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221.
Shaw Cliff S. J. Thibault Yves Edgar Alan D. Lloyd Felicity E. 《Contributions to Mineralogy and Petrology》1998,132(4):354-370
Experiments dissolving orthopyroxene (En93) in a variety of Si-undersaturated alkaline melts at 1 atmosphere and variable f
O2 demonstrate that orthopyroxene dissolves to form olivine, Si-rich melt and clinopyroxene. These phases form a texturally
and chemically distinct boundary layer around the partly dissolved orthopyroxene crystals. The occurrence of clinopyroxene
in the boundary layer is due to inward diffusion of Ca from the solvent melt to the boundary layer causing clinopyroxene saturation.
Compositional profiles through the solvent and the boundary layer for a number of experiments demonstrate rapid diffusion
of cations across the boundary layer – solvent interface. SiO2 diffuses outward from the boundary layer whereas CaO and Al2O3 diffuse toward the Si-enriched boundary layer melt. The rate of Al diffusion is slower under reducing conditions compared
to the rates in experiments performed in air. Concentrations of FeO and MgO in the boundary layer and solvent are approximately
equal indicating rapid diffusion and attainment of equilibrium despite ongoing crystallisation of clinopyroxene within the
boundary layer. The behaviour of Na2O and K2O is strongly affected by f
O2. Under reducing conditions Na2O and K2O concentrations are approximately equal in the boundary layer and solvent indicating normal diffusion down the concentration
gradient and attainment of equilibrium. Under oxidising conditions, K2O and to a lesser extent Na2O, have compositional profiles indicative of uphill diffusion likely due to their preference for more polymerised Si- and
Al-rich melts. Under reduced conditions Al-enrichment in the boundary layer melt is not as extreme and uphill diffusion did
not occur. The composition of the solvent melt after the experiments indicates that it was contaminated by the boundary layer
by convective mixing due to the onset of hydrodynamic instabilities brought on by density and viscosity contrasts between
the two melts. Despite using a wide variety of solvent melt compositions we find that the boundary layer melts converge toward
a common composition at high SiO2 contents. The composition of glass generated by orthopyroxene dissolution at 1 atmosphere is similar in many respects to
Si-rich glass found in many orthopyroxene-rich mantle xenoliths that have been attributed to high pressure in situ processes
including mantle metasomatism. The results of this study suggest that at least some Si-rich melts are likely to have formed
by dissolution of xenolith orthopyroxene at low pressure possibly by their Si-undersaturated host magmas.
Received: 30 August 1996 / Accepted: 15 April 1998 相似文献
222.
Willard S. Moore 《Journal of Earth System Science》1998,107(4):343-349
The fate of dissolved material delivered to the coastal ocean depends on its reactivity and the rate at which it is mixed
offshore. To measure the rate of exchange of coastal waters, we employ two short-lived radium isotopes,223Ra and224Ra. Along the coast of South Carolina, shore-perpendicular profiles of223Ra and224Ra in surface waters show consistent gradients which may be modeled to yield eddy diffusion coefficients of 350–540 m2s−1. Coupling the exchange rate with offshore concentration gradients yields estimates of offshore fluxes of dissolved materials.
For systems in steady state, the offshore fluxes must be balanced by new inputs from rivers, groundwater, sewers or other
sources. Two tracers that show promise in evaluating groundwater input are barium and226Ra. These tracers have high relative concentrations in the fluids and low-reactivity in the coastal ocean. Applying the eddy
diffusion coefficients to the offshore gradient of226Ra concentration provides an estimate of the offshore flux of226Ra. Measuring the concentrations of226Ra in subsurface fluids provides an estimate of the fluid flux necessary to provide the226Ra. These estimates indicate that the volume of groundwater required to support these fluxes is of the order of 40% of the
surface water flow. 相似文献
223.
Moore Emerson Skinner Meixner Arens & Jernigan 《Monthly notices of the Royal Astronomical Society》1998,299(4):1209-1214
We present arcsec-resolution images at 8.2, 10.0 and 11.3 μm of the unusual young object WL 16 in Ophiuchus, which has an extended envelope of fluorescing hydrocarbon molecules. To the limit of achieved sensitivity, the faint 10.0-μm continuum has a surface-brightness distribution that is not distinguishable from those at 8.2 and 11.3 μm, where the luminosity is known to be dominated by the polycyclic aromatic hydrocarbon (PAH) emission features. We conclude that the 10-μm continuum either arises from non-equilibrium heating of small dust grains that are well mixed with the hydrocarbons or is quasi-continuous emission from the PAH particles themselves, rather than thermal equilibrium emission from macroscopic dust grains, and that there is no significant silicate absorption variation across the source. The extended hydrocarbon emission may trace a flattened, equatorial distribution of circumstellar material or arise in bipolar lobes. The former case is slightly favoured, based on currently available data, and would imply that WL 16 is a relatively evolved Herbig Ae star, the equatorial plane of which has been almost cleared of normal dust, leaving only fluorescing hydrocarbons and larger coagulated particles as a possibly transient fossil of the original circumstellar disc. 相似文献
224.
Field relations, petrographic features, major and selected trace element compositions, and Sr- and Pb- isotope characteristics indicate that the Coire Uaigneich Granophyre (CUG) was formed by the mixing of two magmas. One of these, a liquid of high 87Sr/86Sr ratio (ca. 0.731) formed by the anatexis of late Precambrian Torridonian sediments, contained relict quartz and zircon. The other liquid was an acid differentiate of basaltic magma and was enriched in incompatible elements such as Zr and Y. The two magmas mixed in the proportions of approximately two parts anatectic melt to one part acid differentiate. Hydrothermal metamorphism had no significant effect on the bulk chemistry of the CUG. 相似文献
225.
