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41.
42.
The data deduced from the UV-spectroscope on theCopernicus satellite strongly suggest that the most important ionization source in interstellar space near the solar system is a UV radiation field originating from B-stars. Adopting this hypothesis, we have used the ionization state of several elements in the interstellar medium observed byCopernicus to determine the required radiation field. From this, the degree of ionization of elements that could not be observed byCopernicus is estimated.It is shown that this interpretation of thecopernicus data can be made consistent with neutral interstellar hydrogen densities inferred from extraterrestrial L observations and with electron densities deduced from pulsar dispersion measures. Furthermore, it is shown that the ratio of neutral interstellar helium to neutral interstellar hydrogen is likely to be 2 to 3 times as large as the cosmic abundance ratio of these elements. The possibility that this ratio is about 10 times as large, meaning equal interstellar neutral hydrogen and helium densities near the solar system, cannot be ruled out. It would, however, require an interstellar radiation temperature near 9000 K. A comparison of the intensity of the interplanetary back scattered He 584 Å and the H 1216 Å radiation would lead to a direct determination of this ratio provided the solar radiation at these lines is known. 相似文献
43.
Jason L. Blum Iris Knoebl Patrick Larkin Kevin J. Kroll Nancy D. Denslow 《Marine environmental research》2004,58(2-5):565
In this study male largemouth bass (LMB) were exposed to the naturally occurring androgens, dihydrotestosterone (DHT) or 11-ketotestosterone (11-KT) in order to identify genes that are differentially regulated by these steroid hormones. Using subtractive hybridization on livers of fish treated with DHT against vehicle control, many novel LMB genes were cloned. These genes were added to our gene library and arrayed. Six genes were up-regulated and five were down-regulated by both androgens. But, each androgen also regulated specific genes. One gene that was identified as a potential androgen marker was spermidine-spermine-N1-acetyltransferase that was up-regulated by both androgens. Determining which genes are responsive to natural androgens will help to identify biochemical pathways that are impacted. 相似文献
44.
Farhana Huq Philipp Blum Michael A. W. Marks Marcus Nowak Stefan B. Haderlein Peter Grathwohl 《Environmental Earth Sciences》2012,67(2):385-394
Dissolution?Cprecipitation phenomena induced by CO2 injection to Altmark Permian sandstone were observed through laboratory experiments carried out under simulated reservoir conditions (125?°C and 50 bars of pressure). The rock sample was collected from the Altmark gas reservoir, which is being considered for enhanced gas recovery. Two sets of experiments were performed with pulverized rock samples in a closed batch reactor with either pure water (run 1) or 3?M aqueous NaCl solution (run 2) and reacted with injected CO2 for 3, 5, and 9?days. The liquid samples were analyzed by inductively coupled plasma optical emission spectroscopy and total reflection X-ray fluorescence, where the latter proved to be a feasible alternative to conventional analytical techniques, especially since only small sample volumes (about 10???l) are needed. Chemical analysis for both fluids (water and NaCl brine) indicated a significant dissolution of calcite and anhydrite in the solution, which might be a crucial process during CO2 injection. The brine solution enhanced the dissolution of calcite and anhydrite compared to pure water at the beginning of the reaction. Moreover, the progressive higher Si4+/Al3+ molar ratios (in average by a factor of 3) in the brine experiments indicated quartz dissolution. Thermodynamic calculations of mineral saturation indices highlighted the dissolution of the Ca-bearing minerals, which was in agreement with experimental results. Modeling enabled an evaluation of the dissolution processes of minerals in a low-salinity region, yet hindrances to model more saline conditions emphasize the need for further laboratory studies in order to parameterize models for deep aquifer conditions. 相似文献
45.
We present a non-invasive technique for measuring the thermal conductivity of fragile and sensitive materials. In the context of planet-formation research, the investigation of the thermal conductivity of porous dust aggregates provide important knowledge about the influence of heating processes, like internal heating by radioactive decay of short-lived nuclei, e.g. 26Al, on the evolution and growth of planetesimals. The determination of the thermal conductivity was performed by a combination of laboratory experiments and numerical simulations. An IR camera measured the temperature distribution of the sample surface heated by a well-characterized laser beam. The thermal conductivity as free parameter in the model calculations, exactly emulating the experiment, was varied until the experimental and numerical temperature distributions showed best agreement. Thus, we determined for three types of porous dust samples, consisting of spherical, 1.5 μm-sized SiO2 particles, with volume filling factors in the range of 15-54%, the thermal conductivity to be 0.002-0.02 W m−1 K−1, respectively. From our results, we can conclude that the thermal conductivity mainly depends on the volume filling factor. Further investigations, which are planned for different materials and varied contact area sizes (produced by sintering), will prove the appropriate dependencies in more detail. 相似文献
46.
