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991.
G. M. da Costa E. Van San E. De Grave R. E. Vandenberghe V. Barrón L. Datas 《Physics and Chemistry of Minerals》2002,29(2):122-131
A novel method for synthesis of aluminium hematites, based upon the homogeneous precipitation of Fe and Al oxinates in various proportions, is presented. The precursor precipitates are heated in air at 700?°C. X-ray diffraction, thermal analyses, BET, FTIR, optical reflection analysis, TEM and Mössbauer spectroscopy at room temperature and 80?K of the resulting products indicate that single-phase hematites are formed with structural Al substitution of up to 10 at%. Interestingly, the particle size (>100?nm) is not substantially reduced by the Al content. Although it remains difficult to obtain a homogeneously distributed Al substitution in the final hematite, this processing line offers a unique opportunity to separate the effects of grain size and Al substitution on the Morin transition temperature (T M) of Al hematite. From the comparison between the present hematites and a series of Al-substituted hematites with lepidocrocite as precursor, it could be shown that the effect on T M, associated with a change of a factor 10 in grain size, is about 1/3 of the effect caused by a change of 10 in the degree of substitution. Finally, it is suggested that proper thermal treatments under different conditions of the same precursors are likely to produce spinel phases. 相似文献
992.
N. R. J. Poolton K. B. Ozanyan J. Wallinga A. S. Murray L. Bøtter-Jensen 《Physics and Chemistry of Minerals》2002,29(3):217-225
Most natural feldspars contain many charged impurities, and display a range of bond angles, distributed about the ideal.
These effects can lead to complications in the structure of the conduction band, giving rise to a tail of energy states (below
the high-mobility conduction band) through which electrons can travel, but with reduced mobility: transport through these
states is expected to be thermally activated. The purpose of this article is twofold. Firstly, we consider what kind of lattice
perturbations could give rise to both localized and extended conduction band-tail states. Secondly, we consider what influence
the band tails have on the luminescence properties of feldspar, where electrons travel through the sample prior to recombination.
The work highlights the dominant role that 0.04–0.05-eV phonons play in both the luminescence excitation and emission processes
of these materials. It also has relevance in the dating of feldspar sediments at elevated temperatures.
Received: 11 May 2001 / Accepted: 6 September 2001 相似文献
993.
994.
A. K. Varma R. M. Gairola A. K. Mathur B. S. Gohil Vijay K. Agarwal 《Journal of Earth System Science》2002,111(3):247-256
In this paper, MSMR geophysical products like Integrated Water Vapour (IWV), Ocean Surface Wind Speed (OWS) and Cloud Liquid
Water (CLW) in different grids of 50, 75 and 150 kms are compared with similar products available from other satellites like
DMSP-SSM/I and TRMMTMI. MSMR derived IWV, OWS and CLW compare well with SSM/I and TMI finished products. Comparison of MSMR
derived CLW with that derived from TMI and SSM/I is relatively in less agreement. This is possibly due to the use of 37 GHz
in SSM/I and TMI that is highly sensitive to CLW, while 37 GHz channels are not available on MSMR. Monthly comparison of MSMR
geophysical products with those from TMI is all carried out for climatological purpose. The monthly comparisons were much
better compared to instantaneous comparisons. In this paper, details of the data analysis and comparison results are presented.
The usefulness of the MSMR vis-à-vis other sensors is also discussed. 相似文献
995.
The fine structure of the FeI λ 532.4185-nm line of neutral iron is studied with high spatial (0.5″) and temporal (9.3 s) resolution using observations of a quiet region at the center of the solar disk. The character of the line asymmetry depends strongly on the nature of the velocity field, i.e., on whether it is due to convective or wave motions. The magnitude of the asymmetry due to acoustic waves is comparable to that due to convective motions. The propagation of acoustic waves in moving granules and intergranular lanes is studied by solving a system of hydrodynamical equations in a three-dimensional model for the solar atmosphere. The temporal variations in the bisector of the line synthesized in a non-LTE approximation agree well with the observational data. 相似文献
996.
Origin of spongy textures in clinopyroxene and spinel from mantle xenoliths, Hessian Depression, Germany 总被引:1,自引:0,他引:1
Summary Spongy textures are observed in anhydrous Group 1 mantle xenoliths (harzburgite, lherzolite and wehrlite) hosted in Tertiary
alkali basaltic lavas from the Hessian Depression, Germany. These textures are developed only on clinopyroxene and spinel,
and occur as rims or cross-cutting veinlets and patches showing optical continuity with the host grain. They are often associated
with pools of amorphous glassy material. There is no preferential development of spongy domains against the xenolith-lava
contact suggesting that the host magma did not play any significant role in their formation. Spongy clinopyroxene and spinel
occur in all rock types, but, are more pervasive in wehrlite.
Chemically, spongy domains of clinopyroxene and spinel are more refractory than unaffected areas, which is consistent with
their formation through a partial melting event. The associated glassy material shows chemical characteristics which suggest
that the melt pools are genetically related to the development of the spongy textures. The partial melting event was probably
triggered by the infiltration of a low-density fluid. The fluid may have evolved from a silicate melt responsible for the
metasomatic Fe-enrichment recorded in wehrlite. In this context, the more pervasive development of spongy clinopyroxene in
wehrlite may be explained by a higher concentration of the evolved fluid phase at proximity to its silicate melt source.
Received March 15, 2000; revised version accepted September 6, 2001 相似文献
997.
