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81.
The δ13C values of thirty-four individual amino acids and two pyridine carboxylic acids have been obtained fromthe Murchison meteorite. They were found to range from +4.9 to +52.8‰, with statistically significant differences observed both within and between amino acid subgroups. The 13C content of α-amino acids declines with increasing chain length, a trend similar to the ones previously observed for carboxylic acids and alkanes. Also 2-methyl-2-amino acids were found to be heavier in 13C than the corresponding 2-H homologues. The3-, 4-, and 5-amino acids do not show a comparable declining trend in δ13C values and neither do the amino dicarboxylic acids. This variability in δ 13C values can be interpreted as to indicate that the synthetic histories of soluble organics in meteorites may have been diverse even within groups of compounds with very similar functional group composition. 相似文献
82.
Since the early 1990s, US Forest Service researchers have made thousands of bedload measurements in steep, coarse‐grained channels in Colorado and Wyoming, USA. In this paper we use data from 19 of those sites to characterize patterns and rates of coarse sediment transport for a range of channel types and sizes, including step–pool, plane‐bed, pool–riffle, and near‐braided channels. This effort builds upon previous work where we applied a piecewise regression model to (1) relate flow to rates of bedload transport and (2) define phases of transport in coarse‐grained channels. Earlier, the model was tested using bedload data from eight sites on the Fraser Experimental Forest near Fraser, Colorado. The analysis showed good application to those data and to data from four supplementary channels to which the procedure was applied. The earlier results were, however, derived from data collected at sites that, for the most part, have quite similar geology and runoff regimes. In this paper we evaluate further the application of piecewise regression to data from channels with a wider range of geomorphic conditions. The results corroborate with those from the earlier work in that there is a relatively narrow range of discharges at which a substantial change in the nature of bedload transport occurs. The transition from primarily low rates of sand transport (phase I) to higher rates of sand and coarse gravel transport (phase II) occurs, on average, at about 80 per cent of the bankfull (1·5‐year return interval) discharge. A comparison of grain sizes moved during the two phases showed that coarse gravel is rarely trapped in the samplers during phase I transport. Moreover, the movement and capture of the D16 to D25 grain size of the bed surface seems to correspond with the onset of phase II transport, particularly in systems with largely static channel surfaces. However, while there were many similarities in observed patterns of bedload transport at the 19 studied sites, each had its own ‘bedload signal’ in that the rate and size of materials transported largely reflected the nature of flow and sediment particular to that system. Published in 2005 by John Wiley & Sons, Ltd. 相似文献
83.
The δD values of over 40 amino acids and two pyridine carboxylic acids of the Murchison and Murray meteorites have been obtained by compound-specific isotopic analyses. For compounds with no known terrestrial distribution, these values range from approximately +330‰ (for cyclic leucine) to +3600‰ (for 2-amino-2,3-dimethylbutyric acid). The latter value is the highest ever recorded for a soluble organic compound in meteorites and nears deuterium to hydrogen ratios observed remotely in interstellar molecules. Deuterium content varies significantly between molecular species and is markedly higher for amino acids having a branched alkyl chain. The δD value of Murray l-isovaline, with an enantiomeric excess of ∼ 6% in the meteorite, was within experimental error of that determined for the combined dl-isovaline enantiomers. Overall, the hydrogen isotope composition of meteoritic amino acids is relatively simple and their δD values appear to vary more with the structure of their carbon chains than with the number and relative distribution of their functionalities or 13C content. The magnitude and extent of deuterium enrichment shared by many and varied amino acids in meteorites indicate that cosmic regimes such as those found in the interstellar medium were capable of producing, if not all the amino acids directly, at least a suite of their direct precursors that was abundant, varied, and considerably saturated. 相似文献
84.
Sandra Pizzarello 《Geochimica et cosmochimica acta》2005,69(21):5163
85.
Sandra R. Oliveira Oswaldo D. Miranda & José C. N. de Araujo Reuven Opher 《Monthly notices of the Royal Astronomical Society》1998,301(1):115-130
In this article we extend the study performed in our previous article of the collapse of primordial objects. We here analyse the behaviour of the physical parameters for clouds ranging from 107 to 1015 M⊙ . We study the dynamical evolution of these clouds in two ways: as purely baryonic clouds and as clouds with non-baryonic dark matter included. We start the calculations at the beginning of the recombination era, following the evolution of the structure until the collapse (which we defined as the time when the density contrast of the baryonic matter is greater than 104 ). We analyse the behaviour of several physical parameters of the clouds (e.g. the density contrast and the velocities of the baryonic matter and the dark matter) as a function of time and radial position in the cloud. In this study all physical processes that are relevant to the dynamical evolution of the primordial clouds, such as for example photon drag (due to the cosmic background radiation) and hydrogen molecular production, besides the expansion of the Universe, are included in the calculations. In particular we find that the clouds with dark matter collapse at higher redshift when we compare the results with the purely baryonic models. As a general result we find that the distribution of the non-baryonic dark matter is more concentrated than the baryonic one. It is important to stress that we do not take into account the putative virialization of the non-baryonic dark matter; we just follow the time and spatial evolution of the cloud, solving its hydrodynamical equations. We also studied the role of cooling–heating processes in the purely baryonic clouds. 相似文献
86.