Air pollution over European Russia and Ukraine under the hot summer conditions of 2010 总被引:1,自引:0,他引:1
A. M. Zvyagintsev O. B. Blum A. A. Glazkova S. N. Kotel’nikov I. N. Kuznetsova V. A. Lapchenko E. A. Lezina E. A. Miller V. A. Milyaev A. P. Popikov E. G. Semutnikova O. A. Tarasova I. Yu. Shalygina 《Izvestiya Atmospheric and Oceanic Physics》2011,47(6):699-707
Variations in the concentrations of both primary (PM10, CO, and NOx) and secondary (ozone) pollutants in the atmosphere over the Moscow and Kirov regions, Kiev, and Crimea under the conditions of the anomalously hot summer of 2011 are given and analyzed. The concentrations of ozone, PM10, CO, and NOx in the atmosphere over the Moscow region exceeded their maximum permissible levels almost continuously from late July to late August 2010. The highest level of atmospheric pollution was observed on August 4–9, when the Moscow region was within a severe plume of forest and peatbog fires. The maximum single concentrations of ozone, which exceeded its maximum permissible level two-three times, were accompanied by high concentrations of combustion products: the concentrations of PM10 and CO were also three-seven times higher than their maximum permissible concentrations. The maximum levels of air pollution were observed under the meteorological conditions that were unfavorable for pollution scattering, first of all, at a small vertical temperature gradient in the lower atmospheric boundary layer. The number of additional cases of mortality due to the exceeded maximum permissible concentrations of PM10 and ozone in the atmosphere over Moscow was estimated. Under the weather conditions that were close to those for the Moscow region, the air quality remained mainly satisfactory in the Kirov region, Kiev, and Crimea, which were almost not affected by fires. 相似文献
47.
The extremely porous structure and low strength of most comets and their fragments is opposed to the properties observed in relatively pristine chondritic asteroids, even although both are sharing important chemical similitude. Laboratory experiments and observational evidence suggest that the original extremely porous aggregates that were born from the protoplanetary-disk-forming materials were highly retentive of water and organic compounds present in their forming environment. After consolidation, many of them experienced a particular dynamic history. Some bodies, quickly scattered during the formation of the giant planets and later stored in the Kuiper Belt (KB) or the Oort Cloud (OC) regions, would have suffered a lower degree of impact processing than previously thought. In such category would be comet 81P/Wild 2, whose materials have not experienced aqueous alteration. Other bodies originally volatile-rich that were transiting other regions with higher impact rate were experiencing progressively significant compaction processing, together with subsequent aqueous alteration and loss of volatiles. The release of water from hydrated minerals or interior ices, participated in soaking the forming materials, and transforming their initial mineralogy and physical properties. As a consequence of the physico-chemical evolution promoted by impact processing of undifferentiated bodies, most of the bodies present in the inner solar system are not representative of the planetesimals. Thus, highly porous progenitors and their fragments are the preferential sources of water and organics to the early Earth, even in higher amounts than previously thought. 相似文献
48.
Art F. White Marjorie S. Schulz Davison V. Vivit Tom D. Bullen Alex E. Blum 《Geochimica et cosmochimica acta》2009,73(10):2769-58
The spatial and temporal changes in hydrology and pore water elemental and 87Sr/86Sr compositions are used to determine contemporary weathering rates in a 65- to 226-kyr-old soil chronosequence formed from granitic sediments deposited on marine terraces along coastal California. Soil moisture, tension and saturation exhibit large seasonal variations in shallow soils in response to a Mediterranean climate. These climate effects are dampened in underlying argillic horizons that progressively developed in older soils, and reached steady-state conditions in unsaturated horizons extending to depths in excess of 15 m. Hydraulic fluxes (qh), based on Cl mass balances, vary from 0.06 to 0.22 m yr−1, resulting in fluid residence times in the terraces of 10-24 yrs.As expected for a coastal environment, the order of cation abundances in soil pore waters is comparable to sea water, i.e., Na > Mg > Ca > K > Sr, while the anion sequence Cl > NO3 > HCO3 > SO4 reflects modifying effects of nutrient cycling in the grassland vegetation. Net Cl-corrected solute Na, K and Si increase with depth, denoting inputs from feldspar weathering. Solute 87Sr/86Sr ratios exhibit progressive mixing of sea water-dominated precipitation with inputs from less radiogenic plagioclase. While net Sr and Ca concentrations are anomalously high in shallow soils due to biological cycling, they decline with depth to low and/or negative net concentrations. Ca/Mg, Sr/Mg and 87Sr/86Sr solute and exchange ratios are similar in all the terraces, denoting active exchange equilibration with selectivities close to unity for both detrital smectite and secondary kaolinite. Large differences in the magnitudes of the pore waters and exchange reservoirs result in short-term buffering of the solute Ca, Sr, and Mg. Such buffering over geologic time scales can not be sustained due to declining inputs from residual plagioclase and smectite, implying periodic resetting of the exchange reservoir such as by past vegetational changes and/or climate.Pore waters approach thermodynamic saturation with respect to albite at depth in the younger terraces, indicating that weathering rates ultimately become transport-limited and dependent on hydrologic flux. Contemporary rates Rsolute are estimated from linear Na and Si pore weathering gradients bsolute such that
49.
