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41.
Chantal M. Swan David A. Siegel Norman B. Nelson Craig A. Carlson Elora Nasir 《Deep Sea Research Part I: Oceanographic Research Papers》2009,56(12):2175-2192
Recent in situ observations of chromophoric dissolved organic material (CDOM) in the Pacific Ocean reveal the biogeochemical controls on CDOM and indicate predictive potential for open-ocean CDOM in diagnosing particulate organic matter (POM) remineralization rates within ocean basins. Relationships between CDOM and concentrations of dissolved oxygen, nutrients and inorganic carbon in the subthermocline waters of the Pacific reflect the relative influences of water mass ventilation and water-column oxidative remineralization. Apparent in situ oxygen utilization (AOU) accounts for 86% and 61% of variance in CDOM abundance, respectively, in Antarctic Intermediate Water and North Pacific Intermediate Water. In the deep waters of the Pacific below the zone of remineralization, AOU explains 26% of CDOM variability. The AOU–CDOM relationship results from competing biogeochemical and advective processes within the ocean interior. Dissolved organic carbon (DOC) is not statistically linked to the CDOM or AOU distributions, indicating that the majority of CDOM production occurs during the remineralization of sinking POM and thus potentially provides key information about carbon export. Once formed in the ocean interior, CDOM is relatively stable until it reaches the surface ocean where it is destroyed by solar bleaching. Susceptibility to bleaching confers an additional tracer-like quality for CDOM in water masses with active convection, such as mode waters that appear as subsurface CDOM minima. In the surface ocean, atypically low CDOM abundance highlights a region of unusually extreme oligotrophy: the subtropical South Pacific gyre. For these hyper-oligotrophic waters, the present CDOM observations are consistent with analysis of in situ radiometric observations of light attenuation and reflectance, demonstrating the accuracy of the CDOM spectrophotometric observations. Overall, we illustrate how CDOM abundance in the ocean interior can potentially diagnose rates of thermohaline overturning as they affect regional biogeochemistry and export. We further show how relative surface ocean CDOM abundances are driven in large part by processes occurring in the deep layers of the ocean. This is particularly significant for the interpretation of the global surface distribution of CDOM using satellite remote sensing. 相似文献
42.
Ionization fronts, the sharp radiation fronts behind which H/He ionizing photons from massive stars and galaxies propagate
through space, were ubiquitous in the universe from its earliest times. The cosmic dark ages ended with the formation of the
first primeval stars and galaxies a few hundred Myr after the Big Bang. Numerical simulations suggest that stars in this era
were very massive, 25–500 solar masses, with H(II) regions of up to 30,000 light-years in diameter. We present three-dimensional
radiation hydrodynamical calculations that reveal that the I-fronts of the first stars and galaxies were prone to violent
instabilities, enhancing the escape of UV photons into the early intergalactic medium (IGM) and forming clumpy media in which
supernovae later exploded. The enrichment of such clumps with metals by the first supernovae may have led to the prompt formation
of a second generation of low-mass stars, profoundly transforming the nature of the first protogalaxies. Cosmological radiation
hydrodynamics is unique because ionizing photons coupled strongly to both gas flows and primordial chemistry at early epochs,
introducing a hierarchy of disparate characteristic timescales whose relative magnitudes can vary greatly throughout a given
calculation. We describe the adaptive multistep integration scheme we have developed for the self-consistent transport of
both cosmological and galactic ionization fronts. 相似文献
43.
Claudio Marchesi William L. Griffin Carlos J. Garrido Jean-Louis Bodinier Suzanne Y. O’Reilly Norman J. Pearson 《Contributions to Mineralogy and Petrology》2010,159(3):315-330
The western part of the Ronda peridotite massif (Southern Spain) consists mainly of highly foliated spinel-peridotite tectonites
and undeformed granular peridotites that are separated by a recrystallization front. The spinel tectonites are interpreted
as volumes of ancient subcontinental lithospheric mantle and the granular peridotites as a portion of subcontinental lithospheric
mantle that underwent partial melting and pervasive percolation of basaltic melts induced by Cenozoic asthenospheric upwelling.
