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排序方式: 共有417条查询结果,搜索用时 31 毫秒
51.
Norimichi Takenaka Tohru Daimon Akihiro Ueda Keiichi Sato Masaru Kitano Hiroshi Bandow Yasuaki Maeda 《Journal of Atmospheric Chemistry》1998,29(2):135-150
Nitrite oxidation in the tropospheric aqueous phase by freezing was evaluated by freezing a field sample. Nitrite oxidation by dissolved oxygen in the freezing process is much faster than by other oxidation processes, such as reactions with ozone, hydrogen peroxide or dissolved oxygen in an aqueous solution at pHs 3 to –6. At pH 4.5 and 25°C, the lifetime of nitrite in the aqueous phase is ca. 1 hr in oxidation by ozone (6×10-10 mol dm-3), ca. 10 hr in oxidation by H2O2 (2×10-4 mol dm-3), and 7.5 hr (Fischer and Warneck, 1996) in photodissociation at midday in summer. Under the same conditions at a temperature below 0°C, the lifetime of nitrite in the freezing process is estimated as ca. 2 sec when the droplets are frozen within a second. The reaction by freezing is affected by the presence of salts, such as NaCl or KCl, or orgnaic compounds, such as methanol or acetone. The results of freezing a field rain or fog sample showed that nitrite oxidation proceeds below pH 6, and the conversion ratio of nitrate from nitrite increases with decreasing pH. The oxidation of nitrite by freezing was also observed in freezing fog particles generated by an ultrasonic humidifier. The ratios of the concentrations of ions in the winter sample to those in the summer sample (or those in the fog sample) were almost the same values. However, the concentration of nitrite in the winter sample was lower than that estimated by the ratios of other ions. From the present study, it seems that the freezing process plays an important role in the nitrite sink process in the tropospheric aqueous phase. 相似文献
52.
K. Yoshimoto H. Sato Y. Iio H. Ito T. Ohminato M Ohtake 《Pure and Applied Geophysics》1998,153(2-4):489-502
—Borehole seismograms from local earthquakes in the aftershock region of the 1984 western Nagano Prefecture, Japan earthquake were analyzed to measure the frequency-dependent characteristics of P- and S-wave attenuation in the upper crust. The records from a three-component velocity seismometer at the depth of 145m exhibit high S/N-ratio in a wide frequency range up to 100 Hz. Extended coda normalization methods were applied to bandpass-filtered seismograms of frequencies from 25 to 102 Hz. For the attenuation of high-frequency P and S waves, our measurements show Q P -1? 0.052?-0.66 and Q S -1? 0.0034?-0.12 respectively. The frequency dependence of the quality factor of S waves is very weak as compared with that of P waves. The ratio of Q P -1/Q S -1 is larger than unity in the entire analyzed frequency range. 相似文献
53.
A new technique has been developed for measuring the diffusion coefficient in ionic crystals. Based on Einstein's formula expressing the relation between diffusion coefficient and electric mobility, the electrical impedance of a diatomic ionic crystal is derived theoretically as a function of frequency of the applied electric field. In this method, the diffusion coefficients of both cations and anions are determined simultaneously by fitting the measured impedance to the theoretical relation. This method was applied to NaCl single crystals in the temperature range 370–780°C. The impedance was determined over the frequency range 0.01 Hz to 1 kHz, at constant temperature. The diffusion coefficients thus obtained for NaCl agree reasonably well with previous data by means of a radioactive isotope technique. The activation energies for Na+ and Cl? obtained are 1.97±0.03 eV and 2.08±0.06 eV, respectively, in the intrinsic region, and 0.92±0.02 eV and 1.06±0.02 eV in the extrinsic region. It was discovered that there are diffusion blocks of approximately 2 μm width, which obstruct free migration of ions in a single crystal. 相似文献
54.
55.
