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61.
Martha Gledhill Constant M. G. van den Berg Rob F. Nolting Klaas R. Timmermans 《Marine Chemistry》1998,59(3-4)
Variations in the speciation of iron in the northern North Sea were investigated in an area covering at least two different water masses and an algal bloom, using a combination of techniques. Catalytic cathodic stripping voltammetry was used to measure the concentrations of reactive iron (FeR) and total iron (FeT) in unfiltered samples, while dissolved iron (FeD) was measured by GFAAS after extraction of filtered sea water. FeR was defined by the amount of iron that complexed with 20 μM 1-nitroso-2-napthol (NN) at pH 6.9. FeT was determined after UV-digestion at pH 2.4. Concentrations of natural organic iron complexing ligands and values for conditional stability constants, were determined in unfiltered samples by titration. Mean concentrations of 1.3 nM for FeR, 10.0 nM for FeT and 1.7 nM for FeD were obtained for the area sampled. FeR concentrations increased towards the south of the area investigated, as a result of the increased influence of continental run off. FeR concentrations were found to be enhanced below the nutricline (below 40 m) as a result of the remineralisation of organic material. Enhanced levels of FeT were observed in some surface samples and in samples collected below 30 m at stations in the south of the area studied, thought to be a result of high concentrations of biogenic particulate material and the resuspended sediments respectively. FeD concentrations varied between values similar to those of FeT in samples from the north of the area to values similar to those of FeR in the south. The bloom was thought to have influenced the distribution of both FeR and FeT, but less evidence was observed for any influence on FeR and FeD. The concentration of organic complexing ligands, which could possibly include a contribution from adsorption sites on particulate material, increased slightly in the bloom area and in North Sea waters. Iron was found to be fully (99.9%) complexed by the organic complexing ligands at a pH of 6.9 and largely complexed (82–96%) at pH 8. The ligands were almost saturated with iron suggesting that the ligand concentration could limit the concentration of iron occurring as dissolved species. 相似文献
62.
Klaas R. Timmermans Martha Gledhill Rob F. Nolting Marcel J. W. Veldhuis Hein J. W. de Baar Constant M. G.van den Berg 《Marine Chemistry》1998,61(3-4)
Short-term iron enrichment experiments were carried out with samples collected in areas with different phytoplankton activity in the northern North Sea and northeast Atlantic Ocean in the summer of 1993. The research area was dominated by high numbers of pico-phytoplankton, up to 70,000 ml−1. Maximum chlorophyll a concentrations varied from about 1.0 μg l−1 in a high-reflectance zone (caused by loose coccoliths, remnants from a bloom of Emiliania huxleyi) and about 3.5 μg l−1 in a zone in which the phytoplankton were growing, to about 0.5 μg l−1 in the northeast Atlantic Ocean. From the high-reflectance zone to the northeast Atlantic Ocean, nitrate concentrations increased from 0.5 μM to 6.0 μM. Concentrations of reactive iron in surface water showed an opposite trend and decreased from about 2.6 nM in the high-reflectance zone to <1.0 nM in the northeast Atlantic Ocean. In the research area, no signs of true iron deficiency were found, but iron enrichments in the high-reflectance zone, numerically dominated by Synechococcus sp., resulted in increased nitrate uptake. Ammonium uptake was hardly affected. Strong support for the effect of Fe on cell physiology is given by the increase in the f-ratio. Net growth rates of the phytoplankton (changes in cell numbers over 24 h) were almost unchanged. Phytoplankton collected from the northeast Atlantic Ocean, did not show changes in the nitrogen metabolism upon addition of iron. Net growth rates in these incubations were low or negative, with only slightly higher values with additional iron. 相似文献
63.
Replication of results is a basic tenet of science, but in palaeoecology this is very time-consuming and the ‘signal’ is subject to ‘noise’. The derivation of proxy-climate signals from ombrotrophic peat was carried out originally using samples from open peat faces where the stratigraphic relationships could be easily observed. Now that such sections are rare and often degraded there is a need to demonstrate that data can be replicated from core profiles. Ten short cores taken from two adjacent bogs have been analysed for macrofossils and show a coherent series of changes, which are also similar to previous profiles from the same sites. It is concluded that variation between profiles is slight and less than observations of present vegetation mosaics might suggest. Recommendations for a standard approach to fieldwork on raised bogs that emphasises the utility of subfossil pool layers are proposed and the need for a secure chronology is stressed. © 1998 John Wiley & Sons, Ltd. 相似文献
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Gravimetric monitoring of the first field‐wide steam injection in a fractured carbonate field in Oman – a feasibility study
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Marcin Glegola Pavel Ditmar Femke Vossepoel Rob Arts Fahad Al‐Kindy Roland Klees 《Geophysical Prospecting》2015,63(5):1256-1271
Gas‐Oil Gravity Drainage is to be enhanced by steam injection in a highly fractured, low permeability carbonate field in Oman. Following a successful pilot, field‐wide steam injection is being implemented, first of this type in the world. A dedicated monitoring program has been designed to track changes in the reservoir. Various observations are to be acquired, including, surface deformation, temperature measurements, microseismic, well logs, pressure and saturation measurements to monitor the reservoir. Because significant changes in the reservoir density are expected, time‐lapse gravimetry is also being considered. In this paper we investigate the feasibility of gravimetric monitoring of the thermally enhanced gravity drainage process at the carbonate field in Oman. For this purpose, forward gravity modelling is performed. Based on field groundwater measurements, the estimates of the hydrological signal are considered and it is investigated under what conditions the groundwater influences can be minimized. Using regularized inversion of synthetic gravity data, we analyse the achievable accuracy of heat‐front position estimates. In case of large groundwater variations at the field, the gravity observations can be significantly affected and, consequently, the accuracy of heat‐front monitoring can be deteriorated. We show that, by applying gravity corrections based on local observations of groundwater, the hydrological influences can to a large extent be reduced and the accuracy of estimates can be improved. We conclude that gravimetric monitoring of the heat‐front evolution has a great potential. 相似文献