The Re–Os isotopic signature of sulfides from the granular domain and the recrystallization front mostly coincides with that
of grains in the spinel tectonites. This indicates that the Re–Os radiometric system in sulfides was highly resistant to partial
melting and percolation of melts induced by Cenozoic lithospheric thermal erosion. The Re–Os isotopic systematics of sulfides
in the Ronda peridotites thus mostly conserve the geochemical memory of ancient magmatic events in the subcontinental lithospheric
mantle. Os model ages record two Proterozoic melting episodes at ~1.6 to 1.8 and 1.2–1.4 Ga, respectively. The emplacement
of the massif into the subcontinental lithospheric mantle probably coincided with one of these depletion events. A later metasomatic
episode caused the precipitation of a new generation of sulfides at ~0.7 to 0.9 Ga. These Proterozoic Os model ages are consistent
with results obtained for several mantle suites in Central/Western Europe and Northern Africa as well as with the Nd model
ages of the continental crust of these regions. This suggests that the events recorded in mantle sulfides of the Ronda peridotites
reflect different stages of generation of the continental crust in the ancient Gondwana supercontinent. 相似文献
44.
On 16 July 1945, the first atomic bomb was detonated at the Alamogordo Bombing range in New Mexico, USA. Swept up into the nuclear cloud was the surrounding desert sand, which melted to form a green glassy material called ‘trinitite’. Contained within the glass are melted bits of the first atomic bomb and the support structures and various radionuclides formed during the detonation. The glass itself is marvelously complex at the tens to hundreds of micrometre scale, and besides glasses of varying composition also contains unmelted quartz grains. Air transport of the melted material led to the formation of spheres and dumbbell shaped glass particles. Similar glasses are formed during all ground level nuclear detonations and contain forensic information that can be used to identify the atomic device. 相似文献
45.
Ekaterina P. Reguir Alfredo Camacho Panseok Yang Anton R. Chakhmouradian Vadim S. Kamenetsky Norman M. Halden 《Mineralogy and Petrology》2010,100(3-4):95-103
The U-Pb geochronology of perovskite is a powerful tool in constraining the emplacement age of silica-undersaturated rocks. The trace-element and U-Pb isotopic compositions of perovskite from clinopyroxenite and silicocarbonatite from the Afrikanda plutonic complex (Kola, Russia) were determined by laser-ablation inductively-coupled mass-spectrometry (LA-ICP-MS). In addition, the Sr isotopic composition of perovskite was measured by isotope-dilution mass-spectrometry to better constrain the relations between its host rocks. Perovskite from the two rock types shows a different degree of enrichment in Na, Mg, Mn, Pb, Fe, Al, V, rare-earth elements, Zr, Hf, Th, U and Ta. The perovskite 87Sr/86Sr values are within analytical uncertainty of one another and fall within the range of mantle values. The 206Pb/238U ages (corrected for common lead using 207Pb-method) of perovskite from silicocarbonatite statistically yield a single population with a weighted mean of 371?±?8 Ma (2σ; MSWD?=?0.071). This age is indistinguishable, within uncertainty, to the clinopyroxenite weighted mean 206Pb/238U age of 374?±?10 Ma (2σ; MSWD?=?0.18). Our data are in good agreement with the previous geochronological study of the Afrikanda complex. The observed variations in trace-element composition of perovskite from silicocarbonatite and clinopyroxenite indicate that these rocks are not related by crystal fractionation. The Sr isotopic ratios and the fact that the two rocks are coeval suggest that they were either produced from a single parental melt by liquid immiscibility, or from two separate magmas derived at different degrees of partial melting from an isotopically equilibrated, but modally complex mantle source. 相似文献
46.
Water is an invaluable resource, and equitable access to it is a fundamental human right. Disenfranchised groups often lose access to water resources because their interests are not well represented by decision makers. Excluding these groups from resource management policy often results in myopic decisions that contribute to further ecosystem damage. We describe the ecological degradation of Lake Urmia in Iran, which has recently experienced increased salinity and declining water quantity. The lake is a UNESCO Biosphere Reserve and Ramsar site, and supports unique biodiversity in the region. The lake's decline is driven by the destruction of Zagros forests and the government's water policies, which diverted water to more politically connected agricultural land users, increasing social inequity and prompting more deforestation. The most straightforward restoration solution is to discontinue the diversions and allow critical inflows to recharge Lake Urmia, preserving the lake and wetlands for migratory birds, tourists, and local communities. 相似文献
47.
