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71.
The role of pollution versus natural geological sources for lead enrichment in recent lake sediments and surface forest soils 总被引:3,自引:0,他引:3
M.-L. Brännvall H. Kurkkio R. Bindler O. Emteryd I. Renberg 《Environmental Geology》2001,40(9):1057-1065
This paper assesses the role of airborne pollution and natural geological sources for lead enrichment in lake sediments and in surface soils of boreal forests. This assessment is based on analyses of stable lead isotopes (206Pb and 207Pb) and lead concentrations in sediment cores (>30 lakes), ombrotrophic peat and soil samples in Sweden. The 206Pb/207Pb ratio and concentration profiles in the sediment cores change synchronously over the last 3,000 years in different lakes, temporal concentration changes in sediments and peat deposits are very consistent, and these temporal concentration changes coincide well with the history of lead production in Europe. The 206Pb/207Pb ratio is almost the same in all soil mor samples (1.152ǂ.009; n=94), and similar to values recorded in aerosols, despite very high and different 206Pb/207Pb ratio of the mineral soil in the C-horizon (1.3-1.7). This study provides evidence that lead enrichment in recent sediments and peat, and in the mor layer are caused by deposition of pollution lead and not natural processes. 相似文献
72.
D. W. Arlander D. Brüning U. Schmidt D. H. Ehhalt 《Journal of Atmospheric Chemistry》1995,22(3):243-249
A series of 72 measurements of the acetaldehyde (CH3CHO) mixing ratio were made in the lower troposphere during TROPOZ II. These measurements are the first ever made of the background level of this trace gas in the free troposphere. The data show a vertical decrease of the CH3CHO mixing ratio with increasing altitude and indicate higher CH3CHO concentrations in the Northern Hemisphere — in general agreement with a model-derived average CH3CHO distribution. Deviations of the observed CH3CHO mixing ratios from the modelled mean distribution are correlated with similar deviations in the corresponding HCHO mixing ratios. 相似文献
73.
R. Heino R. Brázdil E. Førland H. Tuomenvirta H. Alexandersson M. Beniston C. Pfister M. Rebetez G. Rosenhagen S. Rösner J. Wibig 《Climatic change》1999,42(1):151-181
A study of the long-term changes of various climatic extremes was made jointly by a number of European countries. It was found that the changes in maximum and minimum temperatures follow, in broad terms, the corresponding well-documented mean temperature changes. Minimum temperatures, however, have increased slightly more than maximum temperatures, although both have increased. As a result, the study confirms that the diurnal temperature range has mostly decreased during the present century in Northern and Central Europe. Frost has become less frequent. Two extreme-related precipitation characteristics, the annual maximum daily precipitation and the number of days with precipitation 10 mm, show no major trends or changes in their interannual variability. An analysis of return periods indicated that in the Nordic countries there were high frequencies of extraordinary 1-day rainfalls both in the 1930s and since the 1980s. There have been no long-term changes in the number of high wind speeds in the German Bight. Occurrences of thunderstorms and hails show a decreasing tendency in the Czech Republic during the last 50 years. Finally, using proxy data sources, a 500-year temperature and precipitation event graph for the Swiss Mittelland is presented. It shows large interdecadal variations as well as the exceptionality of the latest decade 1986-1995. 相似文献
74.
Summary A strategy was developed to overcome the difficulty of unknown forcing for the modelling of fields of wind roses with meso- and microscale models. It was applied to a site with heavy orographically structured terrain. The supra-scale winds which act as forcing for the model were calculated from a measured distribution of surface winds by an optimized inversion technique. The method is applicable to all types of mesoscale models.With 3 Figures 相似文献
75.
