61.
The main purpose of this study is to model the δ13C values of methane derived from coal by combining kinetic-simulating experiment with the gas chromatography-isotope ratio mass spectrum (GC-IRMS) analysis. The stable carbon isotopic variation of methane in pyrolysates with heating temperature indicates that the assumptions for both a constant kinetic isotope effect (α) and a uniform initial isotopic composition (δ13Co) are impractical for explaining the carbon isotopic fractionation during coalification. For purposes of simplification, two approaches are used in this paper to deal with the heterogeneity of terrestrial organic matter. One is that, assuming a uniform initial isotopic composition (i.e., δ13Ci, o=δ13Co) for all methane-generating precursors in coal, the isotopic variation of methane is fitted by adjusting ΔEa, i (Ea13C, i−Ea12C, i) for each hypothetical reaction. The other is that, assuming a constant kinetic isotope effect during the whole gas formation, that is all ΔEa, i values are identical, the modeling of methane isotopic composition is achieved by changing the 13CH4 generation potential of each reaction (fi, 13C), namely, by adjusting the initial δ13C value (δ13Ci, o) for each methane-generating precursor. Results of the kinetic calculation shows that the two simulating methods can yield a similar result at a geological heating rate of 2 °C/My, which further demonstrates that those natural gases with methane δ13C value being approximately −36‰ are possibly sourced from the upper Triassic coal measure strata in the Northwestern Sichuan Basin. 相似文献
62.
The Indo–Asian continental collision is known to have had a great impact on crustal deformation in south-central Asia, but its effects on the sublithospheric mantle remain uncertain. Studies of seismic anisotropy and volcanism have suggested that the collision may have driven significant lateral mantle flow under the Asian continent, similar to the observed lateral extrusion of Asian crustal blocks. Here we present supporting evidence from P-wave travel time seismic tomography and numerical modeling. The tomography shows continuous low-velocity asthenospheric mantle structures extending from the Tibetan plateau to eastern China, consistent with the notion of a collision-driven lateral mantle extrusion. Numerical simulations suggest that, at the presence of a low-viscosity asthenosphere, continued mass injection under the Indo–Asian collision zone over the past 50 My could have driven significant lateral extrusion of the asthenospheric mantle, leading to diffuse asthenospheric upwelling, rifting, and widespread Cenozoic volcanism in eastern China. 相似文献
63.
Yuhong Liao Ansong Geng Yongqiang Xiong Dehan Liu Jialan Lu Jinzhong Liu Haizu Zhang Xinhua Geng 《Organic Geochemistry》2004,35(11-12):1479
Expulsion of petroleum from source rock is a complex part of the entire migration process. There exist fractional effects on chemical compositions in hydrocarbon expulsion. Does the carbon isotopic fractionation occur during expulsion and to what extent? Here the influence of hydrocarbon expulsion on carbon isotopic compositions of individual n-alkanes from pyrolysates of selected terrestrial kerogens from Tuha basin and Fushun, Liaoning Province of China has been experimentally studied. The pyrogeneration-expulsion experiments were carried out under semi-closed system. The carbon isotopic compositions of individual n-alkanes were measured by GC-IRMS. The main conclusions are as follows. First, there is carbon isotopic fractionation associated with hydrocarbon expulsion from Type III kerogens in Tuha Basin. There exist differences of carbon isotopic compositions between the unexpelled n-alkanes and expelled n-alkanes from Tuha desmocollinite and Tuha mudstone. Second, there is almost no carbon isotopic fractionation associated with hydrocarbon expulsion from Type II kerogens in Fushun and Liaohe Basin. Third, carbon isotopic fractionation in hydrocarbon expulsion should be considered in making oil-source correlation of Type III kerogens at least in the Tuha Basin. Further studies need to be carried out to determine whether this is true in other basins. Fourth, oil and source at different maturity levels cannot be correlated directly for Type III kerogens since the carbon isotopic compositions of expelled hydrocarbons at different temperatures are different. The expelled hydrocarbons are usually lighter (depleted in 13C) than the hydrocarbons remaining in the source rock at the same maturity. 相似文献
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LIU Jihua SHI Xuefa Chen Lirong HUANG Yongyang Wang Yinxi Cui Yingchun BU Wenrui 《中国科学D辑(英文版)》2005,48(5)
Clay fractions in the non-calcareous surface sediments from the eastern Pacific were analyzed for clay minerals, REE and 143Nd/144Nd. Montmorillonite/illite ratio (M/I ratio), total REE contents ((REE), LREE/HREE ratio and cerium anomaly (бCe) may effectively indicate the genesis of clay minerals. Clay fractions with M/I ratio >1, бCe (0.85, (REE (400 μg/g, LREE/HREE ratio (4, and REE patterns similar to those of pelagic sediments are terrigenous and autogenetic mixed clay fractions and contain more autogenetic montmorillonite. Clay fractions with M/I ratio <1, бCe=0.86 to 1.5, ΣREE=200 to 350 μg/g, LREE/HREE ratio (6 and REE distribution patterns similar to that of China loess are identified as terrigenous clay fraction. The 143Nd/144Nd ratios or (э)Nd values of clay fractions inherit the features of terrigenous sources of clay minerals. Clay fractions are divided into 4 types according to (э)Nd values. Terrigenous clay minerals of type I with the (э)Nd values of -8 to -6 originate mainly from North American fluvial deposits. Those of type II with the (э)Nd values of -9 to -7 are mainly from the East Asia and North American fluvial deposits. Those of type III with (э)Nd values of -6 to -3 could come from the central and eastern Pacific volcanic islands. Those of type IV with (э)Nd values of -13 to -12 may be from East Asia eolian. The terrigenous and autogenetic mixed clay fractions show patchy distributions, indicating that there are volcanic or hot-spot activities in the eastern Pacific plate, while the terrigenous clay fractions cover a large part of the study area, proving that the terrigenous clay minerals are dominant in the eastern Pacific. 相似文献
67.
云南东北部拱王山末次冰期 总被引:1,自引:0,他引:1
1 Introduction The Gongwang mountains constitute one of the few high m ountains of irrefutable late Pleistocene glaciation in eastern China. This area is one of the m ost extensively studied Quaternary geologicallocationsin eastern China and the interpret… 相似文献
68.
Assessment of flow paths and confluences for saltwater intrusion in a deltaic river network 下载免费PDF全文
Saltwater intrusion is a serious issue in estuarine deltas all over the world due to rapid urban sprawl and water shortage. Therefore, detecting the major flow paths or locations at risk of saltwater intrusion in estuarine ecosystems is important for mitigating saltwater intrusion. In this paper, we introduce a centrality index, the betweenness centrality (BC), to address this problem. Using the BC as the weighted attribute of the river network, we identify the critical confluences for saltwater intrusion and detect the preferential flow paths for saltwater intrusion through the least‐cost‐path algorithm from a graph theory approach. Moreover, we analyse the responses of the BC values of confluences calculated in the river network to salinity. Our results show that the major flow paths and critical confluences for saltwater intrusion in a deltaic river network can be represented by the least cost paths and the BC values of confluences, respectively. In addition, a significant positive correlation between the BC values of confluences and salinity is determined in the Pearl River Delta. Changes in the salinity can produce significant variation in the BC values of confluences. Therefore, freshwater can be diverted into these major flow paths and critical confluences to improve river network management under saltwater intrusion. Copyright © 2015 John Wiley & Sons, Ltd. 相似文献
69.
New magnetostratigraphic and pedostratigraphic investigations of loess deposits in north‐east China and their implications for regional environmental change during the Mid‐Pleistocene climatic transition 下载免费PDF全文
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