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81.
The distributions of uranium, radium and thorium isotopes in two anoxic fjords: Framvaren Fjord (Norway) and Saanich Inlet (British Columbia) 总被引:1,自引:0,他引:1
Depth profiles of the naturally-occurring radionuclides 238U, 234U, 226Ra, 228Ra and 228Th were obtained in two diverse anoxic marine environments; the permanently anoxic Framvaren Fjord in southern Norway and the intermittently anoxic Saanich Inlet in British Columbia. Concentrations of total H2S were over three orders of magnitude greater in the anoxic bottom waters of Framvaren Fjord compared to those in Saanich Inlet.In Framvaren Fjord, the O2/H2S interface was located at 17 m. While dissolved 238U behaved conservatively throughout the oxic and anoxic water columns, concentrations based on the 238U/salinity ratio in oxic oceanic waters were almost 30% lower. Dissolved 226Ra displayed a sharp maximum just below the O2/H2S interface, coinciding with dissolved Mn (II) and Fe (II) maxima in this zone. It is suggested that reductive dissolution of Fe-Mn oxyhydroxides remobilizes 226Ra in this region.In Saanich Inlet, the O2/H2S interface was located at 175 m. Dissolved 238U displayed a strongly nonconservative distribution. The depth profiles of dissolved 226Ra and 228Th correlated well with the distribution of dissolved Mn (II) in the suboxic waters above the O2/H2S interface, suggesting that reduction of particulate Mn regulates the behavior of 226Ra and 228Th in this region.Removal residence times for dissolved 228Th in the surface oxic waters of both systems are longer than those generally reported for particle-reactive radionuclides in coastal marine environments. In the anoxic waters of Framvaren Fjord and Saanich Inlet, however, the dissolved 228Th removal residence times are quite similar to values reported for dissolved 210Pb in the anoxic waters of the Cariaco Trench and the Orca Basin. This implies that the geochemistries of Th and Pb may be similar in anoxic marine waters. 相似文献
82.
Projected sea level rise in Florida 总被引:1,自引:0,他引:1
Future sea level rise will lead to salt water intrusion, beach/dune recession, and many other coastal problems. This paper addresses a data based forecasting approach to provide relative sea level rise estimates at locations in Florida where historical water level data exist. Many past estimates of sea level rise have treated the rise as a linear straight line trend over the historical data set. The present paper has allowed for acceleration (or deceleration) in sea level rise to account for the possibility of anthropogenic global warming and consequent higher (than linear straight line) future sea levels similar to values noted by global climatic modelers. Results of the present analysis show sea level rise for Florida being higher than past straight line trend results. 相似文献
83.
An even–odd signal decomposition is performed on a complex shoreline having a longshore sediment transport gradient. The expected impact of erosion due to a navigation channel and structures is discussed and implications of the transport gradient on the decomposed shoreline signal are noted. 相似文献
84.
85.
Adrian Adam Harpold Douglas A. Burns Todd Walter Stephen B. Shaw Tammo S. Steenhuis 《水文研究》2010,24(26):3759-3771
Monitoring the effects of acidic deposition on aquatic ecosystems in the Northeastern US has generally required regular measurements of stream buffering chemistry (i.e. acid‐neutralizing capacity (ANC) and calcium Ca2+), which can be expensive and time consuming. The goal of this paper was to develop a simple method for predicting baseflow buffering chemistry based on the hydrogeomorphic properties of ten nested watersheds in the Neversink River basin (2·0–176·0 km2), an acid‐sensitive basin in the Catskill Mountains, New York State. The tributaries and main reach watersheds have strongly contrasting mean baseflow ANC values and Ca2+ concentrations, despite rather homogeneous vegetation, bedrock geology, and soils. A stepwise regression was applied to relate 13 hydrogeomorphic properties to the mean baseflow ANC values and Ca2+ concentrations. The regression analysis showed that watersheds with lower ANC values had a higher mean ratio of ‘quickflow’ runoff to precipitation during 20 non‐snowmelt runoff events (referred to as mean runoff ratio). The mean runoff ratio could explain at least 80% of the variability in mean baseflow ANC values and Ca2+ concentrations among the ten watersheds. Greater mean runoff ratios also correlated with steeper slopes and greater drainage densities, thus allowing the prediction of baseflow ANC values (r2 = 0·75) and Ca2+ concentrations (r2 = 0·77) with widely available spatial data alone. These results indicate that hydrogeomorphic properties can predict a watershed's sensitivity to acid deposition in regions where the spatial sources of stream buffering chemistry from the bedrock mineralogy and soils are fairly uniform. Copyright © 2010 John Wiley & Sons, Ltd. 相似文献
86.
87.