A. Sánchez-Lavega G.S. Orton R. Hueso L.N. Fletcher E. García-Melendo I. de Pater H.B. Hammel A. Simon-Miller F. Marchis O. Mousis J. García-Rojas M. Cecconi K. Noll S. Pedraz P. Kalas W. Golisch P. Sears V. Reddy R. Binzel W. Grundy J. Emery A. Rivkin C. Thomas D. Trilling K. Bjorkman A.J. Burgasser H. Campins T.M. Sato Y. Kasaba J. Ziffer R. Mirzoyan H. Bouy 《Icarus》2011,214(2):462-476
We present a study of the long-term evolution of the cloud of aerosols produced in the atmosphere of Jupiter by the impact of an object on 19 July 2009 (Sánchez-Lavega, A. et al. [2010]. Astrophys. J. 715, L155-L159). The work is based on images obtained during 5 months from the impact to 31 December 2009 taken in visible continuum wavelengths and from 20 July 2009 to 28 May 2010 taken in near-infrared deep hydrogen-methane absorption bands at 2.1-2.3 μm. The impact cloud expanded zonally from ∼5000 km (July 19) to 225,000 km (29 October, about 180° in longitude), remaining meridionally localized within a latitude band from 53.5°S to 61.5°S planetographic latitude. During the first two months after its formation the site showed heterogeneous structure with 500-1000 km sized embedded spots. Later the reflectivity of the debris field became more homogeneous due to clump mergers. The cloud was mainly dispersed in longitude by the dominant zonal winds and their meridional shear, during the initial stages, localized motions may have been induced by thermal perturbation caused by the impact’s energy deposition. The tracking of individual spots within the impact cloud shows that the westward jet at 56.5°S latitude increases its eastward velocity with altitude above the tropopause by 5-10 m s−1. The corresponding vertical wind shear is low, about 1 m s−1 per scale height in agreement with previous thermal wind estimations. We found evidence for discrete localized meridional motions with speeds of 1-2 m s−1. Two numerical models are used to simulate the observed cloud dispersion. One is a pure advection of the aerosols by the winds and their shears. The other uses the EPIC code, a nonlinear calculation of the evolution of the potential vorticity field generated by a heat pulse that simulates the impact. Both models reproduce the observed global structure of the cloud and the dominant zonal dispersion of the aerosols, but not the details of the cloud morphology. The reflectivity of the impact cloud decreased exponentially with a characteristic timescale of 15 days; we can explain this behavior with a radiative transfer model of the cloud optical depth coupled to an advection model of the cloud dispersion by the wind shears. The expected sedimentation time in the stratosphere (altitude levels 5-100 mbar) for the small aerosol particles forming the cloud is 45-200 days, thus aerosols were removed vertically over the long term following their zonal dispersion. No evidence of the cloud was detected 10 months after the impact. 相似文献
56.
Large-eddy simulations were conducted to investigate the mechanism of pollutant removal from a three-dimensional street canyon. Five block configurations with aspect ratios (building height to length) of 1, 2, 4, 8 and $\infty $ were used to create an urban-like array. A pollutant was released from a ground-level line source at the centre of the target canyon floor. For smaller aspect ratios, the relative contribution of the turbulent mass flux to net mass flux at the roof level, which was spatially averaged along the roof-level ventilation area, was closer to unity, indicating that turbulent motions mainly affected pollutant removal from the top of the canyon. As aspect ratio increased, the relative contribution became smaller, owing to strong upwind motions. However, the relative contribution again reached near unity for the infinite aspect ratio (i.e. a two-dimensional street canyon) because of lowered lateral flow convergence. At least 75 % of total emissions from the three-dimensional street canyon were attributable to turbulent motions. Pollutant removal by turbulent motions was related to the coherent structures of low-momentum fluid above the canyons. Though the coherent structure size of the low-momentum fluid differed, the positions of low-momentum fluid largely corresponded to instantaneous high concentrations of pollutant above the target canyon, irrespective of canyon geometry. 相似文献
57.
58.
A procedure for tidal analysis with a Bayesian information criterion 总被引:16,自引:0,他引:16
59.
60.
红外相机CASCAM光学设计 总被引:1,自引:1,他引:0
介绍紫金山天文台研制的光学-近红外相机CASCAM(Chinese Academy of Science,CAMera)的光学系统设计.CASCAM相机以红外列阵HAWAII-1和光学CCD为探测器,配备国家天文台兴隆观测站2.16米和1.26米望远镜进行0.4—2.5μm波长范围的成像和偏振成像观测.相机的光学系统由F/9→F/6缩焦系统和Offner反射成像系统构成.优化设计结果表明,光学设计方案已满足天文观测的要求.CASCAM相机在设计上实现了光学-近红外很宽波段的消色差变焦,并在楔形分柬片、常温滤光片轮和折射式焦面摆动技术等方面进行了新的尝试. 相似文献