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163.
不同氧化锰矿物对光催化降解苯酚的影响 总被引:1,自引:0,他引:1
合成层状结构的酸性和碱性水钠锰矿以及隧道结构的锰钾矿和钙锰矿,将其用于苯酚的光催化降解研究。分别采用X射线衍射(XRD)、原子吸收光谱(AAS)、扫描电镜(SEM)、BET氮气吸附法和紫外可见漫反射光谱(UV-Vis DRS)对供试锰氧化物的晶体结构、化学组成、微观形貌、比表面积以及光吸收性能等进行了表征。研究表明,暗反应条件锰氧化物对苯酚的降解作用较弱,而UV-Vis光照能显著促进锰氧化物对苯酚的降解。光照反应12 h后,锰钾矿、酸性水钠锰矿、钙锰矿以及碱性水钠锰矿的苯酚降解率分别为92.1%、77.3%、57.4%和45.8%;对应的TOC去除率分别由暗反应时的6.3%、11.2%、2.0%和4.6%提高至62.1%、43.1%、25.4%和22.5%。4种供试锰氧化物均具有光催化活性,其大小顺序为:锰钾矿>酸性水钠锰矿>钙锰矿>碱性水钠锰矿。UV-Vis光照下氧化锰矿物光化学降解苯酚主要存在3种降解机制———苯酚的直接光解,锰氧化物的化学氧化和锰氧化物的光化学催化,其中光催化降解起主导作用。 相似文献
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166.
不同氧化度碱性水钠锰矿氧化As(Ⅲ)和Cr(Ⅲ) 的动力学特性 总被引:1,自引:0,他引:1
用批量法研究了Mn平均氧化度分别为4.02、3.85和3.70的碱性水钠锰矿对As(Ⅲ)和Cr(Ⅲ)氧化的动力学特性。结果表明,碱性水钠锰矿氧化As(Ⅲ)和Cr(Ⅲ)先经历准一级动力学反应阶段,随后表观速率常数(kobs)逐渐减小至趋近零,达到反应平衡,kobs逐渐减小除了逆反应影响外,还与产物在矿物表面不断积累,钝化反应位点有关。初始反应阶段kobs随氧化度增加而增大,氧化As(Ⅲ)的kobs分别为: 0.095 1、0.039 6和0.007 1 min-1;氧化Cr(Ⅲ)的kobs分别为0.034 2、0.017 8和0.014 8 min-1。氧化As(Ⅲ)的初始反应阶段生成的Mn(Ⅱ)基本保留在矿物表面,对反应位点钝化大,使kobs减小速度快。而Cr(Ⅲ) 氧化初始阶段,Mn(Ⅱ)释放明显滞后于Cr(Ⅵ)释放,但随反应进行逐渐增加,与Cr(Ⅵ)释放量比值接近于反应计量比。故Cr(Ⅲ) 氧化生成Mn(Ⅱ)对位点的钝化远小于As(Ⅲ)氧化,其初始反应阶段后kobs减小速度较慢,且氧化度越高,保持一级动力学的初始反应阶段越长,kobs减小越慢。因此,水钠锰矿的Mn氧化度越高,氧化As(Ⅲ)和Cr(Ⅲ)的反应速率越快,As(Ⅲ)和Cr(Ⅲ)在碱性水钠锰矿表面氧化产物的释放行为是影响其反应动力学特性的重要因素。 相似文献
167.
Yang Zhang Fei Chai Joseph Zhang Yang Ding Min Bao Yunwei Yan Hong Li Wei Yu Liang Chang 《海洋学报(英文版)》2022,41(2):127-138
During the northeast monsoon season, Zhe-Min Coastal Current(ZMCC) travels along the Chinese mainland coast and carries fresh, cold, and eutrophic water. ZMCC is significantly important for the hydrodynamic processes and marine ecosystems along its path. Thus, this bottom-trapped plume deserves to be further discussed in terms of the major driving factor, for which different opinions exist. For this purpose, in this study, a high resolution Semi-implicit Cross-scale Hydroscience Integrated Syste... 相似文献
168.