Mars Global Surveyor (MGS) visible (solarband bolometer) and thermal infrared (IR) spectral limb observations from the Thermal Emission Spectrometer (TES) support quantitative profile retrievals for dust opacity and particle sizes during the 2001 global dust event on Mars. The current analysis considers the behavior of dust lifted to altitudes above 30 km during the course of this storm; in terms of dust vertical mixing, particle sizes, and global distribution. TES global maps of visible (solarband) limb brightness at 60 km altitude indicate a global-scale, seasonally evolving (over 190-240° solar longitudes, LS) longitudinal corridor of vertically extended dust loading (which may be associated with a retrograde propagating, wavenumber 1 Rossby wave). Spherical radiative transfer analysis of selected limb profiles for TES visible and thermal IR radiances provide quantitative vertical profiles of dust opacity, indicating regional conditions of altitude-increasing dust mixing ratios. Observed infrared spectral dependences and visible-to-infrared opacity ratios of dust scattering over 30-60 km altitudes indicate particle sizes characteristic of lower altitudes (cross-section weighted effective radius, ), during conditions of significant dust transport to these altitudes. Conditions of reduced dust loading at 30-60 km altitudes present smaller dust particle sizes . These observations suggest rapid meridional transport at 30-80 km altitudes, with substantial longitudinal variation, of dust lifted to these altitudes over southern hemisphere atmospheric regions characterized by extraordinary (m/s) vertical advection velocities. By LS=230° dust loading above 50 km altitudes decreased markedly at southern latitudes, with a high altitude (60-80 km) haze of fine (likely) water ice particles appearing over 10°S-40°N latitudes. 相似文献
88.
Observations by the Mars Color Imager (MARCI) on board the Mars Reconnaissance Orbiter (MRO) in two ultraviolet (UV, Bands 6 and 7; 258 nm, and 320 nm, respectively) and one visible (Band 1, 436 nm) channels of the 2007 planet encircling dust storm are combined with those made by the two Mars Exploration Rovers (MERs) to better characterize the single scattering albedo (ω0) of martian dust aerosols. Exploiting the low contrast of the surface in the UV (and blue) as well as the reduced importance of surface reflectance under very dusty conditions, we utilize the sampling of photometric angles by the MARCI cross-track geometry to synthesize an analog of the classical Emergence Phase Function (EPF). This so-called “pseudo-EPF”, used in conjunction with the “ground-truth” measurements provided by the MERs, is able to effectively isolate the effects of the dust ω0. The motivation for this approach is the elimination of a significant portion of the type of uncertainty involved in many previous radiative transfer analyses. Furthermore, we produce a self-consistent set of complex refractive indices (m=n+ik) through our use of an explicit microphysical representation of the aerosol scattering properties. Because of uncertainty in the exact size of the dust particles during the epoch of the observations, we consider two effective particle radii (reff) to cover the range anticipated from the literature: 1.6 and 1.8 μm. The resulting set of model-data comparisons, ω0, and m are presented along with an assessment of potential sources of error and uncertainty. Analysis of the Band 1 results is limited to ω0 as a “proof-of-concept” for our approach through a comparison to contemporaneous CRISM EPF results at 440 nm. The derived ω0 are: assuming , and 0.765, for Bands 6, 7, and 1, respectively; for , for the same band order. For either reff case, the total estimated error is 0.022, 0.019, and 0.010, again for Bands 6, 7, and 1. We briefly discuss our retrievals, including the asymmetry parameter (g) associated with our model phase functions, within the context of previous efforts, with an emphasis on the improved precision of our results compared to those in the literature. We also suggest several applications of our results, including an extension of the dust climatological record using MARCI Band 7 pseudo-EPFs outside of 2007 global dust event. Initial work on this particular application using a sample of 135 pseudo-EPFs near the MERs suggests that optical depth retrievals with a precision in the range 0.2-0.4 may be possible under moderate loading conditions (i.e., τ < 1.5). 相似文献
89.
From observations of the metallic species sodium (Na), potassium (K), and magnesium (Mg) in Mercury’s exosphere, we derive implications for source and loss processes. All metallic species observed exhibit a distribution and/or line width characteristic of high to extreme temperature - tens of thousands of degrees K. The temperatures of refractory species, including magnesium and calcium, indicate that the source process for the atoms observed in the tail and near-planet exosphere are consistent with ion sputtering and/or impact vaporization of a molecule with subsequent dissociation into the atomic form. The extended Mg tail is consistent with a surface abundance of 5-8% Mg by number, if 30% of impact-vaporized Mg remains as MgO and half of the impact vapor condenses. Globally, ion sputtering is not a major source of Mg, but locally the sputtered source can be larger than the impact vapor source. We conclude that the Na and K in Mercury’s exosphere can be derived from a regolith composition similar to that of Luna 16 soil (or Apollo 17 orange glass), in which the abundance by number is 0.0027 (0.0028) for Na and 0.0006 (0.0045) for K. 相似文献
90.
Matthew H. Burger Rosemary M. Killen E. Todd Bradley Menelaos Sarantos Nelly Mouawad 《Icarus》2010,209(1):63-74
We present a Monte Carlo model of the distribution of neutral sodium in Mercury’s exosphere and tail using data from the Mercury Atmospheric and Surface Composition Spectrometer (MASCS) on the MErcury Surface, Space ENvironment, GEochemistry, and Ranging (MESSENGER) spacecraft during the first two flybys of the planet in January and September 2008. We show that the dominant source mechanism for ejecting sodium from the surface is photon-stimulated desorption (PSD) and that the desorption rate is limited by the diffusion rate of sodium from the interior of grains in the regolith to the topmost few monolayers where PSD is effective. In the absence of ion precipitation, we find that the sodium source rate is limited to ∼106-107 cm−2 s−1, depending on the sticking efficiency of exospheric sodium that returns to the surface. The diffusion rate must be at least a factor of 5 higher in regions of ion precipitation to explain the MASCS observations during the second MESSENGER flyby. We estimate that impact vaporization of micrometeoroids may provide up to 15% of the total sodium source rate in the regions observed. Although sputtering by precipitating ions was found not to be a significant source of sodium during the MESSENGER flybys, ion precipitation is responsible for increasing the source rate at high latitudes through ion-enhanced diffusion. 相似文献