Extensive (ca. 50,000 km2) shallow-marine platforms (< 250 m) off northern (34°S) and southern (48°S) New Zealand, and more local areas of shelf between, are blanketed by skeletal carbonate sediments > 70% CaCO3), despite proximity to a tectonically active plate margin. In these regions the terrigenous sediment supply is presently low, and growth of epibenthos is fostered by firm substrates (rock, gravels, shells, seaweeds) and the generally energetic nature and high nutrient levels of open-shelf waters. Rapid transition into adjacent terrigenous-dominated facies is characteristic. Irrespective of water depth, the carbonates are coarse-grained and fragmental; carbonate mud is rare. Calcite dominates over aragonite. High-Mg calcite, widespread off northern New Zealand, is rare in the south. Skeletal material is dominated by bryozoans and bivalve molluscs, with significant local contributions from foraminifers, barnacles, calcareous red algae and echinoderms. The name bryomol is suggested for this distinctive temperate-region skeletal carbonate facies, which can be usefully subdivided based on dominant zoarial growth forms of the bryozoan component, known to be habitat-related. Bioerosion is an important mechanism of skeletal fragmentation and degradation. Many grains, especially aragontic bivalves, are infested by endolithic borers and have low preservation potential. Ages of skeletal material in the surficial deposits range from more than 20,000 years B.P. to modern, which is consistent with both low rates of carbonate production and sediment accumulation, and the wide range in preservation state of grains. Some data suggest that the skeletal carbonates are dispersed and mixed mainly during infrequent movement of sand ribbons, sand waves and sand sheets driven by storm-assisted tidal flows. Tracts of modern, palimpsest and relict carbonates can occur in juxtaposition.
The facies characteristics of the New Zealand shelf carbonate deposits contrast significantly with those of the classical Bahaman-type carbonate model. However, they are similar to those reported from many other mid- to high-latitude carbonate shelves, and afford good analogues for most onland occurrences of New Zealand Cenozoic limestones. 相似文献
87.
Sandra Anderson-Fontana Joseph F. Engeln Paul Lundgren Roger L. Larson Seth Stein 《Earth and Planetary Science Letters》1987,86(1)
We have constructed a new bathymetric chart of part of the Chile transform system, based mainly on an R/V “Endeavor” survey from 100°W to its intersection with the East Ridge of the Juan Fernandez microplate at 34°30′S, 109°15′W. A generally continuous lineated trend can be followed through the entire region, with the transform valley being relatively narrow and well-defined from 109°W to approximately 104°30′W. The fracture zone then widens to the east, with at least two probable en echelon offsets to the south at 104° and 102°W. Six new strike-slip mechanisms along the Chile Transform and one normal fault mechanism near the northern end of the Chile Rise, inverted together with other plate motion data from the eastern portion of the boundary, produce a new best fit Euler pole for the Nazca-Antarctic plate pair, providing tighter constraints on the relative plate motions. 相似文献
88.
89.
Saskia M. ten Grotenhuis Sandra Piazolo T. Pakula Cees W. Passchier Paul D. Bons 《Tectonophysics》2002,350(1)
To evaluate if a polymer is suitable for analog modeling, it is essential to know the rheological properties of the material. Polymers used in analog modeling exhibit a complex rheological behavior; only part of which has been taken into account in most modeling studies. The mechanical behavior is strongly dependent on strain rate and temperature, and is characterized by specific dependencies of the storage and loss moduli, related to the elasticity and viscosity, on the deformation rate (frequency).We have measured the storage and loss moduli at a broad range of strain rates and strains, using an oscillatory parallel-disk rheometer. Investigated materials are polydimethylsiloxane (PDMS), mixtures of PDMS and BaSO4 (filler), Rhodorsil Gomme and mixtures of Rhodorsil Gomme and plastilina, all commonly used in analog experiments.Our measurements show that the rheological properties of mixtures of plastilina and Rhodorsil Gomme depend on its deformation history. Therefore, these mixtures are problematic for analog modeling. For mixtures of PDMS and BaSO4, the significance of the elastic component increases with increasing filler content, and accordingly, these mixtures have a limited application for modeling of viscous deformation. Pure PDMS and Rhodorsil Gomme exhibit Newtonian flow behavior at strain rates commonly used in analog modeling. 相似文献
90.
The influence of vorticity and rheology of matrix material on the development of shape-preferred orientation (SPO) of populations of rigid objects was experimentally studied. Experiments in plane strain monoclinic flow were performed to model the fabric development of two populations of rectangular rigid objects with object aspect ratios (Rob) 2 and 3. The density of the rigid object populations was 14% of the total area. Objects were dispersed in a Newtonian and a non-Newtonian, power law matrix material with a power law exponent n of 1.2. The kinematic vorticity number (Wn) of the plane strain monoclinic flow was 1, 0.8 and 0.6 with finite simple shear strain of 4.6, 3.0 and 0.9, respectively. In experiments with Rob=3, the SPO is strongly influenced by Wn and the material properties of the matrix. Deformation of a power law matrix material and low Wn resulted in a stronger SPO than deformation of a linear viscous matrix and high Wn. Strain localization coupled with particle interaction plays a significant role in the development of a shape-preferred orientation. High strain simple shear zones separate trains of rigid objects that are surrounded by low strain zones with Wn lower than the bulk Wn. In fabrics involving populations of objects with Rob=2, rheology of the matrix materials does not systematically influence the intensity of the SPO. 相似文献