This paper describes studies on the integrated risk assessment and zoning of meteorological disaster in Heilongjiang Province,in northeastern China,by using information-diffusion theory and cluster method with 35 years of summer temperature and precipitation data from 74 meteorological stations from 1971 through 2005.The information-diffusion theory has been used extensively in risk assessment,yet almost no one has done research about risk assessment by information-diffusion theory based on meteorological disaster standards.Some research results are as follows:the risk probability of low temperature and cold damage in the northern region is higher than that in the southern region;the risk probability of general low temperature and cold damage in the southwestern region is the highest;the risk probability of serious low temperature and cold damage in the northern region is the highest,followed by the central and southeast region;the high-risk region of arid disaster in Heilongjiang Province was primarily located in the southwestern,central,and southern parts of the province;the high-intensity arid disaster was located in the south-eastern region;the high-risk region of flood in Heilongjiang Province was primarily located from the southwest and then across the central part to the western part of Heilongjiang Province;the high-intensity flood disasters were located in almost every part of Heilongjiang Province.We can conclude from the integrated meteorological disaster risk zoning that the high-risk region of mete-orological disaster is primarily located in the southern and northern part of the province,the moderate-risk region is distributed in the central southern region and western region,the low-risk region is located in the eastern part,and the light-risk region is located in the central western part of Heilongjiang Province. 相似文献
169.
Constraints on the age of the Tuchengzi Formation by LA-ICP-MS dating in northern Hebei-western Liaoning,China 总被引:2,自引:0,他引:2
ZHANG Hong WEI ZhongLiang LIU XiaoMing & LI Dong College of Mechanical Energy Engineering Jiangsu Polytechnic University Changzhou China State Key Laboratory of Continental Dynamics Northwest University Xi’an 《中国科学D辑(英文版)》2009,52(4):461-470
Accurately determining the age of the Tuchengzi Formation has direct influence on confirming the boundary between the Jurassic
and the Cretaceous systems in northern Hebei-western Liaoning, and on related geological problems in China. However, the Tuchengzi
Formation mainly consists of sedimentary rocks, with a poor fossil record and especially lack of index fossils. The Tuchengzi
Formation is also lack of the type of volcanic rocks that can provide an isotopic age. Therefore, the age of the Tuchengzi
Formation has been uncertain. Based on our systematic dating of the tuff interbedded in the Tuchengzi Formation of Chengde
and Jinlingsi-Yangshan basins in northern Hebei-western Liaoning, combined with the dating results of previous researchers,
here we suggest that the age range of the Tuchengzi Formation in northern Hebei-western Liaoning is from 147 Ma to 136 Ma.
It implied that the Tuchengzi Formation was mainly formed in the Early Cretaceous.
Supported by National Natural Science Foundation of China (Grant No. 90714010) 相似文献
170.
湖南白兔潭矿区荷田区段构造特征与找煤前景 总被引:1,自引:0,他引:1
煤炭是湖南省的主要能源,经过多年的勘探开发,暴露区和浅部的煤炭资源已基本采完,因此,在隐伏区寻找新的煤炭资源已成为当务之急。隐伏区找煤主要指“三下”(老地层下、构造下和红层下)找煤,而“老地层下和构造下”找煤主要是指利用推覆构造理论寻找新的煤炭资源。为了深化对区域构造和煤田构造发育规律的认识,为本区煤炭资源勘探和矿井生产地质保障提供新思路、开拓新领域,以当代构造地质理论为指导,结合已有资料,对白兔潭矿区荷田区段的煤田构造进行了研究,揭示了煤田的构造格局,提出了该区可能存在的两种构造模式,对该区找煤前景做出了科学评价,指出了可供进一步勘探的有利区段。 相似文献