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Jasmine Rita Petriglieri Christine Laporte-Magoni Peggy Gunkel-Grillon Mario Tribaudino Danilo Bersani Orietta Sala Monika Le Mestre Ruggero Vigliaturo Nicola Bursi Gandolfi Emma Salvioli-Mariani 《地学前缘(英文版)》2020,11(1):189-202
Covered by ultrabasic units for more than a third of its surface,the New Caledonia(South West Pacific)is one of the largest world producers of Ni-ore from lateritic deposits.Almost all outcrops of geological units and open mines contain serpentine and amphibole,also as asbestos varieties.In this geological context,in which weathering processes had a great contribution in the production and dispersion of mineral fibres into the environment,the development of a routinely analytical strategy,able to discriminate an asbestiform fibre from a non-harmful particle,is a pivotal requisite.However,the acquisition of all these parameters is necessary for determining the risk associated to fibres exposition.A multidisciplinary routinely approach,based on the use of complementary simply-to-use but reliable analytical methods is the only possible strategy.In addition,the instrumental apparatus must be easily transportable on the field,directly on the mining site.The employment of specialized tools such as Polarized Light Microscopy associated to Dispersion Staining method(PLM/DS)and portable Raman spectroscopy for identification of environmental asbestos,are proved extremely effective in the improvement of the performance and rapidity of data acquisition and interpretation.Both PLM/DS and handheld Raman devices confirmed to be discriminant in the detection and characterization of asbestos fibres for both serpentine and amphibole.Furthermore,these techniques proved extremely effective even in the presence of strongly fibrous and altered samples. 相似文献
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Monika Nausch Günther Nausch Hans Ulrich Lass Volker Mohrholz Klaus Nagel Herbert Siegel Norbert Wasmund 《Estuarine, Coastal and Shelf Science》2009,83(4):434-442
In July 2007, phosphorus input by an upwelling event along the east coast of Gotland Island and the response of filamentous cyanobacteria were studied to determine whether introduced phosphorus can intensify cyanobacterial bloom formation in the eastern Gotland Basin. Surface temperature, nutrient concentrations, phytoplankton biomass and its stoichiometry, as well as phosphate uptake rates were determined in two transects between the coasts of Gotland and Latvia and in a short grid offshore of Gotland. In the upwelling area, surface temperatures of 11–12 °C and average dissolved inorganic phosphorus (DIP) concentrations of 0.26 μM were measured. Outside the upwelling, surface temperatures were higher (15.5–16.6 °C) and DIP supplies in the upper 10 m layer were exhausted. Nitrite and nitrate concentrations (0.01–0.22 μM) were very low within and outside the upwelling region. Abundances of filamentous cyanobacteria were highly reduced in the upwelling area, accounting for only 1.4–6.0% of the total phytoplankton biomass, in contrast to 18–20% outside the upwelling. The C:P ratio of filamentous cyanobacteria varied between 32.8 and 310 in the upwelling region, most likely due to the introduction of phosphorus-depleted organisms into the upwelling water. These organisms accumulate DIP in upwelling water and have lower C:P ratios as long as they remain in DIP-rich water. Thus, diazotrophic cyanobacteria benefit from phosphorus input directly in the upwelling region. Outside the upwelling region, the C:P ratios of filamentous cyanobacteria varied widely, between 240 and 463, whereas those of particulate material in the water ranged only between 96 and 224. To reduce their C:P ratio from 300 to 35, cyanobacteria in the upwelling region had to take up 0.05 mmol m−3 DIP, which is about 20% of the available DIP. Thus, a larger biomass of filamentous cyanobacteria may be able to benefit from a given DIP input. As determined from the DIP uptake rates measured in upwelling cells, the time needed to reduce the C:P ratio from 300 to 35 was too long to explain the huge bloom formations that typically occur in summer. However, phosphorus uptake rates increased significantly with increasing C:P ratios, allowing phosphorus accumulation within 4–5 days, a span of time suitable for bloom formation in July and August. 相似文献
64.
Diatom and chrysophyte cyst-based reconstructions of the dates of spring and autumn lake-mixing enabled us to estimate spring
(STanom) and autumn (ATanom) temperature anomalies as well as ice-cover of the last ca. 4,000 years in a lake sediment core (Oberer Landschitzsee, 2,076
m a.s.l.) from the southern slopes of the Austrian Central Alps. The two independently inferred temperature anomalies were
significantly correlated. On average, spring and autumn temperatures were lower during the two millennia B.C than during 0–1,300
A.D. Marked spring and autumn temperature minima occurred at about 1,300 and 600 B.C. At about 1,300 A.D, STanom declined again. Spring-temperature anomalies during Roman and Medieval times equaled or slightly exceeded the modern values
and paralleled tree-line and glacier fluctuations. The de-coupling of autumn and spring climates, which began during the Medieval
period, might indicate changes in major circulation modes. It was assumed that the North-Atlantic influence, triggering winter-rain
climate in the Northern Mediterranean, became weaker during Medieval times, resulting in a trend towards warmer autumns and
overall more continental climate conditions in the study area. Four pulses of land use, inferred from indicator pollen, occurred
during (1) the Early to Late Bronze, (2) the transition from Late Bronze to Early Iron Age (Hallstatt), (3) Late Iron Age
(La Tène, Celtic time) to Roman times, and (4) during high to late Medieval times. Climate seemed to be an important, though
complex, trigger of Alpine land use. 相似文献
65.