Alan P. Heward 《Earth》1981,17(3):223-276
Barrier islands, beaches, wave-dominated deltas and chenier plains probably form more than one-fifth of present coasts, and constitute an even larger proportion of the subsiding lowland coasts likely to be preserved in the stratigraphic record. The geometry, vertical sequences and composition of their deposits are the result of: (1) shoreline behaviour, whether transgressive, regressive or stable; (2) physical processes, particularly the relative intensities of waves and tides; (3) climate; (4) global tectonic setting; and (5) topography of underlying deposits.Published interpretations indicate that equivalent deposits are abundant in the geological record. Sandstones are mostly quartzose, cemented by carbonates and quartz, and have sheet or linear geometries. Ancient deposits can provide evidence of palaeogeography and some are economically significant, particularly as hydrocarbon reservoir rocks.Four end-member sedimentation models are proposed for the interpretation of ancient deposits: (1) transgressive sheet sands associated with deltas; (2) non-deltaic transgressive sheet sands; (3) regressive sheet sands; and (4) linear sand bodies. Probable depositional settings, geometries, characteristics of deposits and palaeocurrent patterns are discussed. 相似文献
226.
Dhanpat Rai R.G. Strickert D.A. Moore R.J. Serne 《Geochimica et cosmochimica acta》1981,45(11):2257-2265
Americium-241 concentrations in solutions contacting contaminated sediments for up to 2 yr were measured as a function of pH. Steady-state concentrations were reached within a few days. The solubility-limited Am concentration was found to decrease approximately 10-fold with one unit increase in pH. The log equilibrium constant for the solubility of Am(soil) solid was found to be ?4.12. The predictions based upon thermodynamic data suggest that Am(aq complex)+ is likely to be Am(OH)2+. Although the chemical formula of Am(soil) was not determined, it does not appear to be Am(OH)3(a).Published data on sorption coefficients of Am by different rocks, soils, and minerals were critically evaluated. Final Am solution concentrations calculated from the sorption coefficients of a variety of earth materials with several solutions agreed well with the concentrations predicted from the solubility of Am(soil) solid, indicating that the sorption coefficient data are controlled by Am precipitation. 相似文献
227.
Willard S. Moore Kenneth W. Bruland Jacqueline Michel 《Earth and Planetary Science Letters》1981,53(3):391-399
Samples from the MANOP Santa Barbara Basin sediment trap intercomparison were analyzed for the isotopes of uranium, thorium, radium, lead, and polonium. All of the traps showed approximately the same compositions and isotopic ratios, indicating that they trapped similar materials. The234Th flux via falling particles was very close to the flux predicted from the production and scavenging rates of234Th from the water column. The210Pb content of the trapped particles and the surface sediments were the same, however, the measured flux of210Pb was seven times greater than the predicted flux. Predicted and measured fluxes of228Th and210Po were similarly out of balance. To explain this apparent inconsistency, we suggest (as others have done) that the Santa Barbara Basin is an area where scavenging from the water column is intensified and where sediments deposited initially on the margins may be physically remobilized on a short time scale. These two effects increase the apparent area from which the basin derives the longer-lived isotopes but does not increase significantly the supply of the short-lived234Th. 相似文献
228.
Emergent Pleistocene sea level indicators in the northern Bahamas include: a bioerosional notch at +5.3 to 5.9 m; sea caves, notches, and marine terraces at about +4.3 m; and lithified coral rubble and reef deposits between 0 and 3 m. Thorium 230 dates of the fossil corals, which were deposited as these features were being produced, span the age range from 100 to 145 thousand years BP with a majority falling between 115 and 130 thousand years BP. The notch at about +5.6 m is interpreted to be the product of a sea level stand 125 thousand years BP, while the features at +4.3 m are believed to be formed sometime later as sea level fell from the higher position. Part of the age span is inherent in the dating technique and possible sample alteration. Another cause of the spread may be mixing of corals of different ages into a single deposit. 相似文献
229.
Subsolidus and melting reactions involving calcic plagioclase in pelitic assemblages in the K-Na-Ca model system occur at higher temperatures than their K-Na counterparts. For the most calcic plagioclase compositions observed in high-grade pelitic rocks (An25-An40) the equilibria are rarely extended by more than 30 ° C above those in KA1O2-NaAlO2-Al2O3-SiO2-H2O, although all discontinuities in facies inferred for the K-Na system are continuously displaced when they involve Ca-bearing plagioclase. The maximum pressure-temperature overlap between muscovite dehydration and initial melting reactions occurs in the pressure range of 4–6 kbar between about 640 ° and 720 ° C. This provides optimum conditions for anatectic melt generation in felsic rocks of the appropriate compositions progressively metamorphosed in kyanite-sillimanite facies series. Progressive regional metamorphism at pressures of 2–4 kbar, corresponding to andalusite-sillimanite facies series, shows little overlap between muscovite dehydration and initial melting reactions. Consequently anatectic melt generation in andalusite-sillimanite facies series would require the participation of biotite in dehydration-melting reactions. Felsic intrusive rock in andalusite-sillimanite terranes could have risen upward from their anatectic sites in high grade kyanite-sillimanite facies series at depth. Many andalusite-sillimanite facies series terranes culminating in migmatites could represent upward movement of kyanite-sillimanite facies series rocks to shallower depths with uplift rates faster than cooling rates. 相似文献
230.