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51.
Taku Tsuchiya Takamitsu Yamanaka Masanori Matsui 《Physics and Chemistry of Minerals》1998,25(2):94-100
A two-body interatomic potential model for GeO2 polymorphs has been determined to simulate the structure change of them by semi-empirical procedure, total lattice energy
minimization of GeO2 polymorphs. Based on this potential, two polymorphs of GeO2; α-quartz-type and rutile-type, have been reproduced using the molecular dynamics (MD) simulation techniques. Crystal structures, bulk moduli, volume thermal expansion coefficients and enthalpies of these
polymorphs of GeO2 were simulated. In spite of the simple form of the potential, these simulated structural values, bulk moduli and thermal
expansivities are in excellent agreement with the reliable experimental data in respect to both polymorphs. Using this potential,
MD simulation was further used to study the structural changes of GeO2 under high pressure. We have investigated the pressure-induced amorphization. As reported in previous experimental studies,
quartz-type GeO2 undergoes pressure-induced crystalline-to-amorphous transformation at room temperature, the same as other quartz compounds;
SiO2, AlPO4. Under hydrostatic compression, in this study, α-quartz-type GeO2 transformed to a denser amorphous state at 7.4 GPa with change of the packing of oxygen ions and increase of germanium coordination.
At higher pressure still, rutile-type GeO2 transformed to a new phase of CaCl2-type structure as a post-rutile candidate.
Received: 29 July 1996 / Revised, accepted: 30 April 1997 相似文献
52.
Raman spectra of Ni2SiO4 spinel (O h 7 Z=8) have been measured in the temperature range from 20 to 600 °C and the Raman active vibrations (A 1g +E g +3F 2g ) have been assigned. A calculation of the optically active lattice vibrations of this spinel has been made, assuming a potential function which combines general valence and short range force constants. The values of the force constants at 20 and 500 °C have been calculated from the vibrational frequencies of the observed Raman spectra and infrared (IR) spectral data. The Ni spinel at 20 °C has a prominently small Si-O bond stretching force constant of K(SiO)=2.356 ~ 2.680 md/Å and a large Ni-O bond stretching constant of K(NiO)=0.843 ~ 1.062 md/Å and these force constants at 500 °C decrease to K(SiO)=2.327 ~ 2.494 md/Å and K(NiO)=0.861 ~ 0.990 md/Å. The Si-O bond is noticeably weakened at high temperatures, despite the small thermal expantion from 1.657 Å (20 °C) to 1.660 Å (500 °C). These changes of the interatomic force constants of the spinel at high temperatures are in accord with the thermal structure changes observed by X-ray diffraction study. The weakened Si-O bond is consistent with the fact that Si atoms in the spinel lattice can diffuse at significant rates at elevated temperature. 相似文献
53.
Shoichiro Fukao Manabu D. Yamanaka Hiromasa Matsumoto Toru Sato Toshitaka Tsuda Susumu Kato 《Pure and Applied Geophysics》1989,130(2-3):463-479
Vertical and temporal variations of three-dimensional wind velocity associated with an upper-tropospheric cold vortex-tropopause funnel system were observed by an MST radar in Japan (the MU radar). Marked changes of vertical velocity and horizontal wind direction were found between the inside and outside of the cold vortex. The vertical velocity activity outside the vortex was asymmetric; it was most active in a sector before the vortex. Unsaturated internal gravity waves in their generation stage contribute predominantly to the vertical velocity activity, suggesting that tropospheric occluded cyclones may be a possible source of middle-atmospheric gravity waves through the geostrophic adjustment process. 相似文献
54.
Manabu D. Yamanaka Shoichiro Fukao Hiromasa Matsumoto Toru Sato Toshitaka Tsuda Susumu Kato 《Pure and Applied Geophysics》1989,130(2-3):481-495
Marked wavelike variations of the lower stratospheric wind observed on 7–10 May, 1985 by an MST radar in Japan (by the MU radar) are analyzed assuming that they are induced by monochromatic internal inertio-gravity waves. These variations are mainly composed of two modes (periods: 22 and 24 hours), both of which have zonal phase velocities (C
X
) slower than the mean westerly wind (). A statistical analysis of the zonal phase velocity shows thatC
X
above andC
X
below the tropopause jet stream, which is considered to be a vivid proof of wave selection due to the tropospheric mean flow and upward wave emission from the tropopause jet. A comparison between the MU radar results and routine meteorological observations leads to the conclusion that the marked waves appear when the jet stream takes a maximum wind speed. 相似文献
55.
