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841.
Milton A. Garcés Roger A. Hansen & Kent G. Lindquist 《Geophysical Journal International》1998,135(1):255-263
The tau– p method of Buland & Chapman (1983) is reformulated for sound waves propagating in a stratified atmosphere under the influence of a height-dependent wind velocity profile. For a given launch angle along a specified azimuth, the ray parameter is redefined to include the influence of the horizontal wind component along the direction of wave propagation. Under the assumption of negligible horizontal wind shear, the horizontal wind component transverse to the ray propagation does not affect the direction of the wave normal, but displaces the reference frame of the moving wavefront, thus altering the observed incidence azimuth. Expressions are derived for the time, horizontal range, and transverse range of the arriving waves as a function of ray parameter. Algorithms for the location of infrasonic wave sources using the modified tau– p formulation in conjunction with regional atmospheric wind and temperature data are discussed. 相似文献
842.
Using a relative rate method, rate constants have been measured for the gas-phase reactions of OH and NO3 radicals with pinonaldehyde, caronaldehyde and sabinaketone at 296 ± 2 K. The OH radical reaction rate constants obtained are (in units of 10–12 cm3 molecule–1 s–1): pinonaldehyde, 48 ± 8; caronaldehyde, 48 ± 8; and sabinaketone, 5.1 ± 1.4, and the NO3 radical reaction rate constants are (in units of 10–14 cm3 molecule–1 s–1): pinonaldehyde, 2.0 ± 0.9; caronaldehyde, 2.5 ± 1.1; and sabinaketone, 0.036 ± 0.023, where the error limits include the estimated overall uncertainties in the rate constants for the reference compounds. Upper limits to the O3 reaction rate constants were also obtained, of <2 × 10–20 cm3 molecule–1 s–1 for pinonaldehyde and caronaldehyde, and <5 × 10–20 cm3 molecule–1 s–1 for sabinaketone. These reaction rate constants are combined with estimated ambient tropospheric concentrations of OH radicals, NO3 radicals and O3 to calculate tropospheric lifetimes and dominant transformation process(es) of these and other monoterpene reaction products. 相似文献
843.
We present a simple virial-type extension to the modified Redlich-Kwong (MRK) equation for calculation of the volumes and fugacities of H2O and CO2 over the pressure range 0.001–50 kbar and 100 to 1400°C (H2O) and 100 to 1600°C (CO2). This extension has been designed to: (a) compensate for the tendency of the MRK equation to overestimate volumes at high pressures, and (b) accommodate the volume behaviour of coexisting gas and liquid phases along the saturation curve. The equation developed for CO2 may be used to derive volumes and fugacities of CO, H2, CH4, N2, O2 and other gases which conform to the corresponding states principle. For H2O the measured volumes of Burnham et al. are significantly higher in the range 4–10 kbar than those presented by other workers. For CO2 the volume behaviour at high pressures derived from published MRK equations are very different (larger volumes, steeper (P/T)V, and hence larger fugacities) from the virial-type equations of Saxena and Fei. Our CORK equation for CO2 yields fugacities which are in closer agreement with the available high pressure experimental decarbonation reactions. 相似文献
844.
From conductance measurements, the negative logarithm of the dissociation constant of the CaHCO3+ ion pair, pK(CaHCO3+), is 0.7, 1.0 and 1.35 within ±0.05 units at 0, 25 and 60°C, respectively. A revaluation of published and unpublished data yields pK(CaCO30) ≈ 3.2 at 25°C. Use of these pK's to compute the dissociation constant of calcite (Kc) from published calcite solubility measurements in pure water gives pKc values which increase markedly with ionic strength. However, if the ion pairs are ignored, computed pKc values are nearly constant with ionic strength. All reasonable attempts to eliminate the trend in pKc by adjusting ion activity coefficients, and/or values of K(CaCO30) failed, so the dilemma remains. Kc values computed from the most reliable published calcite solubility data are in good agreement with such values based on solubility data measured in this study at 5, 15, 35 and 50°C. Study results ignoring ion pairs are accurately represented by the equation log Kc = 13.870 — (3059/T) ?0.04035T, and correspond to ?8.35, ?8.42, and ?8.635 at 0, 25 and 50°C, respectively. The logarithmic expression leads to ΔHro = ?2420 ± 300 cal/mol, ΔCp = ?110 ± 2 cal/deg mol, and ΔSro = ?46.6 ± 1.0 cal/deg mol for the calcite dissociation reaction at 25°C. The dependence of Kc on temperature when CaCO30 and CaHCO3+ are assumed, is described by log Kc = 13.543 ? (3000/T) ? 0.0401T which yields ?8.39, ?8.47, and -8.70 at 0, 25 and 50°C. This gives ΔHro = ?2585 ± 300 cal/mol, ΔCp = ?109 ± 2 cal/deg mol, and ΔSr0 = ?47.4 ± 1.0 cal/deg mol at 25°C. 相似文献
845.