Many previous investigations of mean streamwater transit times (MTT) have been limited by an inability to quantify the MTT dynamics. Here, we draw on (1) a linear relation (r 2 = 0.97) between groundwater 3H/3He ages and dissolved silica (Si) concentrations, combined with (2) predicted streamwater Si concentrations from a multiple-regression relation (R 2 = 0.87) to estimate MTT at 5-min intervals for a 23-year time series of streamflow [water year (WY) 1986 through 2008] at the Panola Mountain Research Watershed, Georgia. The time-based average MTT derived from the 5-min data was ~8.4 ± 2.9 years and the volume-weighted (VW) MTT was ~4.7 years for the study period, reflecting the importance of younger runoff water during high flow. The 5-min MTTs are normally distributed and ranged from 0 to 15 years. Monthly VW MTTs averaged 7.0 ± 3.3 years and ranged from 4 to 6 years during winter and 8–10 years during summer. The annual VW MTTs averaged 5.6 ± 2.0 years and ranged from ~5 years during wet years (2003 and 2005) to >10 years during dry years (2002 and 2008). Stormflows are composed of much younger water than baseflows, and although stormflow only occurs ~17 % of the time, this runoff fraction contributed 39 % of the runoff during the 23-year study period. Combining the 23-year VW MTT (including stormflow) with the annual average baseflow for the period (~212 mm) indicates that active groundwater storage is ~1,000 mm. However, the groundwater storage ranged from 1,040 to 1,950 mm using WY baseflow and WY VW MTT. The approach described herein may be applicable to other watersheds underlain by granitoid bedrock, where weathering is the dominant control on Si concentrations in soils, groundwater, and streamwater. 相似文献
48.
José María González-Jiménez Carlos Villaseca William L. Griffin Suzanne Y. O’Reilly Elena Belousova Eumenio Ancochea Norman J. Pearson 《Contributions to Mineralogy and Petrology》2014,168(2):1-24
Spinel lherzolite and wehrlite xenoliths from the Cenozoic Calatrava volcanic field carry the geochemical imprint of metasomatic agents that have affected the subcontinental lithospheric mantle beneath Central Iberia. Some xenoliths (mainly wehrlites) were enriched in REE, Sr, P, and CO2 by silicic-carbonate-rich metasomatic melts/fluids, while others record the effects of subduction-related hydrous silicate fluids that have precipitated amphibole and induced high Ti/Eu in primary clinopyroxene. The petrographic observations and geochemical data suggest that interstitial glass in the xenoliths represent the quenched products of Si-rich melts that infiltrated the mantle peridotite shortly before the entrainment of the xenoliths in the host magmas that erupted ca 2 million years ago. During their infiltration, the metasomatic melts reacted with peridotite, resulting in silica enrichment, while remobilizing grains of iron-rich monosulfide solid solution (Fe-rich Mss) initially enclosed in, or intergranular to, primary olivine and pyroxenes. In situ laser ablation inductively coupled plasma-mass spectrometry analysis of single sulfide grains reveals that the Fe-rich Mss in glass shows platinum-group element (PGE) patterns and 187Os/188Os compositions identical to the Fe-rich Mss occurring as inclusions in, or at grain boundaries of primary silicates. Moreover, independent of its microstructural position, Fe-rich Mss exhibits PGE and 187Os/188Os signatures typical of Mss either residual after partial melting or crystallized directly from sulfide melts. Our findings reveal that young metasomatic melt(s)/fluid(s) may carry remobilized sulfides with PGE and Os-isotopic signatures identical to those of texturally older sulfides in the peridotite xenolith. These sulfides thus still provide useful information about the timing and nature of older magmatic events in the subcontinental mantle. 相似文献
49.
50.
Douglas S. Hall Gregory W. Henry Dietmar Böhme Peter A. Brooks Sandy Chang Ales Dolzan George L. Fortier Robert E. Fried Russell M. Genet Bruce S. Grim James Hannon Darrel B. Hoff Kevin Krisciunas Howard J. Landis Howard P. Louth Larry P. Lovell Paul Nielsen Bobby E. Powell Harry D. Powell Don Pray Thomas R. Renner Charles W. Rogers Stephen Shervais Douglas M. Slauson Samuel Slote Harold J. Stelzer Arthur J. Stokes Jack C. Troeger Louis C. Turner Norman F. Wasson Kenneth W. Zeigler 《Journal of Astrophysics and Astronomy》1991,12(4):281-287
We present photoelectric photometry of λ And never before published, obtained between February 1982 and December 1990 at 29
different observatories. Then we combine it with all other photometry available to us (previously published, contained in
the I.A.U. Commission 27 Archives, and obtained with the Vanderbilt 16-inch automatic telescope but not yet published), to
yield a 14.8-year data base. Analysis reveals a long-term cycle in mean brightness, with a full range of 0m.15 and a period of 11.4 ± 0.4 years. Because most of our new photometry was concentrated in the 1983-84 observing season,
we analyze that one well-defined light curve with a two-spot model. Spot A keeps a 0m.04 amplitude throughout four rotation cycles whereas the amplitude of spot B diminishes from 0m.09 down almost to 0m.03. The spot rotation periods were 55d.9 ± 0d.6 and 520d.8 ± 1d.0, respectively. 相似文献