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To understand the aqueous species important for transport of rhenium under supercritical conditions, we conducted a series of solubility experiments on the Re–ReO2 buffer assemblage and ReS2. In these experiments, pH was buffered by the K–feldspar–muscovite–quartz assemblage; in sulfur-free systems was buffered by the Re–ReO2 assemblage; and and in sulfur-containing systems were buffered by the magnetite–pyrite–pyrrhotite assemblage. Our experimental studies indicate that the species ReCl4 0 is dominant at 400°C in slightly acidic to near-neutral, and chloride-rich (total chloride concentrations ranging from 0.5 to 1.0 M) environments, and ReCl3 + may predominate at 500°C in a solution with total chloride concentrations ranging from 0.5 to 1.5 M. The results also demonstrate that the solubility of ReS2 is about two orders of magnitude less than that of ReO2. This finding not only suggests that ReS2 (or a ReS2 component in molybdenite) is the solubility-controlling phase in sulfur-containing, reducing environments but also implies that a mixing process involving an oxidized, rhenium-containing solution and a solution with reduced sulfur is one of the most effective mechanisms for deposition of rhenium. In analogy with Re, TcS2 may be the stable Tc-bearing phase in deep geological repositories of radioactive wastes. 相似文献
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利用改进的TurboEdit算法与Chebyshev多项式探测与修复周跳 总被引:1,自引:0,他引:1
根据利用TurboEdit方法对GPS观测数据进行周跳探测的特点,设计了固定弧段长度的滑动窗口拟合模型,对其中的Geometry-Free组合法进行改进;在探测出周跳后,利用最小二乘Chebyshev多项式拟合来修复周跳。实验结果表明,改进后的TurboEdit算法可以探测出等周的1周小周跳、等周的大周跳和连续的小周跳、大周跳,同时,最小二乘Chebyshev多项式拟合可以精确修复以上周跳对。 相似文献
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Yongliang Xiong 《Applied Geochemistry》2011,26(7):1130-1137
Naturally occurring organic ligands, such as acetate, citrate, malonate, oxalate, and succinate, play important roles in mobility and accumulation of La and other rare earth elements in low temperature systems under Earth surface conditions. However, a comprehensive and consistent thermodynamic database covering the complexes of rare earth elements with those naturally occurring organic ligands is lacking. In this study, thermodynamic data of organic species of rare earth elements (REE) represented by La, with an emphasis on their aqueous complexes with organic ligands, are critically reviewed. The organic ligands covered by this study include acetate, citrate, malonate, oxalate and succinate. In this critical review, the Specific Interaction Theory (SIT) model is adopted for extrapolation to infinite dilution. This model is a reliable activity coefficient model valid for a wide range of ionic strengths. These critically reviewed data, including complex formation constants, SIT interaction coefficients and solubility product constants, would enable accurate modeling of the speciation and solubility of REE in various environments including high ionic strength environments, providing insight into mobility and enrichment of REE in various environments. 相似文献
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克停哈尔铜钼多金属矿床是2013~2014年在青海省祁漫塔格成矿带新发现的一处小型矿床,大地构造位置属东昆仑祁漫塔格早古生代裂陷槽,位于柴达木盆地西南缘.区内出露地层主要有古元古代金水口岩群和寒武—奥陶纪滩间山群,金水口岩群碳酸盐岩是矽卡岩型铁多金属矿产出的有利地层.华力西期闪长岩、印支期中酸性花岗岩类发育,印支期似斑状花岗闪长岩是区内铜钼矿的主要含矿岩体.区内构造活动强烈,北西西—北西向的压性、压扭性断裂组成了区域主体构造骨架,多期多组构造交错,为成矿提供了良好通道.矿区成矿具有多期次系列成矿的特征,形成以含矿斑岩体为中心的斑岩铜钼矿化,外围为矽卡岩型铁多金属矿及脉状铅锌矿化的岩浆热液成矿系列. 相似文献
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