The paper reviews the methods described in the literature for the determination of total dissolved free primary amines (TDFPA) by fluorescence. A wide set of reaction conditions can be found, but they rely on few experiments for their validation. Among fluorogenic compounds, o-phthaldialdehyde (OPA) is more sensitive than fluorescamine and was thus examined here. However, the use of mercaptoethanol (ME) in the reaction (as an additional derivatization compound) is able to generate unreliable results, in particular when standardization relies on glycine. We suggest replacing ME with 3-mercaptopropionic acid (MPA) which induces more stable and comparable fluorescence among amine compounds. A systematic study was therefore undertaken to define reagent concentrations and pH effects on the reaction rates for a variety of primary amines with particular focus on amino acids. The reaction rate is increased by increasing OPA concentration and pH, but slowed by excess MPA. Ammonium interference is influenced by several factors, but spectral investigation showed that the choice of conditions can drastically reduce it. The magnitudes of natural and OPA-induced background fluorescence signals have been assessed in various mediums and it is shown that their contribution to the signal amounts to a large fraction, when not most, of the measured fluorescence. A segmented flow method is proposed with a protocol for adequate correction of biases. 相似文献
846.
The economic and human importance of the coastal zone, which is already considerable, is destined to increase rapidly as we near the next century. Owing to natural causes, compounded by anthropogenic actions, it is also under threat: erosion is steadily pushing back the shoreline. Tourism and shore recreation, major sources of income in the zone, are threatened. Various countermeasures have been taken, but often with disappointing results. Beach nourishment has shown great promise. The largest of such undertakings has recently been completed along a stretch of the Belgian coast. 相似文献
847.
Kathleen Crane Lynn Johnson Bruce Appelgate Clyde Nishimura Roger Buck Chris Jones Peter Vogt Rubin Kos’yan 《Marine Geophysical Researches》1997,19(4):319-338
On 21 May 1989, a major earthquake swarm on the Reykjanes Ridge at59°44 N, 29°32 W at a water depth of about 1000 m andabout 500 km southwest of Iceland was detected on both the WorldwideStandard Seismic Network (WWSSN) and Icelandic seismic networks. As part ofa multi-institutional response to this swarm, the Naval ResearchLaboratory arranged for a P3 Orion Aircraft to deploy sonobuoys and AXBTs inthe immediate vicinity of the swarm activity. The detection of the swarmmotivated a survey of the region in 1990, using the towed SeaMARC IIside-looking sonar system. In 1990–1991 the Russian ShirshovInstitute of Oceanology offered the use of its MIR deep-divingsubmersibles to investigate the rise axis for recent volcanism. During 1992,a scientific team comprised of five US and ten Russian scientists mobilizedthe twin, deep diving Russian submersibles to study the spreading axis ofthe Reykjanes Ridge. The resulting data analyses allows us to conclude thatthe 1989 seismic swarm event occurred adjacent to and east of the largeaxial high in the center of our survey area. The length, width and depthrange of the earthquakes were very similar to major seismic swarm eventsconfined to fissure systems in the Krafla region of Iceland. It is likelythat the earthquake swarm was located on a fresh, well-defined systemof fissures and faults extending south of the northernmost axial highstudied. The earthquake swarm was probably associated with an emanation oflava creating a region of high backscatter, located just to the east of thecentral axial high. In addition, the region of high-backscatterremains unsampled because it lay underneath the nadir of the processedSeaMARC tracks used to plan the submersible survey. However many sampleswere taken and structural studies of the evolving Reykjanes Ridge werecarried out. 相似文献
848.