Simultaneous estimation of effects of source, propagation path, and local site amplification was carried out using observed strong motion records in a frequency range from 0.8 to 20 Hz for the purpose of empirical evaluation of the local site effects in different geological conditions in the northwestern part of Turkey. The analyzed data are S-wave portions of 162 accelerograms from 39 shallow events observed at 14 sites of BYTNet array. A spectral separation method was applied to the observed S-wave spectra. The solutions for source spectra, inelasticity factor of propagation path for S-waves (Q s-value), and factor of site amplification at each site were obtained in a least squares sense. In the analysis, we assumed that the factor of the site amplification at a reference site is the same as that of theoretical amplification of S-waves to the soil model whose bottom layer has an S-wave velocity around 2.15 km/s. The estimated Q s-value of the propagation path is modeled as Q s(f)?=?87.4f0.78. The estimated site amplifications are characterized into three groups. The sites in the first group belong to rock site with no dominant peaks at a frequency range of 2 to 10 Hz. The second group of hard soil sites is characterized with moderately dominant peaks at a frequency of 5 Hz. The last group for soft soil sites has common peaks at a frequency of 4 Hz with larger amplitudes than those in the hard soil group. We, then, compare the amplifications with average S-wave velocity in top 30 m of the shallow S-wave profiles and proposed linear empirical formula between them at each frequency. We, furthermore, inverted the observed amplification factors into S-wave velocity and Q s-value profiles of the deep soil over the basement. 相似文献
56.
Masahito Shigemitsu Yutaka W. Watanabe Yasuhiro Yamanaka Hajime Kawakami Makio C. Honda 《Journal of Oceanography》2010,66(5):697-708
We used time-series sediment trap data for four major components, organic matter and ballast minerals (CaCO3, opal, and lithogenic matter) from 150, 540, and 1000 m in the western subarctic Pacific (WSAP), where opal is the predominant
mineral in sinking particles, to develop four simple models for settling particles, including the “ballast model”. The ballast
model is based on the concept that most of the organic matter “rain” in the deep sea is carried by the minerals. These four
models are designed to simultaneously reproduce the flux of each major component of settling particles at 540 and 1000 m by
using the data for each component at 150 m as initial values. Among the four models, the ballast model, which considers the
sinking velocity increase with depth, was identified as the best using the Akaike information criterion as a measure of the
model fit to data. This model successfully reproduced the flux of organic matter at 540 and 1000 m, indicating that the ballast
model concept works well in the shallow zone of the WSAP on a seasonal timescale. This also suggests that ballast minerals
not only physically protect the organic matter from degradation during the settling process but also enhance the sinking velocity
and reduce the degree of decomposition. 相似文献
57.
The atmosphere-ocean exchange of climatically important gases is determined by the transfer velocity (k) and concentration gradient across the interface. Based on observations in the northwestern subarctic Pacific and Sagami
Bay, we report here the results of the first ever application of the natural abundance of triple isotopes of dissolved oxygen
(16O, 17O and 18O) for direct estimation of k and propose a new relationship with wind speed. The k values estimated from nighttime variations in oxygen isotopes are found to be higher than the direct estimations at low wind
speed (<5 m s−1) and lower at high wind speeds (>13 m s−1) and showed significant spatial variability. The method presented here can be used to derive seasonal and spatial variations
in k and the influence of surface conditions on the value, leading to improved estimates of biogenic/anthropogenic gas exchange
at the air-sea interface. 相似文献
58.
59.
60.
Takamitsu Yamanaka Yutaka Komatsu Hironori Nomori 《Physics and Chemistry of Minerals》2007,34(5):307-318
Many of ilmenites ABO3 compounds bearing transition elements have semiconductive, ferroelectric and antiferromagnetic properties. The high-pressure
diffraction studies of FeTiO3 have been conducted up to 8.2 GPa using synchrotron radiation in KEK at Tsukuba with diamond anvil cell. The compression
mechanism of FeTiO3 ilmenite has been investigated by the structure refinements converged to the reliable factors R = 0.05. The deformations of the FeO6 and TiO6 octahedra were reduced with increasing pressure. In order to elucidate the electric conductivity change with pressure, electron
density distribution of ilmenite have been executed by maximum entropy method (MEM) using single-crystal diffraction intensity
data. MEM based on F
obs(hkl) of FeTiO3 clearly shows electron density in comparison with the difference Fourier synthesis based on F
obs(hkl) − F
calc(hkl). The radial distribution of the electron density indicates electron localization around the cation positions. The bonding
electron density found in bond Fe–O and Ti–O is lowered with pressure. The isotropic temperature factors B
iso become smaller with increasing pressure. Nevertheless the thermal vibration is considerably restrained by the compression,
the electric conductivity is enhanced with pressure. Neither charge transfer nor electron hopping between Fe and Ti along
the c axis in FeTiO3 is plausible under high pressure. But the electric conductivity due to electron super-exchange in Fe–Fe and Ti–Ti has been
clarified by the MEM electron density distribution. The anisotropy in the electric conductivity has been clarified. 相似文献