Validation of a fish farm waste resuspension model by use of a particulate tracer discharged from a point source in a coastal environment 总被引:2,自引:0,他引:2
Chris J. Cromey Thom D. Nickell Kenneth D. Black Paul G. Provost Colin R. Griffiths 《Estuaries and Coasts》2002,25(5):916-929
To validate a resuspension model of particulate material (salmonid farm wastes), a UV fluorescent particle tracer was selected with similar settling characteristics. Tracer was introduced to the seabed (water depth ≈30 m) and sediment samples taken on days 0, 3, 10, 17 and 30 to measure the horizontal and vertical distribution of tracer in sediments. A concentric sampling grid was established at radii of 25, 50, 100, 150, 200, 400, 700 and 1, 000 m from the source on transects 30° apart. The bulk of the deployed tracer was initially concentrated in an area 25 m radius from the release point; tracer was observed to steadily decrease to zero over a period of 30 days. In a 200 m region measured from the release point in the direction of the residual current, the redeposition of tracer was low. A Lagrangian particle tracking model was validated using these observed data by varying resuspension model parameters within limits to obtain the best agreement between spatial and temporal distributions. The validated model generally gave good predictions of total mass budgets (±7% of total tracer released), particulary where tracer concentrations were high near the release point. Best fit model parameters (critical erosion shear stress=0.018 N m−2, erodibility constan=60 g m−2 d−1) are at the low end of reported parameters for coastal resuspension models. Such a low critical erosion shear stress indicates that the frequency of resuspension and deposition events for freshly deposited material is high. 相似文献
998.
999.
1000.
I.N. Tolstikhin I.L. KamenskyB. Marty V.A. NivinV.R. Vetrin E.G. BalaganskayaS.V. Ikorsky M.A. GannibalD. Weiss A. VerhulstD. Demaiffe 《Geochimica et cosmochimica acta》2002,66(5):881-901
During the Devonian magmatism (370 Ma ago) ∼20 ultrabasic-alkaline-carbonatite complexes (UACC) were formed in the Kola Peninsula (north-east of the Baltic Shield). In order to understand mantle and crust sources and processes having set these complexes, rare gases were studied in ∼300 rocks and mineral separates from 9 UACC, and concentrations of parent Li, K, U, and Th were measured in ∼70 samples. 4He/3He ratios in He released by fusion vary from pure radiogenic values ∼108 down to 6 × 104. The cosmogenic and extraterrestrial sources as well as the radiogenic production are unable to account for the extremely high abundances of 3He, up to 4 × 10−9 cc/g, indicating a mantle-derived fluid in the Kola rocks. In some samples helium extracted by crushing shows quite low 4He/3He = 3 × 104, well below the mean ratio in mid ocean ridge basalts (MORB), (8.9 ± 1.0) × 104, indicating the contribution of 3He-rich plume component. Magnetites are principal carriers of this component. Trapped 3He is extracted from these minerals at high temperatures 1100°C to 1600°C which may correspond to decrepitation or annealing primary fluid inclusions, whereas radiogenic 4He is manly released at a temperature range of 500°C to 1200°C, probably corresponding to activation of 4He sites degraded by U, Th decay.Similar 4He/3He ratios were observed in Oligocene flood basalts from the Ethiopian plume. According to a paleo-plate-tectonic reconstruction, 450 Ma ago the Baltica (including the Kola Peninsula) continent drifted not far from the present-day site of that plume. It appears that both magmatic provinces could relate to one and the same deep-seated mantle source.The neon isotopic compositions confirm the occurrence of a plume component since, within a conventional 20Ne/22Ne versus 21Ne/22Ne diagram, the regression line for Kola samples is indistinguishable from those typical of plumes, such as Loihi (Hawaii). 20Ne/22Ne ratios (up to 12.1) correlate well with 40Ar/36Ar ones, allowing to infer a source 40Ar/36Ar ratio of about 4000 for the mantle end-member, which is 10 times lower than that of the MORB source end-member. In (3He/22Ne)PRIM versus (4He/21Ne)RAD plot the Kola samples are within array established for plume and MORB samples; almost constant production ratio of (4He/21Ne)RAD ≅ 2 × 107 is translated via this array into (3He/22Ne)PRIM ∼ 10. The latter value approaches the solar ratio implying the non-fractionated solar-like rare gas pattern in a plume source.The Kola UACC show systematic variations in the respective contributions of in situ-produced radiogenic isotopes and mantle-derived isotopes. Since these complexes were essentially plutonic, we propose that the depth of emplacement exerted a primary control on the retention of both trapped and radiogenic species, which is consistent with geological observations. The available data allow to infer the following sequence of processes for the emplacement and evolution of Kola Devonian UACC: 1) Ascent of the plume from the lower mantle to the subcontinental lithosphere; the plume triggered mantle metasomatism not later than ∼700 to 400 Ma ago. 2) Metasomatism of the lithosphere (beneath the central part of the Kola Peninsula), including enrichment in volatile (e.g., He, Ne) and in incompatible (e.g., U, Th) elements. 3) Multistage intrusions of parental melts, their degassing, and crystallisation differentiation ∼370 Ma ago. 4) Postcrystallisation migration of fluids, including loss of radiogenic and of trapped helium. Based on model compositions of the principle terrestrial reservoirs we estimate the contributions (by mass) of the plume material, the upper mantle material, and the atmosphere (air-saturated groundwater), into the source of parent melt at ∼2%, 97.95%, and ∼0.05%, respectively. 相似文献