Didier Jollivet Jean-Claude Faugeres Roger Griboulard Daniel Desbruyers Gerard Blanc 《Progress in Oceanography》1990,24(1-4)
Deep faunal assemblages were observed on cold seeps, between 1000 and 2000m depth, along the southern termination of the Barbados accretionary prism, during the Caracolante II and Diapicar cruises. Faunal composition and microdistribution of a cold seep community were analyzed at one site using deep-sea photographs and seismic (3.5 Kz) profiles. The community is dominated by large mussels up to 20cm long (possibly related to the genus Bathymodiolus), tiny vesicomyid clams, and vestimentiferan clusters in which animals are up to 2m long. There is a high density of sponges (three species), bryozoans and gorgonians. Other taxa occasionally associated with this assemblage include galatheid crabs, anemones, holothurians and possibly pennatulaceans which are numerous at boundaries of the site. A typical deep-sea fauna of fish, asteroids and ophiuroids is also scattered about the vicinity. This seep community is distributed as a band of discontinuous colonies, 40–50m in width and more than 10km in length. Living colonies alternate with accumulations shells and bare areas. The substratum is hard mud covered by a ferrugineous crust and cemented by carbonates. The early diagenetic character of the bottom and the occurrence of biological assemblages indicate that seepages of sulphur and/or methane, which have been revealed along the decollement zone of the Barbados prism, must diffuse through the sea floor. These biological and geological features are located on the crests of NE-SW anticlinal ridges and mud volcanoes which have been built by diaprism. 相似文献
849.
We analyze previously published geodetic data and intensity values for the M s = 8.1 Shillong (1897), M s = 7.8 Kangra (1905), and M s = 8.2 Nepal/Bihar (1934) earthquakes to investigate the rupture zones of these earthquakes as well as the amplification of ground motions throughout the Punjab, Ganges and Brahmaputra valleys. For each earthquake we subtract the observed MSK intensities from a synthetic intensity derived from an inferred planar rupture model of the earthquake, combined with an attenuation function derived from instrumentally recorded earthquakes. The resulting residuals are contoured to identify regions of anomalous intensity caused primarily by local site effects. Observations indicative of liquefaction are treated separately from other indications of shaking severity lest they inflate inferred residual shaking estimates. Despite this precaution we find that intensites are 1–3 units higher near the major rivers, as well as at the edges of the Ganges basin. We find evidence for a post-critical Moho reflection from the 1897 and 1905 earthquakes that raises intensities 1–2 units at distances of the order of 150 km from the rupture zone, and we find that the 1905 earthquake triggered a substantial subsequent earthquake at Dehra Dun, at a distance of approximately 150 km. Four or more M = 8 earthquakes are apparently overdue in the region based on seismic moment summation in the past 500 years. Results from the current study permit anticipated intensities in these future earthquakes to be refined to incorporate site effects derived from dense macroseismic data. 相似文献
850.
Adriana C. Flores-Díaz Roger Guevara Hernández Manuel E. Mendoza Rosario Langrave Alexander Quevedo Manuel Maass 《自然地理学》2018,39(2):118-139
Riparian systems have been included as a key component in ecosystem management because of their role in buffering the impact of land-use activities on fluvial systems. Riparian knowledge can be enhanced with a typology that reflects the multiple relationships occurring throughout the landscape. We propose a hierarchical procedure based on biophysical aspects for building local to regional typologies for guiding research and management, using the Cuitzmala River Basin as a case study. The variables involved were obtained from geospatial databases, water balances, and topographic profiles. The levels and variables are context (altitude, geoform [mountains/hills/plains], and runoff coefficient), structure (stream order, longitudinal slope, hydroperiod, and segment length), and microstructure (lateral slope, bankfull width, and length-to-width ratio). We consider humidity and functional gradient along the basin to identify groups of streams and fluvial networks. Inside each network, we described structural and microstructural features associated with riparian functions, linking them with management decisions. Therefore, the proposed hierarchical procedure can help in making riparian heterogeneity visible, focusing research and management goals, and allowing the recognition of a spatial dimension of the processes being studied. 相似文献