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221.
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Interstitial water samples were collected from the Guatemala Basin using an in situ sampler and by centrifuging box core sediment samples. Results from these two sampling methods for Mn, Si, PO4 agree well. There is a systematic difference in the alkalinity values, however, which suggests that CaCO3 (s) precipitates from the box core samples when they are brought from in situ pressure at 1 atm. Thus the alkalinity on box core samples is less than that on samples collected in situ. The magnitude of the alkalinity decrease can be calculated using basic thermodynamic principles and the observed and predicted differences agree well.Both sampling methods show a sharp drop in pH just below the sediment water interface which can be explained by the oxidation of organic matter by O2 in the absence of CaCO3. Alkalinity increases during the reduction of MnO2(s) and release of Mn2+ to the interstitial water. The result is that interstitial waters become undersaturated with CaCO3 immediately below the sediment/water interface and then return to or nearly to saturation at depth. 相似文献
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Surface chemistry concepts developed for heterogeneous oxide surfaces are illustrated with Cu, Cd, and Zn adsorption data on a well defined, model surface—goethite (αFeOOH)—and then applied to define the interaction or Zn with interfacial sediments from the Guatemala Basin at MANOP site H.Apparent equilibrium binding constants which describe metal associations with a surface, whose sites are composed of a spectrum of binding energies, are independent of adsorption density when sites are available in excess, but dependent on adsorption density when sites are limited. This conclusion makes it especially important to properly apply laboratory experimental results to describe adsorption processes in the natural environment. Therefore, a means for estimating the maximum adsorption density of an element on natural particles is discussed and used to estimate the quantity of Zn in interfacial sediments at MANOP site H which can be ascribed to the process of adsorption. 相似文献
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The coastal bays and lagoons of Maryland extend the full length of the state's Atlantic coast and compose a substantial ecosystem at the land-sea margin that is characterized by shallow depth, a well-mixed water column, slow exchange with the coastal ocean, and minimal freshwater input from the land. For at least 25 years, various types of measurements have been made intermittently in these systems, but almost no effort has been made to determine if water quality or habitat conditions have changed over the years or if distinctive spatial gradients in these features have developed in response to changing land uses. The purpose of this work was to examine this fragmented database and determine if such patterns have emerged and how they may be related to land uses. Turbidity, dissolved inorganic phosphate, algal biomass, and primary production rates in most areas of the coastal bays followed a regular seasonal pattern, which was well correlated with water temperature. Nitrate concentrations were low (<5 μM), and only modestly higher in tributary creeks (<20 μM). Additionally, there was little indication of the spring bloom typical of river-dominated systems. There does appear to be a strong spatial gradient in water quality conditions (more eutrophic in the upper bays, especially in tributary creeks). Comparisons of water quality data collected between 1970 and 1991 indicate little temporal change in most areas and some small improvements in a few areas, probably related to decreases in point-source discharges. Seagrass communities were once extensive in these systems but at present are restricted to the eastern portion of the lower bays where water clarity is sufficient to support plant survival. Even in these areas, seagrass densities have recently decreased. Examination of diel dissolved oxygen data collected in the summer indicates progressively larger diel excursions from lower to upper bays and from open bays to tributary subsystems; however, hypoxic conditions (<2 mg 1?1) were rarely observed in any location. Nitrogen input data (point, surface runoff, groundwater and atmospheric deposition to surface waters) were assembled for seven regions of the coastal bay system; annual loading rates ranged from 2.4 g N m?2 yr?1 to 39.7 g N m?2 yr?1. Compared with a sampling of loading rates to other coastal systems, those to the upper and lower bays were low while those to tributaries were moderate to high. Regression analysis indicated significant relationships between annual nitrogen loading rates and average annual total nitrogen and chlorophyll a concentrations in the water column. Similar analyses also indicated significant relationships between chlorophyll a and the magnitude of diel dissolved oxygen changes in the water column. It is concluded that these simple models, which could be improved with a well-designed monitoring program, could be used as quantitative management tools to relate habitat conditions to nutrient loading rates. 相似文献
227.
An episode of high lake levels prior to the last maximum glaciation has been identified at many localities in wastern Australia. Similar events have been recognized at playa lakes in central Australia, where gypsum dunes along playa margins formed during one or more episodes of high groundwater discharge, with a large influx of calcium sulphate.At Lake Lewis, exposures at two islands show similar sediment sequences: three pedogenic gypcrete layers interbedded with aeolian quartz and gypsum sand horizons form three units within gypsum dunes up to 7 m high. The lowest unit has cliffed edges buried by the upper units, indicating a significant time break. Four TL dates (coarse-grained quartz) show that this lowest unit was deposited at or before 70–80 ka. The middle unit of mixed gypsum and quartz sand capped by gypcrete represents the major phase of gypsum dune formation, and 6 TL dates range from 33 to 46 ka with overlapping error bars. These are slightly younger but statistically similar to TL dates (from 39 to 59 ka) of the shoreline gypsum dune at Lake Amadeus in the same region. The top unit of the two islands, up to 1 m thick, has not yet been well dated. One date is inconsistent with the well dated middle layer below, possibly because of incomplete bleaching, and has been rejected. The other date (17 ± 5 ka) is much younger which possibly indicates a minor and local reactivation of old gypsum sediments. At the lake margin, there are quartz dunes overlying the gypsum dunes, and a buried aeolian quartz sand layer occurs in a lake-margin terrace. These represent reactivation of the regional quartz dune field after the major gypsum dune formation. Two consistent TL dates (21 ± 4 ka and 23 ± 6 ka) indicate that regional dunes were active at about the time of the Last Glacial Maximum. 相似文献
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229.
Chapman M 《GeoJournal》1987,15(4):347-365
The context for this paper is the nature of generalization deriving from the study of particular cases of human behaviour. With specific reference to field research on population movement conducted amongst individuals, households, small groups, and village communities in third world societies, it challenges the convention that both generalization and extrapolation are based inevitably and exclusively on the number of cases or events subject to examination. An evaluation is made of the methodological aspects of four different studies of population mobility at microscale, undertaken between 1965 and 1977 in the Solomon Islands and northwest Thailand. On this basis, integrated field designs that incorporate a range of intersecting instruments are favoured for their technical flexibility and logical strength. With case studies of third world villages, market centres, and urban neighbourhoods, generalization and extrapolation is based on depth of understanding and the power of theoretical connections. 相似文献
230.
Rainfall samples were collected from several hundred rainfall events. Up to nine samples per event were collected from sites 3–500 m apart. They differed substantially in both concentration and composition, even though great care was taken to wash all collectors beforehand. Dryfall, storage and analytical procedures could not explain the variation. When data for rainfall events of similar size (but very different cation inputs) were examined, the major differences were associated with the prevailing wind direction. Events leading to high concentrations were associated with easterly winds and showed the influence of a marine source. Chemical concentration and composition were not altered by the occurrence of a drought year followed by a very wet year. The mean pH was 5·3 and ranged from 4·6 to 5·8. For a given event, a difference of 0·5 often occurred between collection sites. Regular seasonal variations in the concentration of NO3-N and the NO3/NH4 ratio occurred, with the ratio being higher in summer due primarily to bush fires. Organic nitrogen comprised 14% of total nitrogen. 相似文献