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Turbidity currents descending the slopes of deep‐water extensional basins or passive continental margins commonly encounter normal‐fault escarpments, but such large‐magnitude phenomena are hydraulically difficult to replicate at small scale in the laboratory. This study uses advanced computational fluid dynamics numerical simulations to monitor the response of large, natural‐scale unconfined turbidity currents (100 m thick and 2000 m wide at the inlet gate) to normal‐fault topography with a maximum relief of nearly 300 m. For comparative purposes, the turbidity current is first released on a non‐faulted pristine slope of 1·5° (simulation model 1). The expanding and waxing flow bypasses the slope without recognizable deposition within the visibility limit of 8 vol.% sand grain packing. Similar flow is then released towards the tip (model 2) and towards the centre (model 3) of a normal‐fault escarpment. In both of these latter models, the sand carried by flow tends to be entrapped in four distinct depozones: an upslope near‐gate zone of flow abrupt expansion and self‐regulation; a flow‐transverse zone at the fault footwall edge; a flow‐transverse zone at the immediate hangingwall; and a similar transverse zone near the crest of the hangingwall counter‐slope, where some of the deposited sand also tends to be reshuffled to the previous zone by a secondary reverse underflow. The near‐bottom reverse flow appears to be generated on a counter‐slope of 1·1°, increased to 2·0° by deposition. The Kelvin–Helmholtz interface instability plays an important role by causing three‐dimensional fluctuations in the flow velocity magnitude and sediment concentration. The thick deposits of large single‐surge flows may thus show hydraulic fluctuations resembling those widely ascribed to hyperpycnal flows. The study indicates further that the turbiditic slope fans formed on such fault topographies are likely to be patchy and hence may differ considerably from the existing slope‐fan conceptual models when it comes to the spatial prediction of main sand depozones. 相似文献
69.
Vertical hydraulic gradient is commonly measured in rivers, lakes, and streams for studies of groundwater–surface water interaction. While a number of methods with subtle differences have been applied, these methods can generally be separated into two categories; measuring surface water elevation and pressure in the subsurface separately or making direct measurements of the head difference with a manometer. Making separate head measurements allows for the use of electronic pressure sensors, providing large datasets that are particularly useful when the vertical hydraulic gradient fluctuates over time. On the other hand, using a manometer-based method provides an easier and more rapid measurement with a simpler computation to calculate the vertical hydraulic gradient. In this study, we evaluated a wet/wet differential pressure sensor for use in measuring vertical hydraulic gradient. This approach combines the advantage of high-temporal frequency measurements obtained with instrumented piezometers with the simplicity and reduced potential for human-induced error obtained with a manometer board method. Our results showed that the wet/wet differential pressure sensor provided results comparable to more traditional methods, making it an acceptable method for future use. 相似文献
70.
Oliver B. Duffy Rob L. Gawthorpe Matthew Docherty Simon H. Brocklehurst 《Basin Research》2013,25(3):310-330
The Southern Tail‐End Graben, Danish Central Graben, is characterized by a lateral variation in the thickness and mobility of pre‐rift Zechstein Supergroup evaporites, allowing investigation of how supra‐basement evaporite variability influences rift structural style and tectono‐stratigraphy. The study area is divided into two structural domains based on interpretations of the depositional thickness and mobility of the Zechstein Supergroup. Within each domain, we examine the overall basin morphology and the structural styles in the pre‐Zechstein and supra‐Zechstein (cover) units. Furthermore, integration of two‐way travel‐time (TWT)‐structure and ‐thickness maps allows fault activity and evaporite migration maps to be generated for pre‐ and syn‐rift stratal units within the two domains, permitting constraints to be placed on: (i) the timing of activity on pre‐Zechstein and cover faults and (ii) the onset, duration and migration direction of mobile evaporites. The northern domain is interpreted to be free from evaporite‐influence, and has developed in a manner typical of brittle‐only, basement‐involved rifts. Syn‐rift basins display classical half‐graben geometries bounded by thick‐skinned faults. In contrast, the southern domain is interpreted to be evaporite‐influenced, and cover structure reflects a southward increase in the thickness and mobility of the Zechstein Supergroup evaporites. Fault‐related and evaporite‐related folding is prominent in the southern domain, together with variable degrees of decoupling of sub‐Zechstein and cover fault and fold systems. The addition of mobile evaporites to the rift results in: (i) complex and spatially variable modes of tectono‐stratigraphic evolution; (ii) syn‐rift stratal geometries which are condensed above evaporite swells and over‐thickened in areas of withdrawal; (iii) compartmentalized syn‐rift depocentres; and (iv) masking of rift‐related megasequence boundaries. Through demonstrating these deviations from the characteristics of rifts free from evaporite influence, we highlight the first order control evaporites may exert upon rift structural style and the distribution and thicknesses of syn‐rift units. 相似文献