Burghard Brümmer Birgit Busack Heinrich Hoeber Gottfried Kruspe 《Boundary-Layer Meteorology》1994,68(1-2):75-108
Observations made on 8 and 9 May 1988 by aircraft and two ships in and around the marginal ice zone of the Fram Strait during on-ice air flow under cloudy and cloud-free conditions are presented.The thermodynamic modification of the air mass moving from the open water to the ice over horizontal distances of 100–300 km is only a few tenth of a degree for temperature and a few tenth of a gram per kilogram for specific humidity. This is due to the small temperature differences between sea and ice surfaces. During the day, the ice surface is even warmer than the sea surface. The stably stratified 200–400 m deep boundary layer is often topped by a moisture inversion leading to downward fluxes of sensible as well as latent heat.The radiation and energy balance at the surface are measured as functions of ice cover, cloud cover and sun elevation angle. The net radiationR
Nis the dominating term of the energy budget. During the day, the difference ofR
Nbetween clear and overcast sky is only a few W/m2 over ice, but 100–200 W/m2 over water. During the night,R
Nover ice is more sensitive to cloud cover.The kinematic structure is characterized by strong shears of the longitudinal and the transversal wind component. The profile of the latter one shows an inflection point near the top of the boundary layer. Dynamically-driven roll circulations are numerically separated from the mean flow. The secondary flow patterns have wavelengths of about 1 km and contribute substantially to the total variances and covariances. 相似文献
76.
Dendrochronology for the last 1400 years in eastern Tibet 总被引:11,自引:0,他引:11
Achim Bräuning 《GeoJournal》1994,34(1):75-95
Twentyfour tree-ring chronologies of various tree-species(Picea, Abies, Larix, Juniperus) from sites near the upper timberline in eastern Tibet were established, the longest one dating back to 620 A.D. A new classification of pointer intervals is presented, distinguishing between different kinds of signatures in a tree-ring series and amount of growth change in relation to the previous year. The various types of signatures can be related to meteorological events like cold winters and summers, summer drought or to recreation reactions after years of reduced growth. The distribution pattern and type of pointer intervals combined with ring width variation enables the detection of periods of favourable or unfavourable growth conditions with regard to climate history. Based on far-distance correlations and signature analysis regions of similar tree-growth are mapped out. 相似文献
77.
B. Wyncke P. F. McMillan W. L. Brown R. E. Openshaw F. Bréhat 《Physics and Chemistry of Minerals》1981,7(1):31-34
The far infrared powder absorption spectra (10–200 cm?1) for a maximum microcline sample (obtained by ion-exchange from Amelia albite) and for a natural maximum microcline were measured at steps of 10 K on lowering and raising the temperature between 300 and 110 K. Of the absorption bands at 97.5, 113.5, 137.5, 148, and 157 cm?1 occurring at room temperature, those at 157 and eventually 148 cm?1 showed evidence of a phase transition and only that at 157 cm?1 showed hysteresis. The transition occurs at 245±5 K on lowering the temperature and the low-temperature form can be superheated to 300 K in the case of the ion-exchange sample. Oriented thin sections parallel to (001) and (010) were also measured to 110 K as a function of the direction of the electric vector E, but could not be unambiguously interpreted. Though the effect is very slight it is tentatively proposed that the phase transition (already characterized by calorimetry and lattice parameters) involves changes in K-O and T-O-T bonds. 相似文献
78.
79.
80.
Characterization of sediments in an abandoned mining area; a case study of Mansfeld region,Germany 总被引:1,自引:0,他引:1
Rainer?WennrichEmail author Jürgen?Mattusch Peter?Morgenstern Klaus?Freyer Hanns-Christian?Treutler Hans-Joachim?St?rk Lutz?Brüggemann Albrecht?Paschke Birgit?Daus Holger?Weiss 《Environmental Geology》2004,45(6):818-833
The distribution of selected heavy metals, including some radionuclides, metalloids and non-metals was determined in stream sediments in a region influenced by abandoned copper mining and ore processing activities. A considerable amount of the ore processing waste with a very complex composition and highly elevated concentrations of zinc, sulfur, lead, copper, arsenic, and a lot of other elements in the range between 100 and 1,000 mg/kg (Sb, Mn, Ni, Cr, Cd, Hg, and Ag) was piled up on mine dumps. The dispersion of the pollutants originating from this source and their environmental impact were investigated. Both, sediments and original waste material were studied to indicate the pathways and the mobilization behavior of different pollutants. For this purpose, the process of the elution of pollutants by application of different fractionation schemes was studied. The capabilities of different analytical techniques are shown for the analysis of solid samples (X-ray fluorescence spectrometry, Gamma-spectrometry) and liquid ones (ICP-atomic emission spectrometry, ICP-mass spectrometry and different techniques of atomic absorption). Additionally, the coupling of ion chromatography and ICP-MS detection was used to study the distribution of arsenic species in the sediment cores of a lake which acts as a natural sink for the region. 相似文献