Climatic and tectonic controls on chemical weathering in the New Zealand Southern Alps 总被引:2,自引:0,他引:2
Climatic and tectonic controls on the relative abundance of solutes in streams draining the New Zealand Southern Alps were investigated by analyzing the elemental and Sr isotope geochemistry of stream waters, bedload sediment, and hydrothermal calcite veins. The average relative molar abundance of major cations and Si in all stream waters follows the order Ca2+ (50%) > Si (22%) > Na+ (17%) > Mg2+ (6%) > K+ (5%). For major anions, the relative molar abundance is HCO3− (89%) > SO42− (7%) > Cl− (4%). Weathering reactions involving plagioclase and volumetrically small amounts of hydrothermal calcite define the ionic chemistry of stream waters, but nearly all streams have a carbonate-dominated Ca2+ and HCO3− mass-balance. Stream water Ca/Sr and 87Sr/86Sr ratios vary from 0.173 to 0.439 μmol/nmol and from 0.7078 to 0.7114, respectively. Consistent with the ionic budget, these ratios lie solely within the range of values measured for bedload carbonate (Ca/Sr = 0.178 to 0.886 μmol/nmol; 87Sr/86Sr = 0.7081 to 0.7118) and hydrothermal calcite veins (Ca/Sr = 0.491 to 3.33 μmol/nmol; 87Sr/86Sr = 0.7076 to 0.7097).Streams draining regions in the Southern Alps with high rates of physical erosion induced by rapid tectonic uplift and an extremely wet climate contain ∼10% more Ca2+ and ∼30% more Sr2+ from carbonate weathering compared to streams draining regions in drier, more stable landscapes. Similarly, streams draining glaciated watersheds contain ∼25% more Sr2+ from carbonate weathering compared to streams draining non-glaciated watersheds. The highest abundance of carbonate-derived solutes in the most physically active regions of the Southern Alps is attributed to the tectonic exhumation and mechanical denudation of metamorphic bedrock, which contains trace amounts of calcite estimated to weather ∼350 times faster than plagioclase in this environment. In contrast, regions in the Southern Alps experiencing lower rates of uplift and erosion have a greater abundance of silicate- versus carbonate-derived cations. These findings highlight a strong coupling between physical controls on landscape development and sources of solutes to stream waters. Using the Southern Alps as a model for assessing the role of active tectonics in geochemical cycles, this study suggests that rapid mountain uplift results in an enhanced influence of carbonate weathering on the dissolved ion composition delivered to seawater. 相似文献
50.
Ralph K. Davis Darryll T. Pederson Darryl A. Blum James D. Carr 《Ground Water Monitoring & Remediation》1993,13(2):134-141
Lincolns municipal wellfield consists of 44 wells developed in an alluvial aquifer adjacent to the Platte River near Ashland, Nebraska Induced recharge from the river is the primary source of water for the wellfield. Wafer samples were collected on a periodic basis from the Platte River arid two transects of monitoring wells. These samples were analyzed for the herbicide atrazine, which was used as a tracer of induced recharge in this stream-aquifer system. Atrazine concentrations in the river and aquifer were much less than 1.0 ppb during late fall and winter, but increased to as high as 18.9 ppb during spring and summer, associated with runoff from upgradient agricultural lands. There was approximately a 21-day lag time from the first detection of increasing atrazine concentration in the river to the first detection in monitoring wells immediately adjacent to the river. This lag time was relatively constant throughout the year and from one year to the next, even with major fluctuations of river stage and wellfield production. This consistency of lag time indicated that the travel times from the river to the first set of monitoring wells immediately adjacent to the river were fairly constant.
Paths of preferential flow were identified in the aquifer at a depth of 25 to 35 feet below land surface. This aquifer zone appeared to play a significant role in movement of water from beneath the river into the wellfield.
Aquifer dispersivity was calculated using a method described by Hoehn and Santschi (1987). Macrodispersivity (AL ) was shown to increase linearly over the scale of the wellfield. Calculated values of AL were within limits of other reported values for this type of aquifer material and agreed well with values reported by Hoehn and Santschi (1987); These findings will be extremely beneficial for planning and management of the municipal wellfield. 相似文献
Paths of preferential flow were identified in the aquifer at a depth of 25 to 35 feet below land surface. This aquifer zone appeared to play a significant role in movement of water from beneath the river into the wellfield.
Aquifer dispersivity was calculated using a method described by Hoehn and Santschi (1987). Macrodispersivity (A