In the upwelling area along the Namibian coast of SW-Africa sulphur discolorations were investigated to study the impact of hydrogen sulphide on the ecosystem using satellite imagery. The formation of colloidal sulphur in the upper water layer results from the oxidation of hydrogen sulphide. The occurrence of sulphur plumes as well as their temporal and spatial development was investigated in relation to the driving meteorological and oceanographic conditions. Because of the sporadic occurrence of sulphur events and the limited number of ship-borne investigations in that area remote sensing of ocean colour is the only method to follow these phenomena continuously and synoptically. In the past the sulphur plumes were studied by true colour images derived from ocean colour satellite data like sea-viewing wide field of view sensor or moderate resolution imaging spectroradiometer and identified by their typical milky turquoise discoloration. 相似文献
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Differently colored natural Brazilian andalusite crystals heat-treated under reducing and oxidizing conditions were analyzed
by optical spectroscopy. The intensity of a broad intense band at around 20,500 cm−1 in the optical absorption spectra of all color zones of the sample is proportional to the product of Ti- and Fe-concentrations
and herewith proves its attribution to electronic Fe2+/Ti4+ IVCT transition. The band is strictly E||c-polarized, causing an intense red coloration of the samples in this polarization. The polarization of the Fe2+/Ti4+ IVCT band in andalusite, E||c, shows that the electronic charge-transfer process takes place in Al–O octahedral groups that share edges with neighbors
on either side, forming chains parallel to the c-axis of the andalusite structure. Under thermal treatments in air, the first noticeable change is some intensification of
the band at 800°C. However, at higher temperatures its intensity decreases until it vanishes at 1,000°C in lightly colored
zones and 1,100°C in darkly colored ones. Under annealing in reducing conditions at 700 and 800°C, the band also slightly
increases and maintains its intensity at treatments at higher temperatures up to 1,000°C. These results demonstrate that weakening
and disappearance of the Fe2+/Ti4+ IVCT band in spectra of andalusite under annealing in air is caused by oxidization of Fe2+ to Fe3+ in IVCT Fe2+/Ti4+-pairs. Some intensification of the band at 800°C is, most probably, due to thermally induced diffusion of Fe2+ and Ti4+ in the structure that leads to aggregation of “isolated” Ti4+ and Fe2+ ions into Fe2+–Ti4+-pairs. At higher temperatures, the competing process of Fe2+ → Fe3+ oxidation overcomes such “coupling” and the band continues to decrease. The different thermal stability of the band in lightly
and darkly colored zones of the samples evidence some self-stabilization over an interaction of Fe2+/Ti4+-pairs involved in IVCT process. 相似文献
69.
Martin Danišík Jaroslav Kadlec Christoph Glotzbach Anett Weisheit István Dunkl Milan Kohút Noreen J. Evans Monika Orvošová Brad J. McDonald 《Swiss Journal of Geoscience》2011,104(2):285-298
A combination of four thermochronometers [zircon fission track (ZFT), zircon (U–Th)/He (ZHe), apatite fission track (AFT)
and apatite (U–Th–[Sm])/He (AHe) dating methods] applied to a valley to ridge transect is used to resolve the issues of metamorphic,
exhumation and topographic evolution of the Nízke Tatry Mts. in the Western Carpathians. The ZFT ages of 132.1 ± 8.3, 155.1 ± 12.9,
146.8 ± 8.6 and 144.9 ± 11.0 Ma show that Variscan crystalline basement of the Nízke Tatry Mts. was heated to temperatures
>210°C during the Mesozoic and experienced a low-grade Alpine metamorphic overprint. ZHe and AFT ages, clustering at ~55–40
and ~45–40 Ma, respectively, revealed a rapid Eocene cooling event, documenting erosional and/or tectonic exhumation related
to the collapse of the Carpathian orogenic wedge. This is the first evidence that exhumation of crystalline cores in the Western
Carpathians took place in the Eocene and not in the Cretaceous as traditionally believed. Bimodal AFT length distributions,
Early Miocene AHe ages and thermal modelling results suggest that the samples were heated to temperatures of ~55–90°C during
Oligocene–Miocene times. This thermal event may be related either to the Oligocene/Miocene sedimentary burial, or Miocene
magmatic activity and increased heat flow. This finding supports the concept of thermal instability of the Carpathian crystalline
bodies during the post-Eocene period. 相似文献
70.